Theodore B. Norris

Graphene photodetectors with ultra-broadband and high responsivity at room temperature

The ability to detect light over a broad spectral range is central to several technological applications in imaging, sensing, spectroscopy and communication. Graphene is a promising candidate material for ultra-broadband photodetectors, as its absorption spectrum covers the entire ultraviolet to far-infrared range. However, the responsivity of graphene-based photodetectors has so far been limited to tens of mA W(-1) (refs 5-10) due to the small optical absorption of a monolayer of carbon atoms. Integration of colloidal quantum dots in the light absorption layer can improve the responsivity of graphene photodetectors to ∼ 1 × 10(7) A W(-1) (ref. 11), but the spectral range of photodetection is reduced because light absorption occurs in the quantum dots. Here, we report an ultra-broadband photodetector design based on a graphene double-layer heterostructure. The detector is a phototransistor consisting of a pair of stacked graphene monolayers (top layer, gate; bottom layer, channel) separated by a thin tunnel barrier. Under optical illumination, photoexcited hot carriers generated in the top layer tunnel into the bottom layer, leading to a charge build-up on the gate and a strong photogating effect on the channel conductance. The devices demonstrated room-temperature photodetection from the visible to the mid-infrared range, with mid-infrared responsivity higher than 1 A W(-1), as required by most applications. These results address key challenges for broadband infrared detectors, and are promising for the development of graphene-based hot-carrier optoelectronic applications.

Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate

We demonstrate a promising technique for generating narrow-band terahertz electromagnetic radiation. Femtosecond optical pulses are propagated through a periodically poled lithium-niobate crystal, where the domain length is matched to the walk-off length between the optical and THz pulses. The bandwidth of the THz wave forms is 0.11 at 1.7 THz. Optical rectification gives rise to a THz wave form which corresponds to the domain structure of the periodically poled lithium niobate.

Femtosecond pulse amplification at 250 kHz with a Ti:sapphire regenerative amplifier and application to continuum generation.

Ultrashort optical pulses have been amplified to 1.7 μJ of energy at a repetition rate of 250 kHz with a novel cw argon-pumped Ti:sapphire regenerative amplifier. Acousto-optic switching of the amplifier is used to achieve the high repetition rate. Chirped-pulse amplification is used to avoid nonlinear effects in the amplifier. After recompression, 1-μJ, 130-fs pulses are obtained and are used to generate a white-light continuum in an ethylene glycol jet.

Enhanced two-photon biosensing with double-clad photonic crystal fibers

A double-clad photonic crystal fiber was used to improve detection efficiency over a standard single-mode fiber in a two-photon fluorescence detection scheme in which the dye was excited and the fluorescence was detected back through the same fiber.

In(Ga)As/GaAs self-organized quantum dot lasers: DC and small-signal modulation properties

Self-organized growth of InGaAs/GaAs strained epitaxial layers gives rise to an ordered array of islands via the Stranski-Krastanow growth mode, for misfits >1.8%. These islands are pyramidal in shape with a base diagonal of /spl sim/20 nm and height of /spl sim/6-7 nm, depending of growth parameters. They therefore exhibit electronic properties of zero-dimensional systems, or quantum dots. One or more layers of such quantum dots can be stacked and vertically coupled to form the gain region of lasers. We have investigated the properties of such single-layer quantum dot (SLQD) and multilayer quantum dot (MLQD) lasers with a variety of measurements, including some at cryogenic temperatures. The experiments have been complemented with theoretical calculations of the electronic properties and carrier scattering phenomena in the dots. Our objective has been to elucidate the intrinsic behavior of these devices. The lasers exhibit temperature independent threshold currents up to 85 K, with T/sub 0//spl les/670 K. Typical threshold currents of 200-/spl mu/m long room temperature lasers vary from 6 to 20 mA. The small-signal modulation bandwidths of ridge waveguide lasers are 5-7.5 GHz at 300 K and increased to >20 GHz at 80 K. These bandwidths agree well with electron capture times of /spl sim/30 ps determined from high-frequency laser impedance measurements at 300 K and relaxation times of /spl sim/8 ps measured at 18 K by differential transmission pump-probe experiments. From the calculated results we believe that electron-hole scattering intrinsically limits the high-speed performance of these devices, in spite of differential gains as high as /spl sim/7/spl times/10/sup -14/ cm/sup 2/ at room temperature.

Temperature dependence of narrow-band terahertz generation from periodically poled lithium niobate

Femtosecond optical pulses are used to generate narrow-band terahertz wave forms via optical rectification in a periodically poled lithium niobate crystal. By cooling the crystal to reduce losses due to phonon absorption, we are able to obtain bandwidths as narrow as 18 GHz at a carrier frequency of 1.8 THz. Temperature-dependent measurements show insignificant bandwidth broadening between 10 and 120 K, although the terahertz power substantially decreases as the temperature increases. Absolute power measurements indicate a conversion efficiency of at least 10−5.

Single Particle Plasmon Spectroscopy of Silver Nanowires and Gold Nanorods

The excitation of surface plasmons in individual silver nanowires and gold nanorods is investigated by means of high-resolution electron energy loss spectroscopy in a transmission electron microscope. The transverse and longitudinal modes of these nanostructures are resolved, and the size variation of the plasmon peaks is studied. The effect of electromagnetic coupling between closely spaced nanoparticles is also observed. Finally, the relation between energy-loss measurements and optical spectroscopy of nanoparticle plasmon modes is discussed.

Real-time biomolecular binding detection using a sensitive photonic crystal biosensor.

Real-time measurement of specific biomolecular interactions is critical to many areas of biological research. A number of label-free techniques for directly monitoring biomolecular binding have been developed, but it is still challenging to measure the binding kinetics of very small molecules, to detect low concentrations of analyte molecules, or to detect low affinity interactions. In this study, we report the development of a highly sensitive photonic crystal biosensor for label-free, real-time biomolecular binding analysis. We characterize the performance of this biosensor using a standard streptavidin-biotin binding system. Optimization of the surface functionalization methods for streptavidin immobilization on the silica sensing surface is presented, and the specific binding of biotinylated analyte molecules ranging over 3 orders of magnitude in molecular weight, including very small molecules (<250 Da), DNA oligonucleotides, proteins, and antibodies (>150 000 Da), are detected in real time with a high signal-to-noise ratio. Finally, we document the sensor efficiency for low mass adsorption, as well as multilayered molecular interactions. By all important metrics for sensitivity, we anticipate this photonic crystal biosensor will provide new capabilities for highly sensitive measurements of biomolecular binding.

Power scalable compact THz system based on an ultrafast Yb-doped fiber amplifier

A power-scalable approach for THz generation is demonstrated using optical rectification in GaP pumped by a high power ultrafast Yb-doped fiber amplifier operating at 1.055 mum. A 120-MHz-repetition-rate pulse train of single-cycle THz radiation with 6.5 muW average power is generated using 10 W from a parabolic fiber amplifier. Analysis of the THz power scalability indicates that due to the unique advantages offered by ultrafast optical rectification in GaP and due to the power scalability of fiber lasers, this approach has the potential to generate single-cycle THz pulse trains with average powers up to several mW.

Kilohertz synchronous amplification of 85-femtosecond optical pulses

High-repetition-rate laser pulse amplifiers are desirable for investigations of weak signals because of the ability to use ultrasensitive lock-in detection. We have developed a new oscillator and amplifier capable of providing 10 MW of power at repetition rates in excess of 1 kHz. By focusing this pulse we have obtained the white-light continuum with as little as 250 nJ of energy.