S. Hossein Mousavi

Photonic topological insulators

We review the recent progress on the first experimental demonstration of photonic topological insulators, along with a variety of new ideas associated with it.Recent progress in understanding the topological pr operties of condensed matter has led to the discove ry of time-reversal invariant topological insulators. Because of limitations imposed by nature, topologi cally non-trivial electronic order seems to be uncommon e xcept in small-band-gap semiconductors with strong spin-orbit interactions. In this Article we show t ha artificial electromagnetic structures, known as metamaterials, provide an attractive platform for d esigning photonic analogues of topological insulato rs. We demonstrate that a judicious choice of the metam a erial parameters can create photonic phases that support a pair of helical edge states, and that the se edge states enable one-way photonic transport th at is robust against disorder.

Seeing protein monolayers with naked eye through plasmonic Fano resonances

We introduce an ultrasensitive label-free detection technique based on asymmetric Fano resonances in plasmonic nanoholes with far reaching implications for point-of-care diagnostics. By exploiting extraordinary light transmission phenomena through high-quality factor (Qsolution ∼ 200) subradiant dark modes, we experimentally demonstrate record high figures of merits (FOMs as high as 162) for intrinsic detection limits surpassing that of the gold standard prism coupled surface-plasmon sensors (Kretschmann configuration). Our experimental record high sensitivities are attributed to the nearly complete suppression of the radiative losses that are made possible by the high structural quality of the fabricated devices as well as the subradiant nature of the resonances. Steep dispersion of the plasmonic Fano resonance profiles in high-quality plasmonic sensors exhibit dramatic light intensity changes to the slightest perturbations within their local environment. As a spectacular demonstration of the extraordinary sensitivity and the quality of the fabricated biosensors, we show direct detection of a single monolayer of biomolecules with naked eye using these Fano resonances and the associated Wood’s anomalies. To fabricate high optical-quality sensors, we introduce a high-throughput lift-off free evaporation fabrication technique with extremely uniform and precisely controlled nanofeatures over large areas, leading to resonance line-widths comparable to that of the ideally uniform structures as confirmed by our time-domain simulations. The demonstrated label-free sensing platform offers unique opportunities for point-of-care diagnostics in resource poor settings by eliminating the need for fluorescent labeling and optical detection instrumentation (camera, spectrometer, etc.) as well as mechanical and light isolation.

Improved Electrical Conductivity of Graphene Films Integrated with Metal Nanowires

Polycrystalline graphene grown by chemical vapor deposition (CVD) on metals and transferred onto arbitrary substrates has line defects and disruptions such as wrinkles, ripples, and folding that adversely affect graphene transport properties through the scattering of the charge carriers. It is found that graphene assembled with metal nanowires (NWs) dramatically decreases the resistance of graphene films. Graphene/NW films with a sheet resistance comparable to that of the intrinsic resistance of graphene have been obtained and tested as a transparent electrode replacing indium tin oxide films in electrochromic (EC) devices. The successful integration of such graphene/NW films into EC devices demonstrates their potential for a wide range of optoelectronic device applications.

Inductive Tuning of Fano-Resonant Metasurfaces Using Plasmonic Response of Graphene in the Mid-Infrared

Graphene is widely known for its anomalously strong broadband optical absorptivity of 2.3% that enables seeing its single-atom layer with the naked eye. However, in the mid-infrared part of the spectrum graphene represents a quintessential lossless zero-volume plasmonic material. We experimentally demonstrate that, when integrated with Fano-resonant plasmonic metasurfaces, single-layer graphene (SLG) can be used to tune their mid-infrared optical response. SLGs plasmonic response is shown to induce large blue shifts of the metasurfaces resonance without reducing its spectral sharpness. This effect is explained by a generalized perturbation theory of SLG-metamaterial interaction that accounts for two unique properties of the SLG that set it apart from all other plasmonic materials: its anisotropic response and zero volume. These results pave the way to using gated SLG as a platform for dynamical spectral tuning of infrared metamaterials and metasurfaces.

Topologically robust sound propagation in an angular-momentum-biased graphene-like resonator lattice

Topological insulators do not allow conduction in the bulk, yet they support edge modes that travel along the boundary only in one direction, determined by the carried electron spin, with inherent robustness to defects and disorder. Topological insulators have inspired analogues in photonics and optics, in which one-way edge propagation in topologically protected two-dimensional materials is achieved breaking time-reversal symmetry with a magnetic bias. Here, we introduce the concept of topological order in classical acoustics, realizing robust topological protection and one-way edge propagation of sound in a suitably designed resonator lattice biased with angular momentum, forming the acoustic analogue of a magnetically biased graphene layer. Extending the concept of an acoustic nonreciprocal circulator based on angular-momentum bias, time-reversal symmetry is broken here using moderate rotational motion of air within each element of the lattice, which takes the role of the electron spin in determining the direction of modal edge propagation.

Topologically protected elastic waves in phononic metamaterials

Surface waves in topological states of quantum matter exhibit unique protection from backscattering induced by disorders, making them ideal carriers for both classical and quantum information. Topological matters for electrons and photons are largely limited by the range of bulk properties, and the associated performance trade-offs. In contrast, phononic metamaterials provide access to a much wider range of material properties. Here we demonstrate numerically a phononic topological metamaterial in an elastic-wave analogue of the quantum spin Hall effect. A dual-scale phononic crystal slab is used to support two effective spins for phonons over a broad bandwidth, and strong spin–orbit coupling is realized by breaking spatial mirror symmetry. By preserving the spin polarization with an external load or spatial symmetry, phononic edge states are shown to be robust against scattering from discrete defects as well as disorders in the continuum, demonstrating topological protection for phonons in both static and time-dependent regimes.

Robust reconfigurable electromagnetic pathways within a photonic topological insulator

The discovery of topological photonic states has revolutionized our understanding of electromagnetic propagation and scattering. Endowed with topological robustness, photonic edge modes are not reflected from structural imperfections and disordered regions. Here we demonstrate robust propagation along reconfigurable pathways defined by synthetic gauge fields within a topological photonic metacrystal. The flow of microwave radiation in helical edge modes following arbitrary contours of the synthetic gauge field between bianisotropic metacrystal domains is unimpeded. This is demonstrated in measurements of the spectrum of transmission and time delay along the topological domain walls. These results provide a framework for freely steering electromagnetic radiation within photonic structures.

Three-Dimensional All-Dielectric Photonic Topological Insulator

The theoretical study of a 3D photonic topological metacrystal based on an all-dielectric metamaterial platform shows robust propagation of surface states along 2D domain walls, making it a promising solution for photonics applications. The proposed metacrystal design might also open the way for the observation of elusive fundamental physical phenomena.

Optical properties of Fano-resonant metallic metasurfaces on a substrate

Three different periodic optical metasurfaces exhibiting Fano resonances are studied in mid-IR frequency range in the presence of a substrate. We develop a rigorous semi-analytical technique and calculate how the presence of a substrate affects optical properties of these structures. An analytical minimal model based on the truncated exact technique is introduced and is shown to provide a simple description of the observed behavior. We demonstrate that the presence of a substrate substantially alters the collective response of the structures suppressing Woods anomalies and spatial dispersion of the resonances. Different types of Fano resonances are found to be affected differently by the optical contrast between the substrate and the superstrate. The dependence of the spectral position of the resonances on the substrate/superstrate permittivities is studied and the validity of the widely used effective medium approaches is re-examined.

Applying alloyed metal nanoparticles to enhance solar assisted water splitting

Considering hydrogen as a future fuel, development of clean approaches based on solar energy conversion is the main human challenge. Here, for the first time, TiO2 photoanodes are decorated with Au–Ag alloy nanoparticles for efficient photoelectrochemical water splitting. The photoanodes were synthesized using a one-step co-sputtering method. The single surface plasmon resonance peak at 540 nm and also the observed shifts in photoelectron binding energies are fingerprints of homogenous alloyed nanoparticles. Scanning electron microscopy revealed the formation of nearly 40 nm particles on the surface, which was also verified by the simulation of the films optical absorption. Photocurrent measurements showed a 30% increase in the presence of alloy nanoparticles, as well as a 50% reduction in charge transfer resistance of the electrodes. These observations are attributed to adjusting a suitable Schottky barrier in the junction of TiO2/metal particles, which introduces applying alloy noble metallic particles as a new effective strategy for energy and environmental purposes.