Sabih Khan

Characterizing ultrabroadband attosecond lasers.

Recent progress in sub-laser-cycle gating of high-order harmonic generation promises to push the limits on optical pulse durations below the atomic unit of time, 24 as, which corresponds to a bandwidth broader than 75 eV. However, the available techniques for attosecond pulse measurement are valid only for narrow-bandwidth spectra, due to one of the key approximations made in the phase retrieval. Here we report a new technique for characterizing attosecond pulses, whereby the spectral phase of the attosecond pulse is extracted from the oscillation component with the dressing laser frequency in the photoelectron spectrogram. This technique, termed PROOF (Phase Retrieval by Omega Oscillation Filtering), can be applied to characterizing attosecond pulses with ultrabroad bandwidths.

Extreme ultraviolet supercontinua supporting pulse durations of less than one atomic unit of time

Double optical gating of high-harmonic generation was used to obtain supercontinuous spectra in the extreme UV (XUV) region including the water window. The spectra supported a 16 as pulse duration that is below one atomic unit of time (24 as). The dependence of the gated spectra on the carrier-envelope phase of the laser provided evidence that isolated attosecond pulses were generated. In addition, to ensure the temporal coherence of the XUV light, the pulse shape and phase of isolated 107 as XUV pulses using a portion of the spectrum were characterized by attosecond streaking.

Generation of continuum high-order harmonics from carbon plasma using double optical gating

We demonstrated continuum high-order harmonics from carbon plasma using the double optical gating method. The extreme ultraviolet continuum covered 17‐25 eV. The observation of such continuum is the first step towards the generation of high-flux single attosecond pulses from plasma harmonics. (Some figures may appear in colour only in the online journal)

Practical issues of retrieving isolated attosecond pulses

The attosecond streaking technique is used for the characterization of isolated extreme ultraviolet (XUV) attosecond pulses. This type of measurement suffers from low photoelectron counts in the streaked spectrogram, and is thus susceptible to shot noise. For the retrieval of few- or mono-cycle attosecond pulses, high-intensity streaking laser fields are required, which cause the energy spectrum of above-threshold ionized (ATI) electrons to overlap with that of the streaked photoelectrons. It is found by using the principal component generalized projections algorithm that the XUV attosecond pulse can accurately be retrieved for simulated and experimental spectrograms with a peak value of 50 or more photoelectron counts. Also, the minimum streaking intensity is found to be more than 50 times smaller than that required by the classical streaking camera for retrieval of pulses with a spectral bandwidth supporting 90 as transform-limited pulse durations. Furthermore, spatial variation of the streaking laser intensity, collection angle of streaked electrons and time delay jitter between the XUV pulse and streaking field can degrade the quality of the streaked spectrogram. We find that even when the XUV and streaking laser focal spots are comparable in size, the streaking electrons are collected from a 4π solid angle, or the delay fluctuates by more than the attosecond pulse duration, the attosecond pulses can still be accurately retrieved. In order to explain the insusceptibility of the streaked spectrogram to these factors, the linearity of the streaked spectrogram with respect to the streaking field is derived under the saddle point approximation.

A low-loss, robust setup for double optical gating of high harmonic generation

Previously, a second harmonic field was added to a polarization gating field by a Mach–Zehnder interferometer to gate the high harmonic generation process in argon gas. To reduce the losses of the interferometer, we developed a collinear setup consisting of only two quartz plates and a barium borate crystal. The high intensity at the focus allowed the double optical gating to be performed on neon gas. As a result, a supercontinuous spectrum was produced capable of supporting 130as. There is no delay jitter between the second harmonic field and the polarization gating field associated in this setup, which is necessary for generating stable single isolated attosecond pulses.

Retrieval of satellite pulses of single isolated attosecond pulses

Synopsis: When isolated attosecond pulses are reconstructed from an ideal streaked spectrogram, the relative intensity of accompanying satellite pulses can be identified from interference. However, the interference pattern can be distorted by variation of the streaking laser intensity in the focal volume or by the use of large delay steps in acquiring the spectrogram. We investigate these effects on the reconstruction of satellite pulses with fulland halfcycle separations and find that satellite pulses with full-cycle separation are largely unaffected by these issues.

Ellipticity dependence of 400 nm-driven high harmonic generation

We studied the dependence of high harmonic generation efficiency on the ellipticity of 400 nm driving laser pulses at 7.7 × 1014 W/cm2 and compared it with the 800 nm driving laser under the same conditions. The measured decrease of high harmonic yield with the ellipticity of the 400 nm laser is ∼1.5 times slower that of the 800 nm, which agrees well with theoretical predictions based on a semi-classical model. The results indicate that it is feasible to use the generalized double optical gating with 400 nm lasers for extracting single attosecond pulses with high efficiency.

Direct measurement of an electric field in femtosecond Bessel-Gaussian beams

We demonstrated the mapping of the spatial oscillation of electric fields in the transverse plane of a femtosecond Bessel-Gaussian laser beam from the first principle of classical electrodynamics. An attosecond burst of electrons for probing the electric force was placed in the Bessel beam through photoemission with single isolated 276 as extreme ultraviolet pulses. The direction reversal of the electric field in adjacent Bessel rings was directly confirmed by observing the momentum shift of the probe electrons.

Calibration of electron spectrometer resolution in attosecond streak camera

We report a new method for determining the energy resolution of time-of-flight spectrometers for detecting photoelectrons produced with attosecond XUV pulses. By measuring the width of the 2s2p autoionization line of helium, we found the resolution of our spectrometer to be approximately 0.6 eV for electrons at 35.5 eV. Furthermore, the resolution in the 10 to 35 eV range was determined by applying a retarding potential at the entrance of the drift tube.

Probing laser disturbed doubly excited states with isolated attosecond pulses

Two-electron excitation and autoionization in helium atoms were studied experimentally using isolated attosecond pulses for the first time. The population of the resonance state was modified by intense near infrared laser pulses.