T. Renstrøm

Observation of Large Scissors Resonance Strength in Actinides

The orbital M1 scissors resonance has been measured for the first time in the quasicontinuum of actinides. Particle-γ coincidences are recorded with deuteron and (3)He-induced reactions on (232)Th. The residual nuclei (231,232,233)Th and (232,233) Pa show an unexpectedly strong integrated strength of B(M1)=11-15μ(n)(2) in the E(γ)=1.0-3.5 MeV region. The increased γ-decay probability in actinides due to scissors resonance is important for cross-section calculations for future fuel cycles of fast nuclear reactors and may also have an impact on stellar nucleosynthesis.

Novel technique for constraining r -process (n, γ) reaction rates

A novel technique has been developed, which will open exciting new opportunities for studying the very neutron-rich nuclei involved in the r process. As a proof of principle, the γ spectra from the β decay of ^{76}Ga have been measured with the SuN detector at the National Superconducting Cyclotron Laboratory. The nuclear level density and γ-ray strength function are extracted and used as input to Hauser-Feshbach calculations. The present technique is shown to strongly constrain the ^{75}Ge(n,γ)^{76}Ge cross section and reaction rate.

Constant-temperature level densities in the quasicontinuum of Th and U isotopes

Particle-gamma coincidences have been measured to obtain gamma-ray spectra as a function of excitation energy for 231-233Th and 237-239U. The level densities, which were extracted using the Oslo method, show a constant temperature behavior. The isotopes display very similar temperatures in the quasi-continuum, however, the even-odd isotopes reveal a constant entropy increase Delta S compared to their even-even neighbors. The entropy excess depends on available orbitals for the last unpaired valence neutron of the heated nuclear system. Also, experimental microcanonical temperature and heat capacity have been extracted. Several poles in the heat capacity curve support the idea that an almost continuous melting of Cooper pairs is responsible for the constant-temperature behavior.

Transitional

The level densities and γ-ray strength functions of 105 ,106,111,112Cd have been extracted from particle-γ coincidence data using the Oslo method. The level densities are in very good agreement with known levels at low excitation energy. The γ-ray strength functions display no strong enhancement for low γ energies. However, more low-energy strength is apparent for 105,106Cd than for 111,112Cd. For γ energies above ≈4 MeV, there is evidence for some extra strength, similar to what has been previously observed for the Sn isotopes. The origin of this extra strength is unclear; it might be due to E1 and M1 transitions originating from neutron skin oscillations or the spin-flip resonance, respectively.

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Nuclear reactions where an exotic nucleus captures a neutron are critical for a wide variety of applications, from energy production and national security, to astrophysical processes, and nucleosynthesis. Neutron capture rates are well constrained near stable isotopes where experimental data are available; however, moving far from the valley of stability, uncertainties grow by orders of magnitude. This is due to the complete lack of experimental constraints, as the direct measurement of a neutron-capture reaction on a short-lived nucleus is extremely challenging. Here, we report on the first experimental extraction of a neutron capture reaction rate on ^{69}Ni, a nucleus that is five neutrons away from the last stable isotope of Ni. The implications of this measurement on nucleosynthesis around mass 70 are discussed, and the impact of similar future measurements on the understanding of the origin of the heavy elements in the cosmos is presented.

strength in Cd isotopes

Neutron-rich {96,98}Sr isotopes have been investigated by safe Coulomb excitation of radioactive beams at the REX-ISOLDE facility. Reduced transition probabilities and spectroscopic quadrupole moments have been extracted from the differential Coulomb excitation cross sections. These results allow, for the first time, the drawing of definite conclusions about the shape coexistence of highly deformed prolate and spherical configurations. In particular, a very small mixing between the coexisting states is observed, contrary to other mass regions where strong mixing is present. Experimental results have been compared to beyond-mean-field calculations using the Gogny D1S interaction in a five-dimensional collective Hamiltonian formalism, which reproduce the shape change at N=60.

Experimental Neutron Capture Rate Constraint Far from Stability

We investigated the U238(d,p) reaction as a surrogate for the n+U238 reaction. For this purpose we measured for the first time the γ-decay and fission probabilities of U∗239 simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels method and the distorted-wave Born approximation (DWBA) were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where fission and γ emission compete, the corrected fission probability is in agreement with neutron-induced data, whereas the γ-decay probability is much higher than the neutron-induced data. We have performed calculations of the decay probabilities with the statistical model and of the average angular momentum populated in the U238(d,p) reaction with the DWBA to interpret these results.

Spectroscopic Quadrupole Moments in {96,98}Sr: Evidence for Shape Coexistence in Neutron-Rich Strontium Isotopes at N=60.

We analyze primary γ-ray spectra of the odd-odd (238)Np nucleus extracted from (237)Np(d,pγ)(238)Np coincidence data measured at the Oslo Cyclotron Laboratory. The primary γ spectra cover an excitation-energy region of 0≤E(I)≤5.4  MeV, and allow us to perform a detailed study of the γ-ray strength as a function of excitation energy. Hence, we can test the validity of the generalized Brink-Axel hypothesis, which, in its strictest form, claims no excitation-energy dependence on the γ strength. In this work, using the available high-quality (238)Np data, we show that the γ-ray strength function is to a very large extent independent of the initial and final states. Thus, for the first time, the generalized Brink-Axel hypothesis is experimentally verified for γ transitions between states in the quasicontinuum region, not only for specific collective resonances, but also for the full strength below the neutron separation energy. Based on our findings, the necessary criteria for the generalized Brink-Axel hypothesis to be fulfilled are outlined.

Investigation of the U238(d,p) surrogate reaction via the simultaneous measurement of γ-decay and fission probabilities

Author(s): Renstrom, T; Nyhus, HT; Utsunomiya, H; Schwengner, R; Goriely, S; Larsen, AC; Filipescu, DM; Gheorghe, I; Bernstein, LA; Bleuel, DL; Glodariu, T; Gorgen, A; Guttormsen, M; Hagen, TW; Kheswa, BV; Lui, YW; Negi, D; Ruud, IE; Shima, T; Siem, S; Takahisa, K; Tesileanu, O; Tornyi, TG; Tveten, GM; Wiedeking, M | Abstract:

Validity of the generalized Brink-Axel hypothesis in

Author(s): Renstrom, T; Nyhus, HT; Utsunomiya, H; Schwengner, R; Goriely, S; Larsen, AC; Filipescu, DM; Gheorghe, I; Bernstein, LA; Bleuel, DL; Glodariu, T; Gorgen, A; Guttormsen, M; Hagen, TW; Kheswa, BV; Lui, YW; Negi, D; Ruud, IE; Shima, T; Siem, S; Takahisa, K; Tesileanu, O; Tornyi, TG; Tveten, GM; Wiedeking, M | Abstract: