Scott J. Sharpe

Efficient gas-phase generation of coherent vacuum ultraviolet radiation.

We report the demonstration of a pulsed atomic lead (Pb) vapor-based vacuum ultraviolet frequency converter from 233 to 186 nm with unity photon-conversion efficiency. This conversion is attained without phase matching.

Multi-watt 589nm fiber laser source

We have demonstrated 3.5W of 589nm light from a fiber laser using periodically poled stoichio-metric Lithium Tantalate (PPSLT) as the frequency conversion crystal. The system employs 938nm and 1583nm fiber lasers, which were sum-frequency mixed in PPSLT to generate 589nm light. The 938nm fiber laser consists of a single frequency diode laser master oscillator (200mW), which was amplified in two stages to >15W using cladding pumped Nd3+ fiber amplifiers. The fiber amplifiers operate at 938nm and minimize amplified spontaneous emission at 1088nm by employing a specialty fiber design, which maximizes the core size relative to the cladding diameter. This design allows the 3-level laser system to operate at high inversion, thus making it competitive with the 1088nm 4-level laser transition. At 15W, the 938nm laser has an M2 of 1.1 and good polarization (correctable with a quarter and half wave plate to >15:1). The 1583nm fiber laser consists of a Koheras 1583nm fiber DFB laser that is pre-amplified to 100mW, phase modulated and then amplified to 14W in a commercial IPG fiber amplifier. As a part of our research efforts we are also investigating pulsed laser formats and power scaling of the 589nm system. We will discuss the fiber laser design and operation as well as our results in power scaling at 589nm.

Widely tunable rapid-scanning mid-infrared laser spectrometer for industrial gas process stream analysis

A mid-infrared spectrometer with a tuning range of >400 cm−1 in the C-H stretching region of the spectrum has been designed and constructed. The spectrometer is based on the difference-frequency generation of two tunable diode lasers in periodically poled lithium niobate waveguides. Tuning is achieved by varying a single parameter, the wavelength of one of the near-infrared input lasers. The instrument can be tuned over the entire tuning range in less than 1 s. By taking advantage of the wide tuning range, the instrument has been used to analyze a mixture of methane, ethylene, and propylene. Each of these major components was measured with an accuracy of better than 2% (where the error is defined as a percentage of the measured value) in a single 30 s long scan. When optimized, the spectrometer has the potential to meet both the performance requirements and the practical requirements for real-time process control in petrochemical manufacturing. The general principles for the design of mid-infrared spectrometers with wide tuning ranges are explained, including the use of variable waveguide fabrication recipes to create broad phase-matching resonances (which lead to broad tuning) in the desired location.

Optical frequency conversion by a rotating molecular wave plate

We demonstrate efficient four-wave mixing in low-pressure molecular deuterium without the need for phase matching. We use two laser fields with opposite circular polarizations to produce a strong excitation of a rovibrational transition at a frequency of 3167 cm(-1) . The coherent molecular motion, in turn, modulates a third laser field (also circularly polarized) and results in highly efficient single-sideband conversion.

High-power solid-state sodium guidestar laser for the Gemini North Observatory

We report on the first successful installation of a commercial solid-state sodium guidestar laser system (GLS). The GLS developed at LMCT was delivered to Gemini North Observatory in February of 2005. The laser is a single beacon system that implements a novel laser architecture and represents a critical step towards addressing the need of the astronomy and military adaptive optics (AO) communities for a robust turn-key commercial GLS. The laser was installed on the center section of the 8 m Gemini North telescope, with the output beam relayed to a laser launch telescope located behind the 1 m diameter secondary mirror. The laser went through a three week performance evaluation between November and December 2005 wherein it consistently generated 12 W average power with measured M2 < 1.1 while locked to the D2 line at +/- 100 MHz. The system was required to perform during a 12-hour test period during three runs of 4-6 consecutive nights each. The laser architecture is based on continuous wave (CW) mode-locked solid-state lasers. The mode-locked format enables more efficient SFG conversion, and dispenses with complex resonant intensity enhancement systems and injection-locking electronics. The linearly-polarized, near-diffraction-limited, modelocked 1319 nm and 1064 nm pulses are generated in separate dual-head diode-pumped resonators. The two IR pulses are input into a single-stage, 30 mm PPSLT sum-frequency generation (SFG) crystal provided by Physical Science, Inc. Visible (589 nm) power of >16 W have been generated, representing a conversion efficiency of 40%.

Generation of high-average-power visible light in periodically poled nearly stoichiometric lithium tantalate

Sum-frequency generation (SFG) of >16 W of 589 nm light has been achieved by a single pass through a 20 mm long, undoped, periodically poled, nearly stoichiometric lithium tantalate (PPSLT) crystal. This, to our knowledge, represents the highest reported average power in the visible produced by a single-pass SFG crystal and the highest visible average power produced by PPSLT. The stoichiometric lithium tantalate crystal was grown directly from the melt without magnesium doping.

Accuracy and linearity of time-domain THz paint thickness measurements

An analysis of the single point reproducibility of TD-THz based paint thickness measurements demonstrated a precision of 130 nm, corresponding to 0.1% of the measured thickness. A detailed model of the anticipated TD-THz waveforms from samples of varying thickness indicates that an intrinsic uncertainty of 0.09% is anticipated in the absence of environmental fluctuations. Therefore, the influence of oscillations in the THz field associated with the initial reflection does not adversely impact the ability to extract accurate paint thickness information, and the noise associated with these oscillations could limit the measurement uncertainty of a calibrated instrument under optimum laboratory conditions. In the case of a deployed sensor, we anticipate that the accuracy will be degraded by environmental fluctuations.

High-average-power visible generation in periodically-poled nearly-stoichiometric lithium tantalate

Sum-frequency generation has been used to generate more than 12 W of average power at 589 nm in a single pass through a crystal of periodically-poled, undoped, nearly-stoichiometric lithium tantalate.

Widely-Tunable Rapid-Scanning Mid-IR Laser Spectrometer for Industrial Gas Process Stream Analysis

A mid-infrared spectrometer with a tuning range of >400 cm(-1) in the C-H stretching region of the spectrum has been designed and constructed. The spectrometer is based on the difference-frequency generation of two tunable diode lasers in periodically poled lithium niobate waveguides. Tuning is achieved by varying a single parameter, the wavelength of one of the near-infrared input lasers. The instrument can be tuned over the entire tuning range in less than 1 s. By taking advantage of the wide tuning range, the instrument has been used to analyze a mixture of methane, ethylene, and propylene. Each of these major components was measured with an accuracy of better than 2% (where the error is defined as a percentage of the measured value) in a single 30 s long scan. When optimized, the spectrometer has the potential to meet both the performance requirements and the practical requirements for real-time process control in petrochemical manufacturing. The general principles for the design of mid-infrared spectrometers with wide tuning ranges are explained, including the use of variable waveguide fabrication recipes to create broad phase-matching resonances (which lead to broad tuning) in the desired location.

Efficient vapor-phase vacuum ultraviolet (VUV) frequency conversion

Summary form only given. The techniques of electromagnetically induced transparency (EIT) may be employed in order to create an effective nonlinear response at a given wavelength which is equal in magnitude to the linear response at that wavelength. Physically, this allows frequency converters wherein 100% photon-to-photon conversion occurs in a single coherence length, i.e., in that distance which causes a /spl pi/ phase slip between the driving polarization and the generated electromagnetic wave. These ideas were first implemented by Jain et al. (1996), to convert 425 nm to 293 nm, in a medium consisting of a single isotope of Pb. This paper reports the demonstration of a vapor-phase VUV frequency converter from 233 nm to 186 nm with an energy conversion efficiency exceeding 35%; the maximum generated signal energy and power were 250 /spl mu/J and 25 kW. The net conversion efficiency to 186 nm, including all beams, is roughly 2%. These wavelengths were chosen to demonstrate the utility of this type of frequency converter to generate wavelengths outside the transparency window of most crystalline media. Our technique involves the application of two strong laser fields which are almost two-photon resonant with a Raman transition of the Pb atoms.