Seok-Ho Jeong

A Numerical Study on Radiation-Induced Oscillatory Instability in CH

Radiation-induced oscillatory instability in CH/Air diffusion flames is numerically investigated by adopting detailed chemistry. Counterflow diffusion flame is employed as a model flamelet and optically thin gas-phase radiation is assumed. Attention is focused on the extinction regime induced by radiative heat loss, which occurs at low strain rate. Once a steady flame structure is obtained for a prescribed value of initial strain rate, transient solution of the flame is calculated after a finite amount of strain-rate perturbation is imposed on the steady flame. Depending on the initial strain rate and the amount of perturbed strain rate, transient evolution of the flame exhibits various types of flame-evolution behaviors. Basically, the dynamic behaviors can be classified into two types, namely oscillatory decaying solution and diverging solution leading to extinction.

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Various flame types are observed in a double concentric burner by varying equivalence ratio and flow rates in each tube. Observed flame types include bunsen-type flame, ring-shaped flame, outer lifted flame, inner lifted flame, and oscillatory lifted flame, The doman of existence of various flames is mapped with equivalence ratio and annular jet velocity. Each flame is investigated through direct photography and OH PLIF. As central air velocity increase, the blowout region is diminished and lifted oscillating flames are observed. Inner lifted flames are observed from bunsen flames or rich shaped flames by increasing central air velocity. For inner lifted flames, annular jet velocity, at flame liftoff decreases with increasing central air jet velocity. Axial velocity profile and temperature fie이 using LDV and CRS, respectively, for a typical inner lifted flame are also measured through which the role of tribrachial flame for stabilization in emphasized.

/Air Diffusion Flames

The effects of SiCladdition on flame structures have been studied in flame hydrolysis deposition (FHD) processes using Coherent anti-Stokes Raman spectroscopy (CARS) and planar laser induced fluorescence (PLIF) to measure temperatures and OH concentrations, respectively. The results demonstrate that even a small amount of SiCl addition can change thermal and chemical structures of H/O diffusion flames. When SiCl is added to a flame temperature decreases in non-reacting zone due to the increases in both specific heat and density of the gas mixture, while flame temperature increase in particle formation zone due to the heat release through hydrolysis and oxidation reactions of SiCl. It is also found that OH concentration decreases dramatically in particle formation zone where temperatures increase. This can be attributed to consumption of oxidative species and generation of HCl during silica formation.

Characteristics of Premixed Flames in a Double Concentric Burner

The extinction of premixed flames under the influence of stretch is studied numerically. A wide range of fuel (hydrogen, ethylene, acetylene, methane, propane and methanol) and air mixtures are established in an opposed jet and their flame properties such as flame speed, flame thickness, thermal diffusivity, and stretch rate at extinction are computed. Computations are made using several chemical kinetic mechanism (Smooke, Kee et al. and Peters). The major result is that, in contrast to the various previous claims of extinction Karlovitz number varying over three orders of magnitude, it is found to be constant around two for all of the mixtures tested. That is, premixed flames are extinguished when the physical flow time decreases (due to increased stretch rate) to the point where it approximately equals the chemical reaction time. Here the relevant chemical reaction time is not the one computed using the one-dimensional flame properties as originally suggested in the formulation of Karlovitz number, but rather it is the one obtained using the stretched flame properties which fully reflect the effect of straining on the flame structure.

Measurements of Temperature and OH Radical Distributions in Flame Hydrolysis Deposition Process

Mixing process of impinging jets of liquid oxidizer and liquid fuel is simulated by using water and sodium carbonate (NaCO) solution. The shapes of liquid sheets are visualized and flowrate distributions are measured by collecting droplets using measuring cells. Mixing charateristics are studied by using acid-base titration. Stable liquid sheets are formed and two liquid jets are well mixed for symmetric impinging jets. Similarity in flowrate distribution for various measuring heights is observed. For asymmetric impinging jets, liquid sheets become unstable as the difference in the velocities of jets increases. In some extreme cases, liquid sheets are not formed and the jets are separated. Dimensionless variables are adopted demonstrating similarly in flowrate distribution. Mixing characteristics vary significantly with experiment conditions.

Numerical study on extinction of premixed flames using local flame properties

Flame oscillation phenomena in a co-flow diffusion flame was experimentally studied with periodic fuel supply using a solenoid valve. The degree of excitation was controlled by changing the volume flux of fuel passing through the valve. Flame oscillation frequencies were measured utilizing a photodiode, a spectrum analyzer, video and high speed movies. Laser planar visualization was employed to study the correlation between the flame oscillation and the toroidal vortices. Observed are three regimes of flame oscillation, where the oscillation frequencies are for the multiples of excitation, the excitation itself and the flame natural oscillation. Both periods of natural oscillation and of excitation induced oscillation exist over one cycle of the excitation in the frequency multiplied regime. It is considered as an effect of balancing the influence of buoyancy driven vortex with that of excitation induced vortex near the excitation rate of 0.2. Flame shapes are become monotonous as increasing the excitation frequency to the range of over two fold of the natural oscillation. The flame oscillation can be modulated to the frequency of either multiples of excitation or excitation itself under certain conditions. This implies that the flame oscillation could be modulated to avoid the resonance frequency of the combustor, and shows the possibility of active control of the flame oscillation.

An experimental study on flow distribution and mixing in impinging jets

Extinction characteristics and acoustic response of hydrogen-air diffusion flames at various pressures are numerically studied by employing counterflow diffusion flame as a model flamelet in turbulent flames in combustion chambers. The numerical results show that extinction strain rate increases linearly with pressure and then decreases, and increases again at high pressures. Thus, flames are classified into three pressure regimes. Such nonmonotonic behavior is caused by the change in chemical kinetic behavior as pressure rises. The investigation of acoustic-pressure response in each regime, for better understanding of combustion instability, shows different characteristics depending on pressure. At low pressures, pressure-rise causes the increase in flame temperature and chain branching/recombination reaction rates, resulting in increased heat release. Therefore, amplification in pressure oscillation is predicted. Similar phenomena are predicted at high pressures. At moderate pressures, weak amplification is predicted since flame temperature and chain branching reaction rate decreases as pressure rises. This acoustic response can be predicted properly only with detailed chemistry or proper reduced chemistry.

An experimental study on instability and control of co-flow diffusion flames

Experimental studies on combustion phenomena within a porous ceramic burner are reported. Main interest of the present work is to investigate fundamental flame behaviors and their effects on the burner operation. Due to high thermal capacity of the porous ceramic materials, the response of flame to burning condition changes is slow and thus to have a stabilized flame is quite difficult and takes much time. It is found that the temperature profile obtained at downstream of the flame zone is not much sensitive to the movement of flame and the speed of flame movement is less than 0.1 mm/sec for the conditions tested. With the premixed LPG/air flame imbedded within the porous ceramic burner, stable combustion regions and unstable combustion regions leading to blowoff or flashback phenomena are observed and mapped on flow velocity versus equivalence ratio diagram. For the development of burner operation technique which is more practical and safe, intermittent burning technique, where the fuel or/and air is supplied to the burner intermittently, is proposed as one of the flame control methods for the porous ceramic burner and tested in this study. Through the experiment, it is realized that the proposed method is acceptable in respect to burner performance and give much flexibility in the operation of porous ceramic burner.

Numerical study on extinction and acoustic response of diluted hydrogen-air diffusion flames with detailed and reduced chemistry

Characteristics of the lifted flame which is generated by issuing of the fuel through the miniature nozzle, d = 0.164 mm, are studied using the planar laser induced fluorescence technique. OH radical is excited on the (8) line of the .SIGMA. .PI.(1, 0) band transition (283.55 nm) and LIF signals are captured at the bands of (0, 0) and (1, 1) transition (306 ~ 326 nm) using the filters and ICCD camera. Hydroxyl radical (OH) profile for nozzle attached flame shows that OH radical populations at the flame sides and flame tip are larger than those at the base. But for the lifted flame (tribrachial flame) case, those are larger at the flame base than at the flame tip and flame sides. The OH radical is more dense near the center line of flame base at the blowing out. This fact proves the Chung and Lees blowout theory-blowout occurs when the flame is anchored at the flame axis. axis.

Experimental study on flame behavior within a porous ceramic burner

To provide standard data of temperature and species concentration in a flame for calibrating the laser based combustion diagnostics, we investigated combustion characteristics of a flat flame burner(Mckennar Product). For various stoichiometric ratios we measured temperature and concentration of OH in the premixed methane/air flame with Coherent anti-Stokes Raman spectroscopy and laser induced fluorescence technique, respectively. Assuming the chemical equilibrium condition at the measured temperature, the mole fraction of the OH radical in the flame was obtained and compared with numerical analysis.