Sabrina Leslie

Spontaneous symmetry breaking in a quenched ferromagnetic spinor Bose–Einstein condensate

A central goal in condensed matter and modern atomic physics is the exploration of quantum phases of matter—in particular, how the universal characteristics of zero-temperature quantum phase transitions differ from those established for thermal phase transitions at non-zero temperature. Compared to conventional condensed matter systems, atomic gases provide a unique opportunity to explore quantum dynamics far from equilibrium. For example, gaseous spinor Bose–Einstein condensates (whose atoms have non-zero internal angular momentum) are quantum fluids that simultaneously realize superfluidity and magnetism, both of which are associated with symmetry breaking. Here we explore spontaneous symmetry breaking in 87Rb spinor condensates, rapidly quenched across a quantum phase transition to a ferromagnetic state. We observe the formation of spin textures, ferromagnetic domains and domain walls, and demonstrate phase-sensitive in situ detection of spin vortices. The latter are topological defects resulting from the symmetry breaking, containing non-zero spin current but no net mass current.

High-resolution magnetometry with a spinor Bose-Einstein condensate.

We demonstrate a precise magnetic microscope based on direct imaging of the Larmor precession of a 87Rb spinor Bose-Einstein condensate. This magnetometer attains a field sensitivity of 8.3 pT/Hz1/2 over a measurement area of 120 microm2, an improvement over the low-frequency field sensitivity of modern SQUID magnetometers. The achieved phase sensitivity is close to the atom shot-noise limit, estimated as 0.15 pT/Hz1/2 for a unity duty cycle measurement, suggesting the possibilities of spatially resolved spin-squeezed magnetometry. This magnetometer marks a significant application of degenerate atomic gases to metrology.

Spontaneously modulated spin textures in a dipolar spinor Bose-Einstein condensate

Helical spin textures in a 87Rb F=1 spinor Bose-Einstein condensate are found to decay spontaneously toward a spatially modulated structure of spin domains. The formation of this modulated phase is ascribed to magnetic dipolar interactions that energetically favor the short-wavelength domains over the long-wavelength spin helix. The reduction of dipolar interactions by a sequence of rf pulses results in a suppression of the modulated phase, thereby confirming the role of dipolar interactions in this process. This study demonstrates the significance of magnetic dipole interactions in degenerate 87Rb F=1 spinor gases.

Direct nondestructive imaging of magnetization in a spin-1 bose-einstein gas

Polarization-dependent phase-contrast imaging is used to resolve the spatial magnetization profile of an optically trapped ultracold gas. This probe is applied to Larmor precession of degenerate and nondegenerate spin-1 87Rb gases. Transverse magnetization of the Bose-Einstein condensate persists for the condensate lifetime, with a spatial response to magnetic field inhomogeneities consistent with a mean-field model of interactions. In comparison, the magnetization of the non-condensed gas decoheres rapidly. Rotational symmetry implies that the Larmor frequency of a spinor condensate be density independent, and thus suitable for precise magnetometry with high spatial resolution.

Convex Lens-Induced Confinement for Imaging Single Molecules

Fluorescence imaging is used to study the dynamics of a wide variety of single molecules in solution or attached to a surface. Two key challenges in this pursuit are (1) to image immobilized single molecules in the presence of a high level of fluorescent background and (2) to image freely diffusing single molecules for long times. Strategies that perform well by one measure often perform poorly by the other. Here, we present a simple modification to a wide-field fluorescence microscope that addresses both challenges and dramatically improves single-molecule imaging. The technique of convex lens-induced confinement (CLIC) restricts molecules to a wedge-shaped gap of nanoscale depth, formed between a plano-convex lens and a planar coverslip. The shallow depth of the imaging volume leads to 20-fold greater rejection of background fluorescence than is achieved with total internal reflection fluorescence (TIRF) imaging. Elimination of out-of-plane diffusion leads to an approximately 10,000-fold longer diffusion-limited observation time per molecule than is achieved with confocal fluorescence correlation spectroscopy. The CLIC system also provides a new means to determine molecular size. The CLIC system does not require any nanofabrication, nor any custom optics, electronics, or computer control.

Amplification of Fluctuations in a Spinor Bose Einstein Condensate

densate are used as an amplifier of quantum spin fluctuations. We demonstrate the spectrum of this amplifier to be tunable, in quantitative agreement with mean-field calculations. We quantify the microscopic spin fluctuations of the initially paramagnetic condensate by applying this amplifier and measuring the resulting macroscopic magnetization. The magnitude of these fluctuations is consistent with predictions of a beyond-mean-field theory. The spinor-condensate-based spin amplifier is thus shown to be nearly quantum-limited at a gain as high as 30 dB. Accompanied by a precise theoretical framework and created in the lab in a highly controlled manner, ultracold atomic systems serve as a platform for studies of quantum dynamics and many-body quantum phases. Among these systems, gaseous spinor Bose Einstein condensates [1, 2, 3, 4, 5], in which atoms may explore all sub-levels of a non-zero hyperfine spin F, provide a compelling opportunity to access the static and dynamical properties of a magnetic superfluid [6, 7, 8, 9, 10]. We previously identified a quantum phase transition in an F = 1 spinor Bose Einstein condensate between a paramagnetic and ferromagnetic phase [9]. This transition is crossed as the quadratic Zeeman energy term, of

Single-molecule fluorescence imaging of processive myosin with enhanced background suppression using linear zero-mode waveguides (ZMWs) and convex lens induced confinement (CLIC)

Resolving single fluorescent molecules in the presence of high fluorophore concentrations remains a challenge in single-molecule biophysics that limits our understanding of weak molecular interactions. Total internal reflection fluorescence (TIRF) imaging, the workhorse of single-molecule fluorescence microscopy, enables experiments at concentrations up to about 100 nM, but many biological interactions have considerably weaker affinities, and thus require at least one species to be at micromolar or higher concentration. Current alternatives to TIRF often require three-dimensional confinement, and thus can be problematic for extended substrates, such as cytoskeletal filaments. To address this challenge, we have demonstrated and applied two new single-molecule fluorescence microscopy techniques, linear zero-mode waveguides (ZMWs) and convex lens induced confinement (CLIC), for imaging the processive motion of molecular motors myosin V and VI along actin filaments. Both technologies will allow imaging in the presence of higher fluorophore concentrations than TIRF microscopy. They will enable new biophysical measurements of a wide range of processive molecular motors that move along filamentous tracks, such as other myosins, dynein, and kinesin. A particularly salient application of these technologies will be to examine chemomechanical coupling by directly imaging fluorescent nucleotide molecules interacting with processive motors as they traverse their actin or microtubule tracks.

Periodic spin textures in a degenerate F=1 87Rb spinor Bose gas

We report on the spin textures produced by cooling unmagnetized

Convex lens-induced nanoscale templating

^{87}\mathrm{Rb}