S. N. Liddick

Half-life of the doubly magic r-process nucleus 78Ni.

Nuclei with magic numbers serve as important benchmarks in nuclear theory. In addition, neutron-rich nuclei play an important role in the astrophysical rapid neutron-capture process (r process). 78Ni is the only doubly magic nucleus that is also an important waiting point in the r process, and serves as a major bottleneck in the synthesis of heavier elements. The half-life of 78Ni has been experimentally deduced for the first time at the Coupled Cyclotron Facility of the National Superconducting Cyclotron Laboratory at Michigan State University, and was found to be 110(+100)(-60) ms. In the same experiment, a first half-life was deduced for 77Ni of 128(+27)(-33) ms, and more precise half-lives were deduced for 75Ni and 76Ni of 344(+20)(-24) ms and 238(+15)(-18) ms, respectively.

Structure of 52,54Ti and shell closures in neutron-rich nuclei above 48Ca

Abstract The level structure of 5422Ti32 has been explored for the first time by combining β-decay measurements from fragmentation products with prompt γ-ray spectroscopy following deep inelastic reactions. The latter technique was also instrumental in tracing 52Ti30 to higher spin. The data provide new tests of effective interactions for full pf-shell calculations in neutron-rich nuclei above 48Ca. The data indicate the presence of a significant subshell gap at N=32 and comparisons between theory and experiment suggest an additional shell closure at N=34 in Ca and Ti isotopes.

Orbital dependent nucleonic pairing in the lightest known isotopes of tin

By studying the (109)Xe→(105)Te→(101)Sn superallowed α-decay chain, we observe low-lying states in (101)Sn, the one-neutron system outside doubly magic (100)Sn. We find that the spins of the ground state (J=7/2) and first excited state (J=5/2) in (101)Sn are reversed with respect to the traditional level ordering postulated for (103)Sn and the heavier tin isotopes. Through simple arguments and state-of-the-art shell-model calculations we explain this unexpected switch in terms of a transition from the single-particle regime to the collective mode in which orbital-dependent pairing correlations dominate.

Half-lives and branchings for {beta}-delayed neutron emission for neutron-rich Co-Cu isotopes in the r-process

The {beta} decays of very neutron-rich nuclides in the Co-Zn region were studied experimentally at the National Superconducting Cyclotron Laboratory using the NSCL {beta}-counting station in conjunction with the neutron detector NERO. We measured the branchings for {beta}-delayed neutron emission (P{sub n} values) for {sup 74}Co (18{+-}15%) and {sup 75-77}Ni (10{+-}2.8%, 14{+-}3.6%, and 30{+-}24%, respectively) for the first time, and remeasured the P{sub n} values of {sup 77-79}Cu, {sup 79,81}Zn, and {sup 82}Ga. For {sup 77-79}Cu and for {sup 81}Zn we obtain significantly larger P{sub n} values compared to previous work. While the new half-lives for the Ni isotopes from this experiment had been reported before, we present here in addition the first half-life measurements of {sup 75}Co (30{+-}11 ms) and {sup 80}Cu (170{sub -50}{sup +110} ms). Our results are compared with theoretical predictions, and their impact on various types of models for the astrophysical rapid neutron-capture process (r-process) is explored. We find that with our new data, the classical r-process model is better able to reproduce the A=78-80 abundance pattern inferred from the solar abundances. The new data also influence r-process models based on the neutrino-driven high-entropy winds in core collapse supernovae.

Novel technique for constraining r -process (n, γ) reaction rates

A novel technique has been developed, which will open exciting new opportunities for studying the very neutron-rich nuclei involved in the r process. As a proof of principle, the γ spectra from the β decay of ^{76}Ga have been measured with the SuN detector at the National Superconducting Cyclotron Laboratory. The nuclear level density and γ-ray strength function are extracted and used as input to Hauser-Feshbach calculations. The present technique is shown to strongly constrain the ^{75}Ge(n,γ)^{76}Ge cross section and reaction rate.

Classical-NOVA CONTRIBUTION to the Milky Way's ²⁶Al abundance: exit channel of the key ²⁵Al(p,γ) ²⁶Si resonance.

Classical novae are expected to contribute to the 1809-keV Galactic γ-ray emission by producing its precursor 26Al, but the yield depends on the thermonuclear rate of the unmeasured 25Al(p,γ)26Si reaction. Using the β decay of 26P to populate the key J(π)=3(+) resonance in this reaction, we report the first evidence for the observation of its exit channel via a 1741.6±0.6(stat)±0.3(syst)  keV primary γ ray, where the uncertainties are statistical and systematic, respectively. By combining the measured γ-ray energy and intensity with other experimental data on 26Si, we find the center-of-mass energy and strength of the resonance to be E(r)=414.9±0.6(stat)±0.3(syst)±0.6(lit.)  keV and ωγ=23±6(stat)(-10)(+11)(lit.)  meV, respectively, where the last uncertainties are from adopted literature data. We use hydrodynamic nova simulations to model 26Al production showing that these measurements effectively eliminate the dominant experimental nuclear-physics uncertainty and we estimate that novae may contribute up to 30% of the Galactic 26Al.

Beta decay studies of nuclei near 32Mg: Investigating the ν(f7/2)-(d3/2) inversion at the N = 20 shell closure

Abstract 32 Mg lies within a region of deformed nuclei commonly referred to as the “island of inversion”. The β decay of 33 Al and 33 Mg has been studied to learn about nuclear structure near 32 Mg. Decay curves and precise half-life measurements are presented for both species. Gamma-ray spectra from correlated 33 Al decay events are also presented. The β -decay properties of 33 Al are shown to be well-described by an sd shell model calculation, suggesting that the ground state of 33 Al lies primarily outside the island of inversion.

Probing Shell Structure and Shape Changes in Neutron-Rich Sulfur Isotopes through Transient-Field g-Factor Measurements on Fast Radioactive Beams of 38S and 40S

The shell structure underlying shape changes in neutron-rich nuclei near N = 28 has been investigated by a novel application of the transient-field technique to measure the first-excited-state g factors in 38S and 40S produced as fast radioactive beams. There is a fine balance between proton and neutron contributions to the magnetic moments in both nuclei. The g factor of deformed 40S does not resemble that of a conventional collective nucleus because spin contributions are more important than usual.

Experimental Neutron Capture Rate Constraint Far from Stability

Nuclear reactions where an exotic nucleus captures a neutron are critical for a wide variety of applications, from energy production and national security, to astrophysical processes, and nucleosynthesis. Neutron capture rates are well constrained near stable isotopes where experimental data are available; however, moving far from the valley of stability, uncertainties grow by orders of magnitude. This is due to the complete lack of experimental constraints, as the direct measurement of a neutron-capture reaction on a short-lived nucleus is extremely challenging. Here, we report on the first experimental extraction of a neutron capture reaction rate on ^{69}Ni, a nucleus that is five neutrons away from the last stable isotope of Ni. The implications of this measurement on nucleosynthesis around mass 70 are discussed, and the impact of similar future measurements on the understanding of the origin of the heavy elements in the cosmos is presented.

Shell structure underlying the evolution of quadrupole collectivity in 38 S and 40 S probed by transient-field g-factor measurements on fast radioactive beams

The shell structure underlying shape changes in neutron-rich nuclei between N=20 and N=28 has been investigated by a novel application of the transient field technique to measure the first-excited state g factors in {sup 38}S and {sup 40}S produced as fast radioactive beams. Details of the new methodology are presented. In both {sup 38}S and {sup 40}S there is a fine balance between the proton and neutron contributions to the magnetic moments. Shell-model calculations that describe the level schemes and quadrupole properties of these nuclei also give a satisfactory explanation of the g factors. In {sup 38}S the g factor is extremely sensitive to the occupation of the neutron p{sub 3/2} orbit above the N=28 shell gap as occupation of this orbit strongly affects the proton configuration. The g factor of deformed {sup 40}S does not resemble that of a conventional collective nucleus because spin contributions are more important than usual.