Seungjong Lee

Composite cure kinetic analysis of unsaturated polyester free radical polymerization

Curing kinetics of unsaturated polyester resin system exhibiting apparent induction periods was investigated by modeling free radical initiation and propagation processes. The isothermal curing induction time as well as the maximum-rate time provided the same activation energy in the Arrhenius relation, and therefore, the isothermal curing master curve was constructed by using the reduced time method. Two model elementary rate equations for radical and monomer were proposed to describe the free radical polymerization of unsaturated polyester resin systems. The power law was adopted to express the conversion dependence function of the initiation efficiency and the monomer reaction rate. Demonstrating the capability of the developed model, the agreement between experimental and predicted data was excellent in both isothermal and dynamic-heating conditions, even with the same model parameters in different thermal conditions.

Corrugation-assisted metal-coated angled fiber facet for wavelength-dependent off-axis directional beaming

We propose a fiber-optic-plasmonic hybrid device that is based on a corrugation-assisted metal-coated angled fiber facet (CA-MCAFF) for wavelength-dependent off-axis directional beaming (WODB). The device breaks into two key structures: One is the MCAFF structure, which is a modified Kretschmann configuration implemented onto a fiber platform, thereby being able to generate a unidirectional surface plasmon with dramatically enhanced properties in terms of non-confined diffracted radiation loss and operational bandwidth. The other is the periodic corrugation structure put on the MCAFF, thereby enabling WODB functionality out of the whole structures. The corrugated metal surface out-couples the surface plasmon mode to free-space optical radiation into a direction that varies with the wavelength of the optical radiation with excellent linearity. We perform extensive numerical investigations based on the finite-element-method and analyze the out-coupling efficiency (OCEout) and spectral bandwidth (SBout) of the proposed device for various designs and conditions. We determine the seven structural parameters of the device via taking sequential optimization steps. We deduce two optimal conditions particularly for the fiber-facet angle, in terms of the averaged OCEout or the SBout in the whole visible wavelength range (400 - 700 nm), which eventually leads to OCEout = 30.4% and SBout = 230 nm or to OCEout = 24.5% and SBout = 245 nm, respectively. These results suggest substantial enhancements in both OCEout and SBout, in comparison with the performance properties of a typical nano-slit-based device having a similar type of WODB functionality. The proposed CA-MCAFF is a simple, compact and efficient WODB device that is fully compatible with the state-of-the-art optical fiber technology.

Comparative experimental analysis of thermal characteristics of Ytterbium-Doped Phosphosilicate and Aluminosilicate fibers

We present a comparative experimental analysis of the thermal spectroscopic characteristics of a phosphosilicate (P)-based ytterbium-doped fiber (YDF) against an aluminosilicate (Al)-based YDF in the temperature range of 25 to 150°C. We also characterize the fibers as gain media in a cladding-pumped amplifier configuration. While both fibers exhibit comparable trends in their thermal characteristics, there are noticeable distinctions in the fluorescence lifetime reduction rate and the spectral dependence of the transition cross-sections. The P- and Al-based YDFs present thermal lifetime reduction rates of 0.012%/°C and 0.026%/°C, respectively. In particular, in the spectral region at ~940 nm, the absorption cross-section of the P-based YDF undergoes significantly less thermal change compared to that of the Al-YDF. In the cladding-pumped amplifier configuration operating at a total gain of 10 dB, the Al-based YDF generally performs betters than the P-based YDF in the temperature range of 25 to 75°C. However, it is highlighted that in the high temperature range of over 75°C, the latter shows a less gain reduction rate than the former, thereby yielding higher relative output power by 3.3% for a 1060-nm signal, for example.

Numerical study on multi-pulse dynamics and shot-to-shot coherence property in quasi-mode-locked regimes of a highly-pumped anomalous dispersion fiber ring cavity

We numerically investigate quasi-mode-locked (QML) multi-pulse dynamics in a fiber ring laser cavity in the anomalous dispersion regime. We show that the laser cavity can operate in five constitutively different QML regimes, depending on the saturation power of the saturable absorber element and the length of the passive fiber section that parameterize the overall nonlinearity and dispersion characteristic of the laser cavity. We classify them into the incoherent noise-like-pulse, partially-coherent noise-like-pulse, symbiotic, partially-coherent multi-soliton, and coherent multi-soliton regimes, accounting for their coherence and multi-pulse formation features. In particular, we numerically clarify and confirm the symbiotic regime for the first time to the best of our knowledge, in which noise-like pulses and multi-solitons coexist stably in the cavity that has recently been observed experimentally. Furthermore, we analyze the shot-to-shot coherence characteristics of the individual QML regimes relative to the amount of the nonlinear-phase shift per roundtrip, and verify a strong correlation between them. We also show that the net-cavity dispersion plays a critical role in determining the multi-pulse dynamics out of the partially-coherent noise-like-pulse, symbiotic, and partially-coherent multi-soliton regimes, when the cavity bears moderate nonlinearity. We quantify and visualize all those characteristics onto contour maps, which will be very useful and helpful in discussing and clarifying the complex QML dynamics.

Combinatorial Study of Supercontinuum Generation Dynamics in Photonic Crystal Fibers Pumped by Ultrafast Fiber Lasers

We numerically study the dynamics of supercontinuum generation (SCG) for a variety of possible combinations of photonic crystal fibers (PCFs) and ultrafast fiber laser pulses that the current technologies offer. Three types of PCFs typically used in SCG and four representative types of ultrafast fiber laser pulses are considered for this combinatorial study. We numerically model and qualitatively discuss the nonlinear evolution of the pulses for their whole 12 combinatorial cases. We also quantitatively analyze their output spectra and organize a performance chart for them in terms of spectral bandwidth, flatness, and degree of spectral coherence. Finally, we suggest the most viable combinations among the given PCFs and ultrafast fiber laser pulses in order for generating a target supercontinuum spectrum for various specific cases.

Metallic Fresnel zone plate implemented on an optical fiber facet for super-variable focusing of light

We propose and investigate a metallic Fresnel zone plate (FZP/MFZP) implemented on a silver-coated optical fiber facet for super-variable focusing of light, the focal point of which can be drastically relocated by varying the wavelength of the incident light. We numerically show that when its nominal focal length is set to 20 μm at 550 nm, its effective focal length can be tuned by ~13.7 μm for 300-nm change in the visible wavelength range. This tuning sensitivity is over 20 times higher than that of a conventional silica-based spherical lens. Even with such high tuning sensitivity with respect to the incident wavelength change, the effective beam radius at the focal point is preserved nearly unchanged, irrespective of the incident wavelength. Then, we fabricate the proposed device, exploiting electron- and focused-ion-beam processes, and experimentally verify its super-variable focusing functionality at typical red, green, and blue wavelengths in the visible wavelength range, which is in good agreement with the numerical prediction. Moreover, we propose a novel MFZP structure that primarily exploits the surface-plasmon-polariton-mediated, extra-ordinary transmission effect. For this we make all the openings of an MFZP, which are determined by the fundamental FZP design formula, be partitioned by multi-rings of all-sub-wavelength annular slits, so that the transmission of azimuthally polarized light is inherently prohibited, thereby leading to super-variable and selective focusing of radially polarized light. We design and fabricate a proof-of-principle structure implemented on a gold-coated fused-silica substrate, and verify its novel characteristics both numerically and experimentally, which are mutually in good agreement. We stress that both the MFZP structures proposed here will be very useful for micro-machining, optical trapping, and biomedical sensing, in particular, which invariably seek compact, high-precision, and flexible focusing schemes.

Temporal dynamics and shot-to-shot stability characteristics of three distinctive partially-mode-locked operation regimes in a fiber ring cavity

We numerically and experimentally study three distinctive partially-mode-locked regimes in a fiber ring laser. We discuss their temporal dynamics and shot-to-shot stability characteristics, which offers a clue to the existence of the partial coherence in such regimes.

Numerical study on spectral coherence of noise-like pulses in a fiber ring cavity configuration

We numerically investigate the noise-like pulse (NLP) operation in a simply modelled fiber ring cavity. Under the different cavity conditions, we verify how the spectral coherence of the NLP is altered.

Formation sequences of noise-like pulse in fiber ring cavity configuration and their effect on the partial coherence

We experimentally investigate the partially coherent nature of noise-like pulses (NLPs) generated from passively mode-locked fiber ring cavity, and emphasize that the coherence of NLPs can be completely different, depending on the NLP formation sequence.

Plasmonic grating-assisted nano-slit implemented in an all-fiberized format for wavelength-dependent beaming

We demonstrate a plasmonic grating-assisted nano-slit implemented in an all-fiberized format for wavelength-dependent beaming. The proposed scheme can be utilized as a simple and compact platform to generate surface plasmons as well as an efficient beaming device to replace conventional diffraction gratings.