Takatsugu Masuda

Competition between helimagnetism and commensurate quantum spin correlations in LiCu2O2

Neutron diffraction and bulk measurements are used to determine the nature of the low-temperature ordered state in LiCu2O2, a S=1/2 spin-chain compound with competing interactions. The spin structure is found to be helimagnetic, with a propagation vector (0.5,zeta,0), zeta=0.174. The nearest-neighbor exchange constant and frustration ratio are estimated to be J(1)=5.8 meV and J(2)/J(1)=0.29, respectively. For idealized quantum spin chains, these parameter values would signify a gapped spin-liquid ground state with commensurate spin correlations. The observed temperature dependence of the magnetic propagation vector in LiCu2O2 is attributed to a competition between incommensurate helimagnetism in the classical spin model and commensurability in the quantum case. It is also proposed that long-range ordering in LiCu2O2 is facilitated by intrinsic nonstoichiometry.

Spin Waves and Magnetic Interactions in LiCu2O2

The quasi-one-dimensional helimagnet LiCu{sub 2}O{sub 2} was studied by single crystal inelastic neutron scattering. The dispersion relation of spin wave excitations was measured in the vicinity of the principal magnetic Bragg reflection. A spin wave theoretical analysis of the data yields an estimate of the relevant exchange constants and explains the mechanism of geometric frustration that leads to helimagnetism. It is found that the simple antiferromagnetic J{sub 1}-J{sub 2} model that was previously proposed is inadequate for LiCu{sub 2}O{sub 2}. The experimental findings are generally in a qualitative agreement with first principles calculations of [A. A. Gippius, E. N. Morozova, A. S. Moskvin, A. V. Zalessky, A. A. Bush, M. Baenitz, H. Rosner, and S.-L. Drechsler, Phys. Rev. B 70, 020406 (2004)], though certain important discrepancies remain to be explained.

Dynamics of composite haldane spin chains in IPA-CuCl3

Magnetic excitations in the quasi-one-dimensional antiferromagnet IPA-CuCl3 are studied by cold neutron inelastic scattering. Strongly dispersive gap excitations are observed. Contrary to previously proposed models, the system is best described as an asymmetric quantum spin ladder. The observed spectrum is interpreted in terms of composite Haldane spin chains. The key difference from actual S=1 chains is a sharp cutoff of the single-magnon spectrum at a certain critical wave vector.

Longitudinal spin density wave order in a quasi-1D Ising-like quantum antiferromagnet.

From neutron diffraction measurements on a quasi-1D Ising-like Co2+ spin compound BaCo2V2O8, we observed an appearance of a novel type of incommensurate ordering in magnetic fields. This ordering is essentially different from the Néel-type ordering, which is expected for the classical system, and the peculiar spin structure is caused by quantum fluctuation inherent in the quantum spin chain. A Tomonaga-Luttinger liquid nature characteristic of the gapless quantum 1D system is responsible for the realization of the incommensurate ordering.

Excitations from a Bose-Einstein Condensate of Magnons in Coupled Spin Ladders

The weakly coupled quasi-one-dimensional spin ladder compound (CH3)2CHNH3CuCl3 is studied by neutron scattering in magnetic fields exceeding the critical field of Bose-Einstein condensation of magnons. Commensurate long-range order and the associated Goldstone mode are detected and found to be similar to those in reference to spin-dimer materials. However, for the upper two massive magnon branches, the observed behavior is totally different, culminating in a drastic collapse of excitation bandwidth beyond the transition point.

Spin-nematic interaction in the multiferroic compound Ba2CoGe2O7.

We demonstrate the existence of the spin-nematic interactions in an easy-plane type antiferromagnet Ba2CoGe2O7 by exploring the magnetic anisotropy and spin dynamics. The combination of neutron scattering and magnetic susceptibility measurements reveals that the origin of the in-plane anisotropy is an antiferro-type interaction of the spin-nematic operator. The relation between the nematic operator and the electric polarization in the ligand symmetry of this compound is presented. The introduction of the spin-nematic interaction is useful to understand the physics of spin and electric dipole in multiferroic compounds.

Instability of magnons in two-dimensional antiferromagnets at high magnetic fields

Spin dynamics of the square lattice Heisenberg antiferromagnet,

Cooperative Ordering of Gapped and Gapless Spin Networks in Cu2Fe2Ge4O13

{\text{Ba}}_{2}{\text{MnGe}}_{2}{\text{O}}_{7}

Energy separation of single-particle and continuum states in an S = 1/2 weakly coupled chains antiferromagnet

, is studied by a combination of bulk measurements, neutron diffraction, and inelastic neutron-scattering techniques. Easy plane type antiferromagnetic order is identified at

Magnetic excitations in the weakly coupled spin dimers and chains material Cu 2 Fe 2 Ge 4 O 13

T\ensuremath{\le}4.0\text{ }\text{K}