Stanley Mrowka

Results With the Neutron Scatter Camera

We describe the design, calibration, and measurements made with the neutron scatter camera. Neutron scatter camera design allows for the determination of the direction and energy of incident neutrons by measuring the position, recoil energy, and time-of-flight (TOF) between elastic scatters in two liquid scintillator cells. The detector response and sensitive energy range (0.5-10 MeV) has been determined by detailed calibrations using a 252Cf neutron source over its field of view (FOV). We present results from several recent deployments. In a laboratory study we detected a 252Cf neutron source at a stand off distance of 30 m. A hidden neutron source was detected inside a large ocean tanker. We measured the integral flux density, differential energy distribution and angular distribution of cosmic neutron background in the fission energy range 0.5-10 MeV at Alameda, CA (sea level), Livermore, CA (174 m), Albuquerque, NM (1615 m) and Fenton Hill, NM (2630 m). The neutron backgrounds are relatively low, and non-isotropic. The camera has been ruggedized, deployed to various locations and has performed various measurements successfully. Our results show fast neutron imaging could be a useful tool for the detection of special nuclear material (SNM).

Results with the neutron scatter camera

We present results from recent deployments with the neutron scatter camera. We successfully detected and pinpointed a hidden 252Cf neutron source in a large ocean tanker at Alameda, CA. In a lab study we detected a 252Cf neutron source at a stand off distance of about 100 ft. We measured the integral flux, differential flux and angular distribution of cosmic neutron background in the fission energy range 0.5–10MeV at Alameda, CA (sea level), Livermore, CA (570 ft), Albuquerque, NM (5300 ft) and Fenton Hill, NM (8630 ft). The neutron backgrounds are relatively low, uniform and well understood. We recently increased the camera effective area 3x. The camera has been successfully ruggedized, deployed to various locations and has performed various measurements. Our results are encouraging and suggest fast neutron imaging could be a useful tool for the detection of special nuclear material (SNM).

Spectral- and Pulse-Shape Discrimination in Triplet-Harvesting Plastic Scintillators

In this work, we describe a method to control the relative proportion of prompt and delayed luminosity of organic-based scintillators via direct and exponential emission from an extrinsic triplet state. This approach involves the incorporation of triplet-harvesting heavy metal complexes in plastic scintillator matrices to convert intrinsically non-luminescent host states to highly emissive guest states. Measurements on these plastic scintillators indicate improved light yields over the undoped polymers and the ability to perform neutron/gamma particle-discrimination. A similar extent of molecular-level control is not possible in traditional organic materials due to complex decay kinetics and the absence of spectral information for the delayed triplet-derived emission. The materials described here address these limitations through efficient host-guest triplet harvesting, which enables particle discrimination according to conventional pulse-shape discrimination (PSD) and a previously unreported spectral-shape discrimination (SSD) scheme.

Advances in imaging fission neutrons with a neutron scatter camera

Special nuclear material (SNM) emits high energy radiation during active and passive interrogation. This radiation can be imaged thus allowing visualization of shielded and/or smuggled SNM. Lower backgrounds and higher penetration through hi-Z materials make neutrons the preferred detectable in many scenarios. We have developed a neutron scatter camera that directly images fast fission neutrons from SNM sources while simultaneously measuring energy spectra. We have made many significant advances in the design and implementation of such instruments leading to an over 30 fold improvement in sensitivity. We will present results from our detector including analysis techniques that we have developed for neutron imaging and particle discrimination techniques. We will discuss camera calibration and performance under realistic threat detection scenarios, and future prospects in this field.

Measurement of the Fast Neutron Energy Spectrum of an

We have measured the neutron energy spectrum of an 241Am-Be(α,n) source between 1.5 MeV and 9 MeV using a neutron scatter camera. The apparatus consists of two segmented planes each with 16 liquid scintillator cells (Eljen EJ-309), for a total of 32 elements; the neutron energy spectrum is measured using double elastic scatter events. After unfolding resolution effects using a maximum likelihood technique, the measurement is compared to reference Am-Be spectra. Further, we discuss the ability of the neutron scatter camera to distinguish between an Am-Be source and a spontaneous fission source.

^{241}{\rm Am\!-\!Be}

Organic scintillators are widely used for fast neutron detection and spectroscopy. Several effects complicate the interpretation of results from detectors based upon these materials. First, fast neutrons will often leave a detector before depositing all of their energy within it. Second, fast neutrons will typically scatter several times within a detector, and there is a non-proportional relationship between the energy of, and the scintillation light produced by, each individual scatter; therefore, there is not a deterministic relationship between the scintillation light observed and the neutron energy deposited. Here we demonstrate a hardware technique for reducing both of these effects. Use of a segmented detector allows for the event-by-event correction of the light yield non-proportionality and for the preferential selection of events with near-complete energy deposition, since these will typically have high segment multiplicities.

Source Using a Neutron Scatter Camera

We present advances with a 32 element scalable, segmented dual mode imager. Scaling up the number of cells results in a 1.4 increase in efficiency over a system we deployed last year. Variable plane separation has been incorporated which further improves the efficiency of the detector. By using 20 cm diameter cells we demonstrate that we could increase sensitivity by a factor of 6. We further demonstrate gamma ray imaging in from Compton scattering. This feature allows for powerful dual mode imaging. Selected results are presented that demonstrate these new capabilities.

Improved fast neutron spectroscopy via detector segmentation

The neutron scatter camera was originally developed for a range of SNM detection applications. We are now exploring the feasibility of applications in treaty verification and warhead monitoring using experimentation, maximum likelihood estimation method (MLEM), detector optimization, and MCNP-PoliMi simulations.

Results with a 32-element dual mode imager

This report summarizes the results of a one-year, feasibility-scale LDRD project that was conducted with the goal of developing new plastic scintillators capable of pulse shape discrimination (PSD) for neutron detection. Copolymers composed of matrix materials such as poly(methyl methacrylate) (PMMA) and blocks containing trans-stilbene (tSB) as the scintillator component were prepared and tested for gamma/neutron response. Block copolymer synthesis utilizing tSBMA proved unsuccessful so random copolymers containing up to 30% tSB were prepared. These copolymers were found to function as scintillators upon exposure to gamma radiation; however, they did not exhibit PSD when exposed to a neutron source. This project, while falling short of its ultimate goal, demonstrated the possible utility of single-component, undoped plastics as scintillators for applications that do not require PSD.

Applying the neutron scatter camera to treaty verification and warhead monitoring

When searching for SNM simply designing a better detector to optimize the signal S from the source is not enough. It is important to know the background B to maximize S/N, where N is the noise in B. Cosmic rays are a dominant source of neutron background. It is therefore important to know their flux, angular and energy distribution. Over the last 50 years work has been done to study cosmic ray neutrons and their variation. The full hemispherical neutron flux is usually quoted at a certain altitude (e.g. Altitude = 0 meters above sea level, pressure = 1033 g/cm2) and geomagnetic rigidity (e.g. GMR = 1.2GV). Neutron fluxes at other locations are scaled from the sea level data using a well determined prescription. However, there is a lack in knowledge of the angular dependence of the neutron flux at sea level. The angular dependence is important for two reasons; first many detectors have an efficiency that changes with the direction of the incident neutron. Second none of the measurements to date have determined how the flux changes with angle, their data must be modeled to estimate the full hemispherical flux. In this paper we present the cosmic neutron background flux measured by a neutron scatter camera in the energy range 0.2-10MeV. Our measurements are in agreement with the best fit to past data. We present for the 1st time the neutron zenith angle dependence at fission energies which is observed to be a function of the form cos2.7thetas.