S. Kazamias

A high-intensity highly coherent soft X-ray femtosecond laser seeded by a high harmonic beam

Synchrotrons have for decades provided invaluable sources of soft X-rays, the application of which has led to significant progress in many areas of science and technology. But future applications of soft X-rays—in structural biology, for example—anticipate the need for pulses with much shorter duration (femtoseconds) and much higher energy (millijoules) than those delivered by synchrotrons. Soft X-ray free-electron lasers should fulfil these requirements but will be limited in number; the pressure on beamtime is therefore likely to be considerable. Laser-driven soft X-ray sources offer a comparatively inexpensive and widely available alternative, but have encountered practical bottlenecks in the quest for high intensities. Here we establish and characterize a soft X-ray laser chain that shows how these bottlenecks can in principle be overcome. By combining the high optical quality available from high-harmonic laser sources (as a seed beam) with a highly energetic soft X-ray laser plasma amplifier, we produce a tabletop soft X-ray femtosecond laser operating at 10 Hz and exhibiting full saturation, high energy, high coherence and full polarization. This technique should be readily applicable on all existing laser-driven soft X-ray facilities.

Submicrometer digital in-line holographic microscopy at 32 nm with high-order harmonics

Soft-x-ray digital in-line microscopic holography is achieved using a fully coherent high-order harmonic source emitting at 32 nm. Combination of commercial-grade soft-x-ray optics and a back-illuminated CCD detector allows a compact and versatile holographic setup. Different experimental geometries have been tested by imaging calibrated 50 nm tips and 1 microm wires. Spatial resolution of 800 nm is measured with magnifications ranging from 30 to 110 and a numerical aperture around 0.01. Finally, the potentiality of three-dimensional numerical reconstruction from a single hologram acquisition is shown experimentally.

Compression of attosecond harmonic pulses by extreme-ultraviolet chirped mirrors

In the race toward attosecond pulses, for which high-order harmonics generated in rare gases are the best candidates, both the harmonic spectral range and the spectral phase have to be controlled. We demonstrate that multilayer extreme-ultraviolet chirped mirrors can be numerically optimized and designed to compensate for the intrinsic harmonic chirp that was recently discovered and that is responsible for temporal broadening of pulses. A simulation shows that an optimized mirror is capable of compressing the duration from approximately 260 to 90 as. This new technique is an interesting solution because of its ability to cover a wider spectral range than other technical devices that have already been proposed to overcome the chirp of high harmonics.

Design and characterization of extreme-ultraviolet broadband mirrors for attosecond science.

A novel multilayer mirror was designed and fabricated based on a recently developed three-material technology aimed both at reaching reflectivities of about 20% and at controlling dispersion over a bandwidth covering photon energies between 35 and 50 eV. The spectral phase upon reflection was retrieved by measuring interferences in a two-color ionization process using high-order harmonics produced from a titanium: sapphire laser. We demonstrate the feasibility of designing and characterizing phase-controlled broadband optics in the extreme-ultraviolet domain, which should facilitate the manipulation of attosecond pulses for applications.

Enhancement of high-order harmonic generation at tuned wavelengths through adaptive control

An adaptive learning loop enhances the efficiency and tuning of high-order harmonic generation. In comparison with simple chirp tuning, we observe a broader tuning range and a twofold to threefold enhancement in integrated photon flux in the cutoff region. The driving pulse temporal phase varies significantly for different tunings and is more complicated than a simple chirp. We compare our experimental results with a one-dimensional, time-dependent model that incorporates the intrinsic atomic response, the experimental pulse temporal phase, ionization effects, and transverse coherence of the spatial mode of the laser. The model agrees with our experimental results and indicates that a specific quantum path coupled with ionization effects determines the optimized harmonic spectrum.

Frequency chirp of harmonic and attosecond pulses

We study the phase of the atomic polarization in the process of high-order harmonic generation. Its dependence on the laser intensity and the harmonic order induce a frequency variation in time (chirp) respectively of the harmonic pulses and attosecond pulses. We review the recent experimental results on the temporal characterization of the harmonic emission and show that measurements performed using very different techniques (like XFROG and RABITT), probing the phase in different parameter spaces, can be connected through the mixed phase derivatives, demonstrating the common underlying physics.

Imaging and quality assessment of high-harmonic focal spots

We present a direct method of studying the focusability of an intense, short-pulse extreme-ultraviolet (XUV) beam obtained by high-harmonic generation. We perform near-field imaging of the focal spot of five high-harmonic orders strongly focused by a broadband toroidal mirror. To visualize the focal spot directly, we image the fluorescence induced by an XUV beam on a cerium-doped YAG crystal on a visible CCD camera. We can thus measure the harmonic spot size on a single image, together with the Strehl ratio, to evaluate the quality of focusing. Such techniques should become instrumental in optimizing the focusing conditions and reaching intensities required for exploring attosecond nonlinear optics in the XUV range.

Optimization toward a high-average-brightness soft-x-ray laser pumped at grazing incidence

We report the near-field imaging characterization of a 10 Hz Ni-like 18.9 nm molybdenum soft-x-ray laser pumped in a grazing incidence pumping (GRIP) geometry with a table-top laser driver. We investigate the effect of varying the GRIP angle on the spatial behavior of the soft-x-ray laser source. After multiparameter optimization, we were able to find conditions to generate routinely a high-repetition-rate soft-x-ray laser with an energy level of up to 3 microJ/pulse and to 6x10(17) photons/s/mm2/mrad2/(0.1% bandwidth) average brightness and 1x10(28) photons/s/mm2/mrad2/(0.1% bandwidth) peak brightness.

Optimization of the non-normal incidence, transient pumped plasma X-ray laser for laser spectroscopy and plasma diagnostics at the facility for antiproton and ion research (FAIR)

Intense and stable laser operation with Ni-like Zr and Ag was demonstrated at pump energies between 2 J and 5 J energy from the PHELIX pre-amplifier section. A novel single mirror focusing scheme for the TCE x-ray laser ~XRL! has been successfully implemented by the LIXAM0MBI0GSI collaboration under different pump geometries. This shows potential for an extension to shorter XRL wavelength. Generation of high quality XRL beams for XRL spectroscopy of highly charged ions is an important issue within the scientific program of PHELIX. Long range perspective is the study of nuclear properties of radioactive isotopes within the FAIR project.

Optimization of a tabletop high-repetition-rate soft x-ray laser pumped in double-pulse single-beam grazing incidence

This Letter reports on the optimization of a tabletop nickel-like molybdenum transient collisionally excited soft x-ray laser (SXRL) at 18.9 nm performed by a double-pulse single-beam grazing incidence pumping (DGRIP). This scheme allows for the first time, to our knowledge, the full control of the pump laser parameters including the pre-pulse duration optimally generating the SXRL amplifier under a grazing incidence. The single-beam geometry of the collinear double-pulse propagation guarantees the ideal overlap of the pre-pulse and main pulse from shot to shot resulting in a more efficient and highly stable SXRL output. SXRL energies up to 2.2 microJ are obtained with a total pump energy less than 1 J for several hours at a 10 Hz repetition rate without realignment under once optimized double pumping pulse parameters including energy ratio, time delay, pre-pulse and main pulse durations, and line focus width.