Tatsuo Iyoku

Development of an Evaluation Model for the Thermal Annealing Effect on Thermal Conductivity of IG-110 Graphite for High-Temperature Gas-Cooled Reactors

The thermal conductivity of graphite components used as in-core components in high-temperature gascooled reactors (HTGRs) is reduced by neutron irradiation during reactor operation. The reduction in thermal conductivity is expected to be reversed by thermal annealing when the irradiated graphite component is heated above its original irradiation temperature. In this study, to develop an evaluation model for the thermal annealing effect on the thermal conductivity of IG-110 graphite for the HTGRs, the thermal annealing effect evaluated quantitatively at irradiation temperatures of up to 1,200°C and neutron fluences of up to 1.5 dpa. Moreover, the thermal conductivity of IG-110 graphite was calculated by using a modified thermal resistance model considering the thermal annealing effect. The following results were obtained. (1) The thermal annealing effect on the thermal conductivity of IG-110 graphite could be evaluated quantitatively and a thermal annealing model was developed based on the experimental results at irradiation temperatures of up to 1,200°C and neutron fluences of up to 1.5 dpa. (2) The thermal conductivities of IG-110 graphite calculated by using the modified thermal resistance model considering the thermal annealing effect showed good agreement with experimental measurements. This study has shown that it is possible to evaluate the annealed thermal conductivity of IG-110 graphite by using the modified thermal resistance model at irradiation temperatures of 550–1150°C and irradiation fluences of up to 1.5 dpa.

Operation and maintenance experience from the HTTR database

The Japan Atomic Energy Agency has been establishing a database of operation and maintenance experience for the High Temperature Engineering Test Reactor. The objective of this database is to share information from operation and maintenance experience and make use of the knowledge gained in the design, construction, and operation of future High Temperature Gas-cooled Reactors (HTGRs). Between 1997 and 2012, more than 1000 events have been registered in this database system. This paper describes trends in operation and maintenance events recorded in this database, including experience gained from the Great East Japan Earthquake. The paper also identifies the following significant items that are expected to be useful in the design of future HTGRs: (1) performance degradation of helium gas compressors, (2) malfunction of the reserved shutdown system in the reactivity control system, (3) problems with emergency gas turbine generators, and (4) consequences of the Great East Japan Earthquake.

Experience and Future Plan of Test Operation Using HTTR

The High Temperature Engineering Test Reactor (HTTR) is the first high-temperature gas-cooled reactor (HTGR) in Japan. The HTTR is a graphite-moderated and helium gas-cooled reactor with thermal power of 30MW and the maximum reactor outlet coolant temperature of 950°C. Main objectives of the HTTR are to establish and develop HTGR technology and to demonstrate process heat application. The HTTR has conducted two test operations which are safety demonstration test and continuous operation. The safety demonstration tests focus on the verification of the inherent safety features of the HTGR that is the negative reactivity feedback effect of the core brings the reactor power safely to a safe and stable level without a reactor scram and the temperature transient of the reactor is slow in case of anticipated operational occurrences (AOOs). The safety demonstration tests include reactivity insertion test, coolant flow reduction test and loss of forced cooling (LOFC) test. Reactivity insertion test and coolant flow reduction test have been conducted since 2002. These tests demonstrated the inherent safety features of the HTGR in case of reactivity insertion and coolant flow reduction, and provided valuable data for code validation. LOFC test will start in the middle of 2010. LOFC is one of the important accident scenarios in the safety assessment of the HTGR. This test result will show extreme safety features of the HTGR and further improve the safety design approach of the HTGR. Obtained data can be useful to validate plant safety analysis codes. The continuous operation has been conducted to obtain plant data to establish HTGR technology and to demonstrate capability of the HTTR to supply stable heat to heat utilization system for long-term. Two operations of 30-day continuous operation in rated operation mode (in which designed reactor outlet coolant temperature of 850°C) and 50-days continuous operation in high temperature test operation mode (in which designed reactor outlet coolant temperature of 950°C) have been conducted so far. The 30-day continuous operation was achieved in 2007 and a good fuel performance to retain fission products within the coated fuel particle was clarified. The HTTR conducts 50-days continuous operation in 2010 to add useful operation data at high temperature to improve technical basis of HTGR and to realize high temperature heat application of HTGR.Copyright

Principle Design of Graphite Components for HTTR and R&D on Nuclear Graphite for HTGR in JAEA

Nuclear energy is one of the most promising energy sources to satisfy energy security, environmental protection, and efficient supply. The High Temperature Gas-cooled Reactor (HTGR) has attractive inherent safety features and it can be used as many kinds of heat applications such as hydrogen production, electricity generation, process heat supply, district heating and desalination. Many countries, especially developing countries, show their interests in HTGR. Graphite materials are used for the core components of the HTGR. IG-110 graphite, fine-grained isotropic graphite, with high strength and high oxidation resistance is used in the High temperature Engineering Test Reactor (HTTR) of Japan Atomic Energy Agency (JAEA) and High Temperature Reactor-Pebble-bed Modules (HTR-PM) in China. IG-110 graphite is a major candidate for the core graphite components of the Very High Temperature Reactor (VHTR) which is one of HTGRs and one of the most promising candidates as the Generation-IV nuclear reactor systems. This paper describes design of core components of HTTR and R&D on nuclear graphite for HTGR. JAEA established the graphite structural design code and inspection standard of graphite to construct the HTTR. JAEA developed an in-service inspection method and a draft graphite structural design code for future HTGR on the basis of the HTTR technologies. Moreover, JAEA are now developing the design data base of IG-110 graphite and IG-430 graphite including irradiation data for HTGR.

ICONE15-10582 Present status of HTTR and its Operational Experience

A High Temperature Gas-cooled Reactor (HTGR) is particularly attractive because of its capability of producing high temperature helium gas and its inherent safety characteristics. Hence, the High Temperature Engineering Test Reactor (HTTR) was successfully constructed at the Oarai Research Establishment of the Japan Atomic Energy Agency. The HTTR achieved the full power of 30MW and reactor outlet coolant temperature of about 850oC on December 7, 2001. After several operation cycles, the HTTR achieved the reactor outlet coolant temperature of 950oC on April 19, 2004. It is the highest coolant temperature outside reactor pressure vessel in the world. This is one of the major milestones in HTGR development of high temperature nuclear process heat application. Extensive tests are planned in the HTTR and a process heat application system will be coupled to the HTTR, where hydrogen will be produced directly from the nuclear energy. This paper gives an overview of the HTTR Project focusing on the latest results from the HTTR test and the future test plan using the HTTR.

Analytical Study on Micro-Indentation Method to Integrity Evaluation for Graphite Components in HTGR

An analytical study on micro-indentation method to integrity evaluation for graphite components was carried out. The indentation method is used as simplicity test to measure mechanical properties of materials. This method is thought to be applicable to evaluate the residual stress from the relationship between indentation load and indentation depth. In this study, in order to confirm the applicability of the micro-indentation method for lifetime evaluation of the graphite component, indentation load-depth behavior under stress/strain condition was evaluated taking account of the specified minimum ultimate strength of IG-110 graphite. Moreover, analytical investigations of indentation load-depth behavior for oxidized graphite and oxidized graphite with residual strain were also carried out. As a result, it can be said that the indentation method is potentially applicable to evaluate the integrity of graphite components. (authors)

Anisotropic Deformation Effect on the Fracture of Core Components Made of Two-Dimensional C/C Composite

The carbon fiber reinforced carbon-carbon composite (C/C composite) is one of the candidates due to its excellent thermal stability as well as high strength. A two-dimensional C/C composite has great anisotropy in those properties in with- and across- fiber directions. It is, therefore, important to consider the anisotropy for the stress evaluation and for the fracture probability of the components. In the present study, FEM analyses on deformation and stress of the component were carried out taking account of the anisotropy. In addition, the fracture probability of the components was evaluated by the statistical fracture theory. It was found that anisotropy affect the thermal stress and the risk of rupture.

Study on Structural Integrity of C/C Composite Using as Core Restraint Mechanism in HTGR

High temperature gas cooled reactor (HTGR) with higher outlet coolant temperature nearly 1000°C is expected for direct utilization of process heat to hydrogen production. The thermal analysis of reactor internals with 3 dimensional, flow paths coupled model was conducted to demonstrate how strictly PSR block gaps must be closed to limit core bypass flow rate ratio lest fuel temperature should exceed admissible level, and the highly heat resistant core restraint mechanism must be developed in consequence. Potential applicability of the core restraint mechanism made of C/C composite, the attractive candidate material, was demonstrated by point design with adequate thickness and FEM stress analysis for material with orthotropic anisotropy .

Annealing Effect of Thermal Conductivity on Thermal Stress Induced Fracture of Nuclear Graphite

Graphite materials are used for structural components in the core of high temperature gas-cooled reactors (HTGRs) because of their excellent thermo/mechanical properties. When the core temperature is raised at an accident, the thermal stress of the components is induced, and it enhances the fracture probability of them. In general, the thermal conductivity of graphite is decreased by neutron irradiation due to irradiation-induced defects preventing heat conduction by phonon. It is hence expected that decreased thermal conductivity is recovered to some extent by thermal annealing at the accident. Therefore, the consideration of the thermal annealing effect is placed as much important subject in the fracture/strength evaluation of the graphite components at the accident. In the present study, the thermal stress and the fracture probability of graphite components influenced by the thermal annealing were investigated by a finite element method (FEM) analysis. It was shown that the annealing effect decreases the thermal stress and a certain level of the fracture probability.

Basic Concept on Structural Design Criteria for Zirconia Ceramics Applying to Nuclear Components

As an advanced in-core material in high temperature gas-cooled reactors (HTGRs), superplastic ceramics is attractive due to the possibility of the plastic working. For the application to the nuclear fields, the basic concept of design criteria was studied for typical superplastic ceramics, tetragonal zirconia polycrystals containing 3mol% yttria (3Y-TZP). The experimental results on 3Y-TZP showed that it is possible to apply the Weibull weakest-link theory to decide the stress limits in the criteria. The Weibull parameter m was evaluated as 9.5 for the bending and as 26.5 for the compressive. The applicability of the Weibull theory was also verified by the bending test results with different span. Based on the graphite structural design guidelines for the High Temperature Engineering Test Reactor (HTTR), the design stress limits for 3Y-TZP was proposed. It was shown that the proposed stress limits have appropriate safety margin and thought to be effective to evaluate the integrity of in-core structure made of 3Y-TZP.