Stefan Karsch

Determination of the Al mole fraction and the band gap bowing of epitaxial AlxGa1−xN films

AlxGa1−xN alloys were grown on c-plane sapphire by plasma-induced molecular beam epitaxy. The Al content x was varied over the whole composition range (0⩽x⩽1). The molar Al fraction was deduced from x-ray diffraction and for comparison by elastic recoil detection analysis. The composition of the alloys calculated from the lattice parameter c underestimates x. This is due to a deformation of the unit cell. The exact Al mole fraction and the biaxial strain of the alloys can be calculated by an additional determination of a, using asymmetric reflections. The results obtained by x-ray diffraction and elastic recoil detection provide evidence for the validity of Vegard’s law in the AlGaN system. In addition, the deviation of the band gap from a linear dependence on x was investigated. We found a downward bowing with a bowing parameter b=1.3 eV.

Generation of sub-mJ terahertz pulses by optical rectification

Recent theoretical calculations predicted an order-of-magnitude increase in the efficiency of terahertz pulse generation by optical rectification in lithium niobate when 500 fs long pump pulses are used, rather than the commonly used ~100 fs pulses. Even by using longer than optimal pump pulses of 1.3 ps duration, 2.5× higher THz pulse energy (125 μJ) was measured with 2.5× higher pump-to-THz energy conversion efficiency (0.25%) than reported previously with shorter pulses. These results verify the advantage of longer pump pulses and support the expectation that mJ-level THz pulses will be available by cooling the crystal and using large pumped area.

Laser -driven soft-X-ray undulator source

High-intensity X-ray sources such as synchrotrons and free-electron lasers need large particle accelerators to drive them. The demonstration of a synchrotron X-ray source that uses a laser-driven particle accelerator could widen the availability of intense X-rays for research in physics, materials science and biology. Synchrotrons and free-electron lasers are the most powerful sources of X-ray radiation. They constitute invaluable tools for a broad range of research1; however, their dependence on large-scale radiofrequency electron accelerators means that only a few of these sources exist worldwide. Laser-driven plasma-wave accelerators2,3,4,5,6,7,8,9,10 provide markedly increased accelerating fields and hence offer the potential to shrink the size and cost of these X-ray sources to the university-laboratory scale. Here, we demonstrate the generation of soft-X-ray undulator radiation with laser-plasma-accelerated electron beams. The well-collimated beams deliver soft-X-ray pulses with an expected pulse duration of ∼10 fs (inferred from plasma-accelerator physics). Our source draws on a 30-cm-long undulator11 and a 1.5-cm-long accelerator delivering stable electron beams10 with energies of ∼210 MeV. The spectrum of the generated undulator radiation typically consists of a main peak centred at a wavelength of ∼18 nm (fundamental), a second peak near ∼9 nm (second harmonic) and a high-energy cutoff at ∼7 nm. Magnetic quadrupole lenses11 ensure efficient electron-beam transport and demonstrate an enabling technology for reproducible generation of tunable undulator radiation. The source is scalable to shorter wavelengths by increasing the electron energy. Our results open the prospect of tunable, brilliant, ultrashort-pulsed X-ray sources for small-scale laboratories.

Terawatt diode-pumped Yb:CaF2 laser

We present what we believe to be the first terawatt diode-pumped laser employing single-crystalline Yb:CaF(2) as the amplifying medium. A maximum pulse energy of 420 mJ at a repetition rate of 1 Hz was achieved by seeding with a stretched femtosecond pulse 2 ns in duration, preamplified to 40 mJ. After recompression, a pulse energy of 197 mJ and a duration of 192 fs were obtained, corresponding to a peak power of 1 TW. Furthermore, nanosecond pulses containing an energy of up to 905 mJ were generated without optical damage.

GeV-scale electron acceleration in a gas-filled capillary discharge waveguide

We report experimental results on laser-driven electron acceleration with low divergence. The electron beam was generated by focussing 750 mJ, 42 fs laser pulses into a gas-filled capillary discharge waveguide at electron densities in the range between 10 18 and 10 19 cm 3 . Quasi-monoenergetic electron bunches with energies as high as 500 MeV have been detected, with features reaching up to 1 GeV, albeit with large shot-to-shot fluctuations. A more stable regime with higher bunch charge (20-45 pC) and less energy (200-300 MeV) could also be observed. The beam divergence and the pointing stability are around or below 1 mrad and 8 mrad, respectively. These findings are consistent with self-injection of electrons into a breaking plasma wave.

Proton spectra from ultraintense laser-plasma interaction with thin foils: Experiments, theory, and simulation

A beam of high energy ions and protons is observed from targets irradiated with intensities up to 5×1019 W/cm2. Maximum proton energy is shown to strongly correlate with laser-irradiance on target. Energy spectra from a magnetic spectrometer show a plateau region near the maximum energy cutoff and modulations in the spectrum at approximately 65% of the cutoff energy. Presented two-dimensional particle-in-cell simulations suggest that modulations in the proton spectrum are caused by the presence of multiple heavy-ion species in the expanding plasma.

A laser-driven nanosecond proton source for radiobiological studies

Ion beams are relevant for radiobiological studies and for tumor therapy. In contrast to conventional accelerators, laser-driven ion acceleration offers a potentially more compact and cost-effective means of delivering ions for radiotherapy. Here, we show that by combining advanced acceleration using nanometer thin targets and beam transport, truly nanosecond quasi-monoenergetic proton bunches can be generated with a table-top laser system, delivering single shot doses up to 7 Gy to living cells. Although in their infancy, laser-ion accelerators allow studying fast radiobiological processes as demonstrated here by measurements of the relative biological effectiveness of nanosecond proton bunches in human tumor cells.

Spectral properties of laser-accelerated mid-Z MeV/u ion beams

Collimated jets of beryllium, carbon, oxygen, fluorine, and palladium ions with >1MeV∕nucleon energies are observed from the rear surface of thin foils irradiated with laser intensities of up to 5×1019W∕cm2. The normally dominant proton acceleration is suppressed when the target is subjected to Joule heating to remove hydrogen-bearing contaminant. This inhibits screening effects and permits effective energy transfer to and acceleration of heavier ion species. The influence of remnant protons on the spectral shape of the next highest charge-to-mass ratio species is shown. Particle-in-cell simulations confirming the experimental findings are presented.

Absolute charge calibration of scintillating screens for relativistic electron detection

We report on new charge calibrations and linearity tests with high-dynamic range for eight different scintillating screens typically used for the detection of relativistic electrons from laser-plasma based acceleration schemes. The absolute charge calibration was done with picosecond electron bunches at the ELBE linear accelerator in Dresden. The lower detection limit in our setup for the most sensitive scintillating screen (KODAK Biomax MS) was 10 fC/mm(2). The screens showed a linear photon-to-charge dependency over several orders of magnitude. An onset of saturation effects starting around 10-100 pC/mm(2) was found for some of the screens. Additionally, a constant light source was employed as a luminosity reference to simplify the transfer of a one-time absolute calibration to different experimental setups.

Comparative spectra and efficiencies of ions laser-accelerated forward from the front and rear surfaces of thin solid foils

The maximum energy of protons that are accelerated forward by high-intensity, short-pulse lasers from either the front or rear surfaces of thin metal foils is compared for a large range of laser intensities and pulse durations. In the regime of moderately long laser pulse durations (300–850fs), and for high laser intensities [(1−6)×1019W∕cm2], rear-surface acceleration is shown experimentally to produce higher energy particles with smaller divergence and a higher efficiency than front-surface acceleration. For similar laser pulse durations but for lower laser intensities (2×1018Wcm−2), the same conclusion is reached from direct proton radiography of the electric fields associated with proton acceleration from the rear surface. For shorter (30–100fs) or longer (1–10ps) laser pulses, the same predominance of rear-surface acceleration in producing the highest energy protons is suggested by simulations and by comparison of analytical models with measured values. For this purpose, we have revised our previous ...