Thomas Roger

Coherent perfect absorption in deeply subwavelength films in the single-photon regime

The technologies of heating, photovoltaics, water photocatalysis and artificial photosynthesis depend on the absorption of light and novel approaches such as coherent absorption from a standing wave promise total dissipation of energy. Extending the control of absorption down to very low light levels and eventually to the single-photon regime is of great interest and yet remains largely unexplored. Here we demonstrate the coherent absorption of single photons in a deeply subwavelength 50% absorber. We show that while the absorption of photons from a travelling wave is probabilistic, standing wave absorption can be observed deterministically, with nearly unitary probability of coupling a photon into a mode of the material, for example, a localized plasmon when this is a metamaterial excited at the plasmon resonance. These results bring a better understanding of the coherent absorption process, which is of central importance for light harvesting, detection, sensing and photonic data processing applications.

Coherent control of light interaction with graphene.

We report the experimental observation of all-optical modulation of light in a graphene film. The graphene film is scanned across a standing wave formed by two counter-propagating laser beams in a Sagnac interferometer. Through a coherent absorption process the on-axis transmission is modulated with close to 80% efficiency. Furthermore, we observe modulation of the scattered energy by mapping the off-axis scattered optical signal: scattering is minimized at a node of the standing wave pattern and maximized at an antinode. The results highlight the possibility to switch and modulate any given optical interaction with deeply sub-wavelength films.

Experimental characterization of nonlocal photon fluids

Quantum gases of atoms and exciton-polaritons are now well-established theoretical and experimental tools for fundamental studies of quantum many-body physics and suggest promising applications to quantum computing. Given their technological complexity, it is of paramount interest to devise other systems where such quantum many-body physics can be investigated at lesser technological expense. Here we examine a relatively well-known system of laser light propagating through thermo-optical defocusing media: based on a hydrodynamic description of light as a quantum fluid of interacting photons, we investigate such systems as a valid room-temperature alternative to atomic or exciton–polariton condensates for studies of many-body physics. First, we show that by using a technique traditionally used in oceanography it is possible to perform a direct measurement of the single-particle part of the dispersion relation of the elementary excitations on top of the photon fluid and to detect its global flow. Then, using a pump-and-probe setup, we investigate the dispersion of excitation modes of the fluid: for very long wavelengths, a sonic, dispersionless propagation is observed that we interpret as a signature of superfluid behavior.

Non-collinear interaction of photons with orbital angular momentum

We study the nonlinear interaction between two non-collinear light beams that carry orbital angular momentum (OAM). More specifically, two incident beams interact at an angle in a medium with a second order nonlinearity and thus generate a third, non-collinear beam at the second harmonic frequency that experiences a reduced conversion efficiency in comparison to that expected based on conventional phase-matching theory. This reduction scales with the input beam OAM and, differently from previous spiral bandwidth calculations, is due to a geometric effect whereby the input OAM is projected along the non-collinear interaction direction. The effect is relevant even at small interaction angles and is further complicated at large angles by a non-conservation of the total OAM in the nonlinear interaction. Experiments are performed under different conditions and are in excellent agreement with the theory. Our results have implications beyond the specific case studied here of second-harmonic generation, in particular for parametric down-conversion of photons or in general for phase-matched non-collinear interactions between beams with different OAM.

Coherent absorption of N00N states

We experimentally investigate two-photon N00N state coherent absorption in a multilayer graphene film and show that coherent loss can be used as a resource for quantum operations.

From coherent shocklets to giant collective incoherent shock waves in nonlocal turbulent flows

Understanding turbulent flows arising from random dispersive waves that interact strongly through nonlinearities is a challenging issue in physics. Here we report the observation of a characteristic transition: strengthening the nonlocal character of the nonlinear response drives the system from a fully turbulent regime, featuring a sea of coherent small-scale dispersive shock waves (shocklets) towards the unexpected emergence of a giant collective incoherent shock wave. The front of such global incoherent shock carries most of the stochastic fluctuations and is responsible for a peculiar folding of the local spectrum. Nonlinear optics experiments performed in a solution of graphene nano-flakes clearly highlight this remarkable transition. Our observations shed new light on the role of long-range interactions in strongly nonlinear wave systems operating far from thermodynamic equilibrium, which reveals analogies with, for example, gravitational systems, and establishes a new scenario that can be common to many turbulent flows in photonic quantum fluids, hydrodynamics and Bose–Einstein condensates.

Geometries for the coherent control of four-wave mixing in graphene multilayers

Deeply sub-wavelength two-dimensional films may exhibit extraordinarily strong nonlinear effects. Here we show that 2D films exhibit the remarkable property of a phase-controllable nonlinearity, i.e., the amplitude of the nonlinear polarisation wave in the medium can be controlled via the pump beam phase and determines whether a probe beam will “feel” or not the nonlinearity. This is in stark contrast to bulk nonlinearities where propagation in the medium averages out any such phase dependence. We perform a series of experiments in multilayer graphene that highlight some of the consequences of the optical nonlinearity phase-dependence, such as the coherent control of nonlinearly diffracted beams, single-pump-beam induced phase-conjugation and the demonstration of a nonlinear mirror characterised by negative reflection. The observed phase sensitivity is not specific to graphene but rather is solely a result of the dimensionality and is therefore expected in all 2D materials.

Optically induced metal-to-dielectric transition in Epsilon-Near-Zero metamaterials.

Epsilon-Near-Zero materials exhibit a transition in the real part of the dielectric permittivity from positive to negative value as a function of wavelength. Here we study metal-dielectric layered metamaterials in the homogenised regime (each layer has strongly subwavelength thickness) with zero real part of the permittivity in the near-infrared region. By optically pumping the metamaterial we experimentally show that close to the Epsilon-Near-Zero (ENZ) wavelength the permittivity exhibits a marked transition from metallic (negative permittivity) to dielectric (positive permittivity) as a function of the optical power. Remarkably, this transition is linear as a function of pump power and occurs on time scales of the order of the 100 fs pump pulse that need not be tuned to a specific wavelength. The linearity of the permittivity increase allows us to express the response of the metamaterial in terms of a standard third order optical nonlinearity: this shows a clear inversion of the roles of the real and imaginary parts in crossing the ENZ wavelength, further supporting an optically induced change in the physical behaviour of the metamaterial.

Optical analogues of the Newton–Schrödinger equation and boson star evolution

Many gravitational phenomena that lie at the core of our understanding of the Universe have not yet been directly observed. An example in this sense is the boson star that has been proposed as an alternative to some compact objects currently interpreted as being black holes. In the weak field limit, these stars are governed by the Newton–Schrodinger equation. Here we present an optical system that, under appropriate conditions, identically reproduces such equation in two dimensions. A rotating boson star is experimentally and numerically modelled by an optical beam propagating through a medium with a positive thermal nonlinearity and is shown to oscillate in time while also stable up to relatively high densities. For higher densities, instabilities lead to an apparent breakup of the star, yet coherence across the whole structure is maintained. These results show that optical analogues can be used to shed new light on inaccessible gravitational objects.

Optical time reversal from time-dependent Epsilon-Near-Zero media

We provide an efficient surface time-reversal of the incident electric field in an ENZ material producing both phase-conjugated and negative refracted beams. The results obtained exploiting degenerate four-wave mixing show an efficiency conversion over 200%.