S. L. Chin

Ultrafast white-light continuum generation and self-focusing in transparent condensed media

We report an investigation of white-light continuum generation and self-focusing by 140-fs Ti:sapphire laser pulses in extended transparent media. It is found that continuum generation is triggered by self-focusing and that both phenomena depend on the medium’s bandgap. There is a bandgap threshold for continuum generation. Above that threshold the continuum’s width increases with increasing bandgap. Furthermore, the beam’s self-focal diameter is discontinuous across the threshold. To explain the observations a mechanism is proposed that involves multiphoton excitation of electrons into the conduction band at the self-focus; the generated free electrons cause spectral superbroadening and limit the self-focal diameter. The continuum beam’s surprisingly low divergence is then investigated and explained in terms of a Kerr lensing effect.

Moving focus in the propagation of ultrashort laser pulses in air

The long light filaments generated in air by powerful ultrashort laser pulses, previously attributed to self-channeling, were investigated by use of gigawatt pulses from a Ti:sapphire chirped-pulse-amplification laser system. A filament contained only a small fraction of the pulse energy and always ended at the diffraction length of the beam (~100 m), independently of the pulse energy. These features are explained by the moving-focus model, which is presented as an alternative to the self-channeling model. Computer simulations involving ionization of the air also support the moving-focus model.

Laser ionization of noble gases by Coulomb-barrier suppression

Laser ionization of noble gases was studied with a 1.053-μm, 1-psec Nd:glass laser. A systematic scan of intensities from mid-1013 W/cm2 to mid-1016 W/cm2 was performed, resulting in the production of charge states as high as Xe12+. Ionization occurs exclusively in the tunneling regime. We compare experimental ion production rates with those predicted by several different theories. Agreement between experimental ion-production curves and theoretical predictions is good for two theoretical models: (1) an elaboration of the Keldysh tunneling model, developed by Ammosov et al. [ Sov. Phys. JETP64, 1191 ( 1986)] and (2) a much more primitive model, based on Coulomb-barrier suppression, in which tunneling and other quantum-mechanical effects are ignored completely. The success of the more primitive model suggests that a new term, barrier-suppression ionization, rather than tunneling or multiphoton ionization, may be the most appropriate at this wavelength and in this range of intensities.

Femtosecond laser filamentation

Filamentation Physics.- Theory of Single Filamentation.- Multiple Filamentation.- Filamentation Nonlinear Optics: General.- Filamentation Nonlinear Optics: Third Harmonic Generation and Four-Wave-Mixing Inside a Filament.- Remote Sensing Using Filamentation.- Challenges Ahead.

Conical emission from laser–plasma interactions in the filamentation of powerful ultrashort laser pulses in air

We performed detailed experimental and numerical investigations of the conical emission (CE) accompanying the filamentation of powerful ultrashort laser pulses in air. It was found that the CE originates from self-phase modulation in the plasma produced by the pulse during propagation. The experiment and the simulation agree on the essential features of the CE: The CE angle decreases with increasing wavelength and is independent of the position along the filament, and there is no CE at Stokes-shifted wavelengths.

Intensity clamping of a femtosecond laser pulse in condensed matter

We measured the supercontinuum spectrum of an intense femtosecond Ti:sapphire laser pulse propagating in condensed optical media (water, chloroform and glass), at various input laser energies, below and above the threshold for filamentation of the laser pulse. It is found that the maximum positive frequency shift of the supercontinuum spectrum remains constant at pulse energies that generate single and mutiple filamentation. The constant shift is due to clamping of the peak intensity inside the filaments.

White-light continuum generation and filamentation during the propagation of ultra-short laser pulses in air

Abstract We present numerical results on the propagation of femtosecond pulses in air including multiphoton ionization, group-velocity dispersion, space–time focusing, self-steepening, Raman response, and higher-order χ (5) defocusing. It is shown that the self-steepening terms cause strong blue shifting of the spectrum generating a white-light continuum. Our results are in good qualitative agreement with experimental observations.

Direct measurement of the critical power of femtosecond Ti:sapphire laser pulse in air

We report a simple experiment to directly determine the critical power for self-focusing in air by measuring the focal shift of the focused femtosecond Ti:sapphire laser pulses. The measured critical power is 10 GW for the 42 fs laser pulse; it gradually decreases to 5 GW for (chirped) pulse duration longer than 200 fs.

Re-focusing during the propagation of a focused femtosecond Ti:Sapphire laser pulse in air

Abstract The dependence of the intensity of a focused Ti:Sapphire laser pulse in air on the propagation distance was studied by measuring the photo-emission spectrum of N 2 and N 2 + . Refocusing was observed directly that agrees with the predictions put forward by Mlejnek et al. [M. Mlejnek, E.M. Wright, J.V. Moloney, Opt. Lett. 23 (1998) 382].

Advances in intense femtosecond laser filamentation in air

This is a review of some recent development in femtosecond filamentation science with emphasis on our collective work. Previously reviewed work in the field will not be discussed. We thus start with a very brief description of the fundamental physics of single filamentation of powerful femtosecond laser pulses in air. Intensity clamping is emphasized. One consequence is that the peak intensity inside one or more filaments would not increase significantly even if one focuses the pulse at very high peak power even up to the peta-watt level. Another is that the clamped intensity is independent of pressure. One interesting outcome of the high intensity inside a filament is filament fusion which comes from the nonlinear change of index of refraction inside the filament leading to cross beam focusing. Because of the high intensity inside the filament, one can envisage nonlinear phenomena taking place inside a filament such as a new type of Raman red shift and the generation of very broad band supercontinuum into the infrared through four-wave-mixing. This is what we call by filamentation nonlinear optics. It includes also terahertz generation from inside the filament. The latter is discussed separately because of its special importance to those working in the field of safety and security in recent years. When the filamenting pulse is linearly polarized, the isotropic nature of air becomes birefringent both electronically (instantaneous) and through molecular wave packet rotation and revival (delayed). Such birefringence is discussed in detailed. Because, in principle, a filament can be projected to a long distance in air, applications to pollution measurement as well as other atmospheric science could be earned out. We call this filamentation atmospheric science. Thus, the following subjects are discussed briefly, namely, lightning control, rain making, remote measurement of electric field, microwave guidance and remote sensing of pollutants. A discussion on the higher order Kerr effect on the physics of filamentation is also given. This is a new hot subject of current debate. This review ends on giving our view of the prospect of progress of this field of filamentation in the future. We believe it hinges upon the development of the laser technology based upon the physical understanding of filamentation and on the reduction in price of the laser system.