Rose Ahlefeldt

Coherence time of over a second in a telecom-compatible quantum memory storage material

A candidate for efficient broadband quantum memory at telecommunication wavelengths is identified. The long coherence time and the efficient optical spin pumping demonstrated in the experiment make it practical for spin-wave storage.

Optical memory bandwidth and multiplexing capacity in the erbium telecommunication window

We study the bandwidth and multiplexing capacity of an erbium-doped optical memory for quantum storage purposes. We concentrate on the protocol ROSE (Revival of a Silenced Echo) because it has the largest potential multiplexing capacity. Our analysis is applicable to other protocols that involve strong optical excitation. We show that the memory performance is limited by instantaneous spectral diffusion and we describe how this effect can be minimised to achieve optimal performance.

Method for assigning satellite lines to crystallographic sites in rare-earth crystals

We describe an experimental technique for associating the satellite lines in a rare earth optical spectrum caused by a defect with the rare earth ions in crystal sites around that defect. This method involves measuring the hyperfine splitting caused by a magnetic dipole-dipole interaction between host ions and a magnetic defect. The method was applied to Ce3+:EuCl3.6H2O to assign 13 of the outermost 22 satellite lines to sites. The assignments show that the optical shift of a satellite line is loosely dependent on the distance to the dopant. The interaction between host and dopant ions is purely dipole-dipole at distances greater than 7 Angstroms, with an additional contribution, likely superexchange, at distances less than 7 Angstroms.

Quantum state transfer through time reversal of an optical channel

Rare earth ions have exceptionally long coherence times, making them an excellent candidate for quantum information processing. A key part of this processing is quantum state transfer. We demonstrate that high fidelity quantum state transfer between two ensembles of rare earth ions can be achieved by time reversing the connecting optical quantum channel, and suggest using a gradient echo memory to perform this time reversal. We demonstrate that the superradiant coupling between the ensemble of ions and an intermediate cavity coupled to the optical channel can lead to higher transfer fidelities than would otherwise be possible with an individual ion. We suggest increasing the size of the ensemble can overcome unwanted loss and decoherence processes that reduce the transfer fidelity.

Optical measurement of heteronuclear cross-relaxation interactions in Tm:YAG

We investigate cross-relaxation interactions between Tm and Al in Tm:YAG using two optical methods: spectral holeburning and stimulated echoes. These interactions lead to a reduction in the hyperfine lifetime at magnetic fields that bring the Tm hyperfine transition into resonance with an Al transition. We develop models for measured echo decay curves and holeburning spectra near a resonance, which are used to show that the Tm-Al interaction has a resonance width of 10~kHz and reduces the hyperfine lifetime to 0.5 ms. The antihole structure is consistent with an interaction dominated by the Al nearest neighbors at 3.0 Angstroms, with some contribution from the next nearest neighbors at 3.6 Angstroms.

Characterisation of EuCl 3 .6H 2 O for multi-qubit quantum processing

We describe a quantum computing architecture that uses satellite lines in rare earth doped EuCl3.6H2O as qubits. The crystallographic sites to which these lines belong are identified and this information is used to predict the performance of the quantum computing system.