Sy Stange

Plasma-enhanced combustion of propane using a silent discharge

It is well known that applying an electric field to a flame can affect its propagation speed, stability, and combustion chemistry. External electrodes, arc discharges, plasma jets, and corona discharges have been employed to allow combustible gas mixtures to operate outside their flammability limits or to increase combustion speed. Previously reported experiments have involved silent electrical discharges applied to propagating flames. These demonstrated that the flame propagation velocity can be increased when the discharge is applied to the unburned gas mixture upstream of a flame. In contrast, the work reported here used a coaxial-cylinder, nonthermal, silent discharge plasma reactor to activate a propane gas stream before it was mixed with air and ignited. With the plasma, the physical appearance of the flame changes (increased stability) and substantial changes in mass spectrometer peaks are observed, indicating that the combustion process is enhanced with the application of the plasma.

On collisionless ion and electron populations in the magnetic nozzle experiment (MNX)

The Magnetic Nozzle Experiment (MNX) is a linear magnetized helicon-heated plasma device, with applications to advanced spacecraft-propulsion methods and solar-corona physics. This paper reviews ion and electron energy distributions measured in MNX with laser-induced fluorescence (LIF) and probes, respectively. Ions, cold and highly collisional in the main MNX region, are accelerated along a uniform magnetic field to sonic then supersonic speeds as they exit the main region through either mechanical or magnetic apertures. A sharp decrease in density downstream of the aperture(s) helps effect a transition from collisional to collisionless plasma. The electrons in the downstream region have an average energy somewhat higher than that in the main region. From LIF ion-velocity measurements, we find upstream of the aperture a presheath of strength Deltaphips=mrTe, where mrTe is the electron temperature in the main region, and length ~3 cm, comparable to the ion-neutral mean-free-path; immediately downstream of the aperture is an electrostatic double layer of strength DeltaphiDL=3-10 mrTe and length 0.3-0.6 cm, 30-600lambdaD. The existence of a small, ca. 0.1%, superthermal electron population with average energy ~10 mrTe is inferred from considerations of spectroscopic line ratios, floating potentials, and Langmuir probe data. The superthermal electrons are suggested to be the source for the large DeltaphiDL

Flame images indicating combustion enhancement by dielectric barrier discharges

The capability of a plasma to enhance combustion has significant practical implications. We present pictures showing the effect of a dielectric barrier discharge applied to propane prior to combustion. The plasma causes an increase in the flame propagation rate, attributed to the production of reactive radicals and fuel fragments in the plasma.

Theoretical and experimental studies of kinetic equilibrium and stability of the virtual cathode in an electron injected inertial electrostatic confinement device

This paper explores the electron-electron two-stream stability limit of a virtual cathode in spherical geometry. Previous work using a constant density slab model [R. A. Nebel and J. M. Finn, Phys. Plasmas 8, 1505 (2001)] suggested that the electron-electron two-stream would become unstable when the well depth of the virtual cathode was 14% of the applied voltage. However, experimental tests on INS-e have achieved virtual cathode fractional well depths ∼60% with no sign of instability. Here, studies with a spherical gridless particle code indicate that fractional well depths greater than 90% can be achieved without two-stream instabilities. Two factors have a major impact on the plasma stability: whether the particles are reflected and the presence of angular momentum. If the particles are reflected then they are guaranteed to be in resonance with the electron plasma frequency at some radius. This can lead to the two stream instabilities if the angular momentum is small. If the angular momentum is large e...

Periodically oscillating plasma sphere

The periodically oscillating plasma sphere, or POPS, is a novel fusion concept first proposed by D. C. Barnes and R. A. Nebel [Fusion Technol. 38, 28 (1998)]. POPS utilizes the self-similar collapse of an oscillating ion cloud in a spherical harmonic oscillator potential well formed by electron injection. Once the ions have been phase-locked, their coherent motion simultaneously produces very high densities and temperatures during the collapse phase of the oscillation. A requirement for POPS is that the electron injection produces a stable harmonic oscillator potential. This has been demonstrated in a gridded inertial electrostatic confinement device and verified by particle simulation. Also, the POPS oscillation has been confirmed experimentally through observation that the ions in the potential well exhibit resonance behavior when driven at the POPS frequency. Excellent agreement between the observed POPS frequencies and the theoretical predictions has been observed for a wide range of potential well de...

Large-scale synthesis of CexLa1−xF3 nanocomposite scintillator materials

Transparent nanocomposites have been developed which consist of nanocrystals embedded in an organic matrix. The materials are comprised of up to 60% by volume of 7–13 nm crystals of the phosphor CexLa1−xF3, and are greater than 70% transparent in the visible region at a thickness of 1 cm. Consistencies of the nanocomposites range from a solid polymer to a wax to a liquid, depending on the workup conditions of the nanoparticle synthesis. These transparent nanophosphor composite materials have potential applications in radiation detection as scintillators, as well as in other areas such as imaging and lighting, and can be produced on large scales up to near-kilogram quantities at near ambient conditions, much lower in temperature than typical nanoparticle syntheses.

LaF3:Ce nanocomposite scintillator for gamma-ray detection

Nanophosphor LaF3:Ce has been synthesized and incorporated into a matrix to form a nanocomposite scintillator suitable for application to γ-ray detection. Owing to the small nanocrystallite size (sub-10 nm), optical emission from the γ / nanophosphor interaction is only weakly Rayleigh scattered (optical attenuation length exceeds 1 cm for 5-nm crystallites), thus yielding a transparent scintillator. The measured energy resolution is ca. 16% for 137Cs γ rays, which may be improved by utilizing brighter nanophosphors. Synthesis of the nanophosphor is achieved via a solution-precipitation method that is inexpensive, amenable to routine processing, and readily scalable to large volumes. These results demonstrate nanocomposite scintillator proof-of- principle and provide a framework for further research in this nascent field of scintillator research.

Enhancement of Propane Flame Stability by Dielectric Barrier Discharges

Abstract Non-thermal plasmas have recently found novel applications in improving fuel combustion. Typical electron temperatures in such plasmas are of order a few electron volts. Such electrons are sufficient to break down fuel molecules and to produce free radicals which may significantly affect combustion efficiency. In this work, we use a dielectric barrier discharge (DBD) to activate propane (C3H8) fuel before it is mixed with air and ignited. The use of activated propane enables us to operate combustion in very lean-burn conditions; for 0.2 lpm propane, air flow was 38 lpm, compared with an air flow of 26 lpm in the absence of a plasma. A residual gas analyzer (RGA) measures the decomposition products of the propane discharge, indicating that atomic and molecular hydrogen are produced in the plasma and that their concentrations depend on the DBD energy density. Based on the observations discussed in this work, we have shown that by activating propane, the DBD increases combustion stability.

Development of a Liquid Scintillator Neutron Multiplicity Counter (LSMC)

A new neutron multiplicity counter is being developed that utilizes the fast response of liquid scintillator detectors. The ability to detect fast (vs. moderated) fission neutrons makes possible a coincidence gate on the order of tens of nanoseconds (vs. tens of microseconds). A neutron counter with such a narrow gate will be much less sensitive to accidental coincidences making it possible to measure items with a high single neutron background to greater accuracy in less time. This includes impure Pu items with high (alpha,n) rates as well as items of low mass HEU where a strong active interrogation source is needed. Liquid scintillator detectors also allow for energy discrimination between interrogation source neutrons and fission neutrons, allowing for even greater assay sensitivity. Designing and building a liquid scintillator multiplicity counter (LSMC) requires a symbiotic effort of simulation and experiment to optimize performance and mitigate hardware costs in the final product. We present preliminary Monte Carlo studies using the GEANT toolkit along with analysis of experimental data used to benchmark and tune the simulation.

Comparison of Fast Neutron Detector Technologies

This report documents the work performed for the Department of Homeland Security Domestic Nuclear Detection O ce as the project Fast Neutron Detection Evaluation under contract HSHQDC-14-X-00022. This study was performed as a follow-on to the project Study of Fast Neutron Signatures and Measurement Techniques for SNM Detection - DNDO CFP11-100 STA-01. That work compared various detector technologies in a portal monitor con guration, focusing on a comparison between a number of fast neutron detection techniques and two standard thermal neutron detection technologies. The conclusions of the earlier work are contained in the report Comparison of Fast Neutron Detector Technologies. This work is designed to address questions raised about assumptions underlying the models built for the earlier project. To that end, liquid scintillators of two di erent sizes{ one a commercial, o -the-shelf (COTS) model of standard dimensions and the other a large, planer module{were characterized at Los Alamos National Laboratory. The results of those measurements were combined with the results of the earlier models to gain a more complete picture of the performance of liquid scintillator as a portal monitor technology.