Romain Pierrat

Theory of the time reversal cavity for electromagnetic fields

We derive a general expression of the electric dyadic Green function in a time-reversal cavity, based on vector diffraction theory in the frequency domain. Our theory gives a rigorous framework to time-reversal experiments using electromagnetic waves and suggests a methodology to design structures generating subwavelength focusing after time reversal.

Photon diffusion coefficient in scattering and absorbing media.

We present a unified derivation of the photon diffusion coefficient for both steady-state and time-dependent transport in disordered absorbing media. The derivation is based on a modal analysis of the time-dependent radiative transfer equation. This approach confirms that the dynamic diffusion coefficient is given by the random-walk result D = cl(*)/3, where l(*) is the transport mean free path and c is the energy velocity, independent of the level of absorption. It also shows that the diffusion coefficient for steady-state transport, often used in biomedical optics, depends on absorption, in agreement with recent theoretical and experimental works. These two results resolve a recurrent controversy in light propagation and imaging in scattering media.

Subwavelength focusing inside an open disordered medium by time reversal at a single point antenna

We study theoretically light focusing at subwavelength scale inside a disordered strongly scattering open medium. We show that broadband time reversal at a single point antenna, in conjunction with near-field interactions and multiple scattering, produces spatial focusing with a quality comparable to that obtained in an ideal closed cavity. This gives new perspectives for super-resolved optical imaging and coherent control of single nanosources or absorbers in complex media.

High-density hyperuniform materials can be transparent

We show that materials made of scatterers distributed on a stealth hyperuniform point pattern can be transparent at densities for which an uncorrelated disordered material would be opaque due to multiple scattering. The conditions for transparency are analyzed using numerical simulations, and an explicit criterion is found based on a perturbative theory. The broad applicability of the concept offers perspectives for various applications in photonics, and more generally in wave physics.

Spatial coherence in complex photonic and plasmonic systems.

The concept of cross density of states characterizes the intrinsic spatial coherence of complex photonic or plasmonic systems, independently of the illumination conditions. Using this tool and the associated intrinsic coherence length, we demonstrate unambiguously the spatial squeezing of eigenmodes on disordered fractal metallic films, thus clarifying a basic issue in plasmonics.

Strong coupling to two-dimensional Anderson localized modes.

We use a scattering formalism to derive a condition of strong coupling between a resonant scatterer and an Anderson localized mode for electromagnetic waves in two dimensions. The strong coupling regime is demonstrated based on exact numerical simulations, in perfect agreement with theory. The strong coupling threshold can be expressed in terms of the Thouless conductance and the Purcell factor. This connects key concepts in transport theory and cavity quantum electrodynamics, and provides a practical tool for the design or analysis of experiments.

Subwavelength focusing in bubbly media using broadband time reversal

Thanks to a Multiple Scattering Theory algorithm, we present a way to focus energy at the deep subwavelength scale, from the far-field, inside a cubic disordered bubble cloud by using broadband Time Reversal (TR). We show that the analytical calculation of an effective wavenumber performing the Independant Scattering Approximation (ISA) matches the numerical results for the focal extension. Subwavelength focusings of λ/100 are reported for simulations with perfect bubbles (no loss). A more realistic case, with viscous and thermal losses, allows us to obtain a λ/14 focal spot, with a low volume fraction of scatterers (Φ = 10−2). Bubbly materials could open new perspective for acoustic actuation in the microfluidic context.

Towards a full characterization of a plasmonic nanostructure with a fluorescent near-field probe

We report on the experimental and theoretical study of the spatial fluctuations of the local density of states (EM-LDOS) and of the fluorescence intensity in the near-field of a gold nanoantenna. EM-LDOS, fluorescence intensity and topography maps are acquired simultaneously by scanning a fluorescent nanosource grafted on the tip of an atomic force microscope at the surface of the sample. The results are in good quantitative agreement with numerical simulations. This work paves the way for a full near-field characterization of an optical nanoantenna.

Light propagation in multilayered scattering media beyond the diffusive regime.

We describe a method to solve the radiative transfer equation (RTE) in multilayered geometry with index mismatch and demonstrate its potential for modeling light propagation in biological systems. The method is compared to Monte Carlo simulations with high accuracy but is much more efficient in terms of computer time. We illustrate the potential of the method by studying a multilayered system containing a weakly scattering layer surrounded by highly scattering layers, with anisotropic scattering and index mismatched interfaces. The calculation of directional transmitted fluxes has shown that the RTE method can be used to calculate relevant quantities in realistic systems in the presence of non-diffusive behavior.

Mapping the Radiative and the Apparent Nonradiative Local Density of States in the Near Field of a Metallic Nanoantenna

We present a novel method to extract the various contributions to the photonic local density of states from near-field fluorescence maps. The approach is based on the simultaneous mapping of the fluorescence intensity and decay rate, and on the rigorous application of the reciprocity theorem. It allows us to separate the contributions of the radiative and the apparent non-radiative local density of states to the change in the decay rate. The apparent non-radiative contribution accounts for losses due to radiation out of the detection solid angle and to absorption in the environment. Data analysis relies on a new analytical calculation, and does not require the use of numerical simulations. One of the most relevant applications of the method is the characterization of nanostructures aimed at maximizing the number of photons emitted in the detection solid angle, which is a crucial issue in modern nanophotonics.