Sunao Katsuki

Improvement of NO/sub X/ removal efficiency using short-width pulsed power

Pulsed power has been used to remove nitric oxide (NO) in a mixture of nitrogen, oxygen, and water vapor simulating the flue gases from a power station stack. The effect of the pulsewidth at a fixed applied voltage on NO removal concentration was studied. The dependence of the energy efficiency of the removal of NO at a fixed applied voltage on the pulsewidth, on the removal ratio of NO and on the discharge current was investigated. This removal energy efficiency increases with decreasing pulsewidth and decreasing removal ratio of NO.

Bacterial decontamination of water by means of pulsed-corona discharges

By using a tungsten wire with 75-/spl mu/m diameter, 2 cm apart from a plane cathode, and applying a 600-ns, 120-kV square wave pulse, we were able to obtain a pulsed-water corona discharge (PWC). The effect of these discharges on bacteria was studied using water contaminated with Escherichia coli or Bacillus subtilis, the latter in both the vegetative and spore state. The strongest effect was obtained on E. coli. The concentration of E. coli could be reduced by three orders of magnitude after applying eight corona discharges to the water. The corresponding energy expenditure is 10 J/cm/sup 3/. The decontamination rate had the largest values at the beginning, and decreased considerably after 15 electrical discharges, reaching a constant residual concentration value of 10/sup -4/ of the initial concentration. For B. subtilis in the vegetative state, it took almost 30 discharges to reach the same result, corresponding to an energy expenditure of 40 J/cm/sup 3/. There was no effect on B. subtilis spores. Comparisons with the pulsed-electric field (PEF) method indicate that the decontamination efficiency of the PWC method is slightly higher than that of the PEF method.

Pulsed streamer discharge characteristics of ozone production in dry air

Experimental investigation of HV short pulsed streamer discharges in dry air-fed ozonizers under various operating conditions are reported. Ozone concentration, energy input and ozone production yield (efficiency) were measured at various voltages (14 to 37 kV), pulse repetition rates (25 to 400 pulses per second, pps), flow rates (1.5 to 3.0 1/min) and different gap spacings (10 to 20 mm) at a pressure of 1.01/spl times/10/sup 5/ Pa in dry air. A spiral copper wire (1 mm in diameter) made to a cylindrical configuration (18 to 38 mm in diameter) in a concentric coaxial electrode system of various dimensions was employed. A magnetic pulse compressor provided the HV and current pulses. Higher voltage and higher repetition rates yielded higher concentrations of ozone at a fixed air flow rate. The present investigation was extended to assess the performance of this pulsed ozone generator using dry air under desired conditions of high concentration and high yield of ozone for industrial applications.

Thermal processes in a streamer discharge in water

The propagation features of a streamer discharge in water have been investigated. Based on the experimental data obtained in the study of water discharges in a nonuniform electric field, due propagation of streamers is explained as the evaporation of water at the tip of the streamer and around it. The energy balance in the process of the streamer propagation is calculated for a sub-microsecond discharge in distilled water. It is shown that the energy released in the pre-breakdown process is sufficient to evaporate the liquid in the streamer channels. Similar velocity of the streamer propagation in both tap and distilled water substantiates negligible effect of ionic current density onto the streamer propagation process. These estimations, based on experiment, have relevance to the discussion of the nature of the dielectric breakdown of water.

Propagation velocity of pulsed streamer discharges in atmospheric air

Pulsed streamer discharges have been extensively used in many applications such as control of NO/sub X/ and SO/sub 2/ from exhaust gases, treatment of dioxins, removal of volatile organic compounds, generation of ozone, and laser excitation. An operation with a high energy efficiency is necessary for practical applications. It is very important to know the propagation mechanism of streamer discharges in order to improve the energy efficiency of pulsed discharge systems. In this paper, the emission from pulsed streamer discharges in a coaxial electrode system in air at 0.1 MPa was observed using a high-speed gated intensified charge-coupled display camera. A concentric wire-cylinder electrodes configuration was used. A positive pulsed voltage having a width of about 100 ns was applied to the central electrode. The streamer discharges were initiated at the inner electrode and terminated at the outer electrode. The propagation velocity of the streamer discharges was 1.8-3.3 mm/ns.

Parallel streamer discharges between wire and plane electrodes in water

Streamer discharges in tap water and distilled water have been generated by applying a voltage pulse from 120 to 175 kV and 500 ns duration to a wire-to-electrode configuration. Electrical and optical diagnostics were used to explore the temporal development of the streamers in tap and distilled water, at various applied voltages and both polarities. With the wire serving as anode, multiple, parallel streamer discharges were generated. The number density of these streamers along the wire decreases with decreasing electric field on the surface of the wire. The dependence of the streamer density on electric field indicates the role of field enhancement at inhomogeneous microstructures along the wire as streamer initiation mechanism. The appearance of the discharge was different for tap and distilled water. However, the measured average streamer propagation velocity from the positive wire to the grounded plane electrode, of 32 mm//spl mu/s, was independent of the water conductivity and the applied voltage. This suggests the existence of a self-sustained electric field at the streamer head. With the wire serving as cathode, only a weak light emission from the area close to the wire was observed, and streamers did not appear for the same voltage amplitude as with the positive polarity. This suggests that an ionic current flowing in the water is not dominant in the streamer propagation process.

Biological effects of narrow band pulsed electric fields

This paper describes the process of narrow band pulsed electric fields (NPEFs) and its effect on mammalian cells. The NPEF consists of a pulse modulated sinusoidal wave (PMSW), which allows delivery of well-defined electric fields in terms of frequency, field strength and deposition energy to the biological systems. 100 mus long sinusoidal electric fields with a frequency of 0.02, 2 or 50 MHz and field strengths of up to 2 kV/cm are applied to CHO cells with variation in the DNA density in the cells investigated by means of Acridine Orange assay. The experiments indicate that 50 MHz fields cause DNA degradation without cell membrane defects, while 0.02 MHz fields lead to an increase in membrane permeability which is similar to the effect known as electroporation. The intermediate frequency of 2 MHz influences both the membrane and DNA. It is demonstrated that the MHz range narrowband electric fields with the amplitude level of 1 kV/cm cause intracellular effects in mammalian cells.

Electrical breakdown of water in microgaps

Experimental and modeling studies on electrical breakdown in water in submillimeter gaps between pin and plane electrodes have been performed. Prebreakdown, breakdown and recovery of the water gaps were studied experimentally by using optical and electrical diagnostics with a temporal resolution on the order of one nanosecond. By using Mach–Zehnder interferometry, the electric field distribution in the prebreakdown phase was determined by means of the Kerr effect. Electric fields values in excess of the computed electric fields, which reach >4 MV cm−1 for applied electrical pulses of 20 ns duration, were recorded at the tip of the pin electrode, an effect which can be explained by a reduced permittivity of water at high electric fields. Breakdown of the gaps, streamer-to-arc transition, was recorded by means of high-speed electrical diagnostics, and through high-speed photography. It was shown, through simulations, that breakdown is initiated by field emission at the interface of preexisting microbubbles. Impact ionization within the micro-bubbles gas then contributes to plasma development. Experiments using pulse–probe methods and Schlieren diagnostics allowed us to follow the development of the disturbance caused by the breakdown over a time of more than milliseconds and to determine the recovery time of a water switch. In order to trigger water switches a trigger electrode with a triple point has been utilized. The results of this research have found application in the construction of compact pulse power generators for bioelectric applications.

Positive- and Negative-Pulsed Streamer Discharges Generated by a 100-ns Pulsed-Power in Atmospheric Air

A Blumlein generator that has a pulsewidth of 100 ns was used to investigate the process of streamer discharge propagation in a coaxial cylindrical reactor using a streak camera. Both positive and negative polarities of the streamer discharges were performed in air at atmospheric pressure. The results showed that the primary and secondary streamers propagated with increasing velocity from the central rod to the outer cylinder electrode in both positive and negative polarities of applied voltages to the rod electrode. The propagation velocity of the streamer heads was in the range of 0.8-1.2 mm/ns for a positive peak applied voltage in the range of 43-60 kV and 0.6 mm/ns for a negative peak applied voltage of -93 kV, respectively. The electric field at streamer onset was calculated to be 12 and 20 MV/m for positive and negative applied voltages, respectively.

Electron Temperature and Electron Density of Underwater Pulsed Discharge Plasma Produced by Solid-State Pulsed-Power Generator

A pulsed discharge produced underwater has been an attractive method to treat waste water. For the optimization and realization of the water treatment system utilizing underwater pulsed discharge, modeling analysis could be one of the essential works. However, there is still no simulation work about the underwater pulsed discharge due to the lack of knowledge about its characteristic parameters such as electron temperature, electron density, and so on. In this paper, the temperature and the electron density in a pulsed discharge plasma produced underwater are measured and presented. A magnetic pulse compressor (MPC) was developed and used to create the electrical discharge in water. The developed MPC is all-solid state and is, therefore, a maintenance-free generator. To define the temperature and the electron density in an underwater pulsed discharge plasma, two kinds of spectroscopic measurements, called the line-pair method and Stark broadening, were carried out. According to the experimental results, the temperature and the electron density in the pulsed discharge plasma between point-plane electrodes immersed in water are determined to be 15000 K and 1018/cm3, respectively.