Rodolfo A. Jalabert

Environment-Independent Decoherence Rate in Classically Chaotic Systems

We study the decoherence of a one-particle system, whose classical correspondent is chaotic, when it evolves coupled to a weak quenched environment. This is done by analytical evaluation of the Loschmidt echo (i.e., the revival of a localized density excitation upon reversal of its time evolution), in the presence of the perturbation. We predict an exponential decay for the Loschmidt echo with a (decoherence) rate which is asymptotically given by the mean Lyapunov exponent of the classical system, and therefore independent of the perturbation strength, within a given range of strengths. Our results are consistent with recent experiments of polarization echoes in nuclear magnetic resonance and numerical simulations.

Universal quantum signatures of chaos in ballistic transport

The conductance of a ballistic quantum dot (having chaotic classical dynamics and being coupled by ballistic point contacts to two electron reservoirs) is computed on the single assumption that its scattering matrix is a member of Dysons circular ensemble. General formulae are obtained for the mean and variance of transport properties in the orthogonal (β = 1), unitary (β = 2), and symplectic (β = 4) symmetry class. Applications include universal conductance fluctuations, weak localization, sub-Poissonian shot noise, and normal-metal-superconductor junctions. The complete distribution P(g) of the conductance g is computed for the case that the coupling to the reservoirs occurs via two quantum point contacts with a single transmitted channel. The result P(g) ∝ g−1 + β/2 is qualitatively different in the three symmetry classes.

Weak localization and integrability in ballistic cavities.

We demonstrate the existence of an interference contribution to the average magnetoconductance, G(B), of ballistic cavities and use it to test the semiclassical theory of quantum billiards. G(B) is qualitatively different for chaotic and regular cavities (saturation versus linear increase) which is explained semiclassically by the differing classical distribution of areas. The magnitude of G(B) is poorly explained by the semiclassical theory of coherent backscattering (elastic enhancement factor); interference between trajectories which are not exactly time reversed must be included

Quantum-chaotic scattering effects in semiconductor microstructures.

We show that classical chaotic scattering has experimentally measurable consequences for the quantum conductance of semiconductor microstructures. These include the existence of conductance fluctuations-a sensitivity of the conductance to either Fermi energy or magnetic field-and weak-localization-a change in the average conductance upon applying a magnetic field. We develop a semiclassical theory and present numerical results for these two effects in which we model the microstructures by billiards attached to leads. We find that the difference between chaotic and regular classical scattering produces a qualitative difference in the fluctuation spectrum and weak-localization lineshape of chaotic and nonchaotic structures. While the semiclassical theory within the diagonal approximation accounts well for the weak-localization lineshape and for the spectrum of the fluctuations, we uncover a surprising failure of the semiclassical diagonal-approximation theory in describing the magnitude of these quantum transport effects.

ORBITAL MAGNETISM IN THE BALLISTIC REGIME: GEOMETRICAL EFFECTS

Abstract We present a general semiclassical theory of the orbital magnetic response of noninteracting electrons confined in two-dimensional potentials. We calculate the magnetic susceptibility of singly-connected and the persistent currents of multiply connected geometries. We concentrate on the geometric effects by studying confinement by perfect (disorder free) potentials stressing the importance of the underlying classical dynamics. We demonstrate that in a constrained geometry the standard Landau diamagnetic response is always present, but is dominated by finite-size corrections of a quasi-random sign which may be orders of magnitude larger. These corrections are very sensitive to the nature of the classical dynamics. Systems which are integrable at zero magnetic field exhibit larger magnetic response than those which are chaotic. This difference arises from the large oscillations of the density of states in integrable systems due to the existence of families of periodic orbits. The connection between quantum and classical behavior naturally arises from the use of semiclassical expansions. This key tool becomes particularly simple and insightful at finite temperature, where only short classical trajectories need to be kept in the expansion. In addition to the general theory for integrable systems, we analyze in detail a few typical examples of experimental relevance: circles, rings and square billiards. In the latter, extensive numerical calculations are used as a check for the success of the semiclassical analysis. We study the weak-field regime where classical trajectories remain essentially unaffected, the intermediate field regime where we identify new oscillations characteristic for ballistic mesoscopic structures, and the high-field regime where the typical de Haas-van Alphen oscillations exhibit finite-size corrections. We address the comparison with experimental data obtained in high-mobility semiconductor microstructures discussing the differences between individual and ensemble measurements, and the applicability of the present model.

Lifetime of the first and second collective excitations in metallic nanoparticles

We determine the lifetime of the surface plasmon in metallic nanoparticles under various conditions, concentrating on the Landau damping, which is the dominant mechanism for intermediate-size particles. Besides the main contribution to the lifetime, which smoothly increases with the size of the particle, our semiclassical evaluation yields an additional oscillating component. For the case of noble metal particles embedded in a dielectric medium, it is crucial to consider the details of the electronic confinement; we show that in this case the lifetime is determined by the shape of the self-consistent potential near the surface. Strong enough perturbations may lead to the second collective excitation of the electronic system. We study its lifetime, which is limited by two decay channels: Landau damping and ionization. We determine the size dependence of both contributions and show that the second collective excitation remains as a well defined resonance.

Oscillatory size dependence of the surface plasmon linewidth in metallic nanoparticles

We study the linewidth of the surface plasmon resonance in the optical absorption spectrum of metallic nanoparticles, when the decay into electron-hole pairs is the dominant channel. Within a semiclassical approach, we find that the electron-hole density-density correlation oscillates as a function of the size of the particles, leading to oscillations of the linewidth. This result is confirmed numerically for alkali and noble-metal particles. While the linewidth can increase strongly, the oscillations persist when the particles are embedded in a matrix.

Surface plasmon in metallic nanoparticles: Renormalization effects due to electron-hole excitations

Received 15 May 2006; revised manuscript received 25 August 2006; published 26 October 2006 The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the surface plasmon resonance. A redshift with respect to the classical Mie frequency appears in addition to the one caused by the spill out of the electronic density outside the nanoparticle. We characterize the spill-out effect by means of a semiclassical expansion and obtain its dependence on temperature and the size of the nanoparticle. We demonstrate that both, the spill-out and the environment-induced shift are necessary to explain the experimentally observed frequencies and confirm our findings by time-dependent local density approximation calculations of the resonance frequency. The size and temperature dependence of the environmental influence results in a qualitative agreement with pump-probe spectroscopic measurements of the differential light transmission.

From the Fermi glass towards the Mott insulator in one dimension: Delocalization and strongly enhanced persistent currents

When a system of spinless fermions in a disordered mesoscopic ring becomes instable between the inhomogeneous configuration driven by the random potential (Anderson insulator) and the homogeneous one driven by repulsive interactions (Mott insulator), the persistent current can be enhanced by orders of magnitude. This is illustrated by a study of the change of the ground state energy under twisted boundary conditions using the density matrix renormalization group algorithm.

Universality of the Lyapunov regime for the Loschmidt echo

The Loschmidt echo (LE) is a magnitude that measures the sensitivity of quantum dynamics to perturbations in the Hamiltonian. For a certain regime of the parameters, the LE decays exponentially with a rate given by the Lyapunov exponent of the underlying classically chaotic system. We develop a semiclassical theory, supported by numerical results in a Lorentz gas model, which allows us to establish and characterize the universality of this Lyapunov regime. In particular, the universality is evidenced by the semiclassical limit of the de Broglie wavelength going to zero, the behavior for times longer than Ehrenfest time, the insensitivity with respect to the form of the perturbation, and the behavior of individual (nonaveraged) initial conditions. Finally, by elaborating a semiclassical approximation to the Wigner function, we are able to distinguish between classical and quantum origin for the different terms of the LE. This approach renders an understanding for the persistence of the Lyapunov regime after the Ehrenfest time, as well as a reinterpretation of our results in terms of the quantum-classical transition.