Sergey Kovalev

High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter

Ultrashort flashes of THz light with low photon energies of a few meV, but strong electric or magnetic field transients have recently been employed to prepare various fascinating nonequilibrium states in matter. Here we present a new class of sources based on superradiant enhancement of radiation from relativistic electron bunches in a compact electron accelerator that we believe will revolutionize experiments in this field. Our prototype source generates high-field THz pulses at unprecedented quasi-continuous-wave repetition rates up to the MHz regime. We demonstrate parameters that exceed state-of-the-art laser-based sources by more than 2 orders of magnitude. The peak fields and the repetition rates are highly scalable and once fully operational this type of sources will routinely provide 1 MV/cm electric fields and 0.3 T magnetic fields at repetition rates of few 100 kHz. We benchmark the unique properties by performing a resonant coherent THz control experiment with few 10 fs resolution.

Probing ultra-fast processes with high dynamic range at 4th-generation light sources: Arrival time and intensity binning at unprecedented repetition rates

Understanding dynamics on ultrafast timescales enables unique and new insights into important processes in the materials and life sciences. In this respect, the fundamental pump-probe approach based on ultra-short photon pulses aims at the creation of stroboscopic movies. Performing such experiments at one of the many recently established accelerator-based 4th-generation light sources such as free-electron lasers or superradiant THz sources allows an enormous widening of the accessible parameter space for the excitation and/or probing light pulses. Compared to table-top devices, critical issues of this type of experiment are fluctuations of the timing between the accelerator and external laser systems and intensity instabilities of the accelerator-based photon sources. Existing solutions have so far been only demonstrated at low repetition rates and/or achieved a limited dynamic range in comparison to table-top experiments, while the 4th generation of accelerator-based light sources is based on superconducting radio-frequency technology, which enables operation at MHz or even GHz repetition rates. In this article, we present the successful demonstration of ultra-fast accelerator-laser pump-probe experiments performed at an unprecedentedly high repetition rate in the few-hundred-kHz regime and with a currently achievable optimal time resolution of 13 fs (rms). Our scheme, based on the pulse-resolved detection of multiple beam parameters relevant for the experiment, allows us to achieve an excellent sensitivity in real-world ultra-fast experiments, as demonstrated for the example of THz-field-driven coherent spin precession.

Terahertz field control of in-plane orbital order in La0.5Sr1.5MnO4

In-plane anisotropic ground states are ubiquitous in correlated solids such as pnictides, cuprates and manganites. They can arise from doping Mott insulators and compete with phases such as superconductivity; however, their origins are debated. Strong coupling between lattice, charge, orbital and spin degrees of freedom results in simultaneous ordering of multiple parameters, masking the mechanism that drives the transition. Here we demonstrate that the orbital domains in a manganite can be oriented by the polarization of a pulsed THz light field. Through the application of a Hubbard model, we show that domain control can be achieved by enhancing the local Coulomb interactions, which drive domain reorientation. Our results highlight the key role played by the Coulomb interaction in the control and manipulation of orbital order in the manganites and demonstrate a new way to use THz to understand and manipulate anisotropic phases in a potentially broad range of correlated materials.

A planar Schottky diode based integrated THz detector for fast electron pulse diagnostics

Semiconductor based THz detectors are potentially cost-effective devices that can be manufactured in standard processes suitable for high frequencies such as GaAs, InP or SiGe. The core element of our detector circuit is an integrated Schottky-barrier diode used as a rectifier which is connected to an on-chip patch antenna. The detector operates at 300 GHz and is manufactured in a commercial GaAs technology. It is part of a multi-element array where each detector is tuned to a specific frequency in the range between 0.1 THz to 1.5 THz. The complete on-chip spectrometer will provide one more option to monitor the longitudinal beam shape properties in modern superconducting linear accelerators by measuring the THz radiation generated by electron bunches. Therefore, it may help to replace single element THz detectors as well as the costly and bulky THz spectrometers. We could conduct first measurements at the undulator THz source of the HZDRs linear accelerator and prove our detector concept. This paper briefly explains the system design and presents the first comparison between simulated data and measurement results of the on-chip Schottky diode detector operating at 300 GHz. We also present a bias-tee circuit developed and built for the measurement.

Near-field THz nanoscopy at novel accelerator-based photon sources (Conference Presentation)

This talk advertises scattering-type scanning near-field infrared micro-spectroscopy (s-SNIM) in the spectral range of 75 to 1.3 THz [1], as provided by the free-electron laser FELBE, the narrow-band laser-light source at Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Germany. We demonstrate the -independent s-SNIM resolution of a few 10 nm by exploring structured Au samples, Graphene-transistors, meta-materials [2], and local ferroelectric phase-transitions down to LHe [3]. s-SNIM secondly was integrated into a THz pump-probe experiment for the inspection of excited states in structured SiGe samples. We developed a novel demodulation technique with high temporal resolution [4] hence achieving an excellent Signal-to-Noise Ratio. Thirdly using the super-radiant TELBE light source [5], HZDR recently extended the wavelength range down to 100 GHz radiation. We adapted our s-SNIM to this TELBE photon-source as well, achieving an equally high spatial resolution as with FELBE. Moreover, the superb 30-fs temporal resolution of TELBE will allow us to study a multitude of physical phenomena with sub-cycle resolution [5,6], such as spin-structures, magnons and phonon polaritons. [1] F. Kuschewski et al., Appl. Phys. Lett. 108 (2016) 113102. [2] S.C. Kehr et al., ACS Photonics 3 (2016) 20. [3] J. Doring et al., Appl. Phys. Lett. 105 (2014) 053109. [4] F. Kuschewski et al., Sci. Rep. 5 (2015) 12582. [5] B. Green et al., Sci. Rep. 6 (2016) 22256. [6] S. Kovalev et al., Struct. Dyn. 4 (2017) 024301.

Magnetic field dependence of antiferromagnetic resonance in NiO

We report on measurements of magnetic field and temperature dependence of antiferromagnetic resonances in the prototypical antiferromagnet NiO. The frequencies of the magnetic resonances in the vicinity of 1 THz have been determined in the time-domain via time-resolved Faraday measurements after selective excitation by narrow-band superradiant terahertz (THz) pulses at temperatures down to 3K and in magnetic fields up to 10 T. The measurements reveal two antiferromagnetic resonance modes, which can be distinguished by their characteristic magnetic field dependencies. The nature of the two modes is discussed by comparison to an eight-sublattice antiferromagnetic model, which includes superexchange between the next-nearest-neighbor Ni spins, magnetic dipolar interactions, cubic magneto-crystalline anisotropy, and Zeeman interaction with the external magnetic field. Our study indicates that a two-sublattice model is insufficient for the description of spin dynamics in NiO, while the magnetic-dipolar interactions and magneto-crystalline anisotropy play important roles.

Super-radiant high-field THz sources operating at quasi-cw rep rates

An overview is given about the state-of-the-art of superradiant THz sources with a particular emphasize on very recent developments towards compact facilities based on super-conducting RF accelerator technology which enable quasi-cw operation at high repetition rates.