Tianqing Jia

FANO RESONANCES IN DISK–RING PLASMONIC NANOSTRUCTURE: STRONG INTERACTION BETWEEN BRIGHT DIPOLAR AND DARK MULTIPOLAR MODE

This Letter presents a plasmonic nanostructure consisting of a nanodisk and a nanoring. The nanodisk is outside of the nanoring. The quadrupolar, hexapolar, and octupolar resonance modes of the nanoring are excited easily by the bright dipolar mode of nanodisks. This nanostructure shows strong interaction and deep Fano dips. In addition, the resonance frequency, depth, and line width of Fano dips can be tuned by changing the geometrical parameters of the nanodisk and nanoring. These plasmonic nanostructures show both high contrast ratio and high figure of merit. Such characters make them suitable for chemical and biological sensing.

Alignment of nanoparticles formed on the surface of 6H-SiC crystals irradiated by two collinear femtosecond laser beams

Nanoripples with periods of 150 and 80 nm are formed on the surface of 6H-SiC crystals irradiated by the p-polarized 800 nm and the s-polarized 400 nm femtosecond lasers, respectively. When both of the two collinear laser beams focus simultaneously on the sample surface, nanoparticles are formed on the whole ablation area, and they array in parallel lines. We propose and confirm that the second harmonics in the sample surface excited by the incident lasers plays an important role in the formation of nanostructures.

Formation of long- and short-periodic nanoripples on stainless steel irradiated by femtosecond laser pulses

In this paper, we report the formation of long-periodic (LP) ripples with a period of 530–600 nm and short-periodic (SP) ripples with a period of 260–320 nm on stainless steel irradiated by 800 nm femtosecond laser pulses. The split of LP ripples plays the decisive role in the formation of SP ripples. We further conduct pump-probe experiments and numerical simulations to study the ultrafast dynamics of the formation of surface periodic ripples.

Periodic nanoripples in the surface and subsurface layers in ZnO irradiated by femtosecond laser pulses

We present the formation of periodic ripples in ZnO crystal irradiated by a wavelength-tunable femtosecond laser. The results indicate that in the surface thin layer, the periods change from 0.1 lambda to lambda with laser fluences and pulse numbers, and in the subsurface layer the periods are always lambda/2n, where n is the refractive index. The formation processes and mechanisms are also discussed.

Fabrication of two-dimensional periodic nanostructures by two-beam interference of femtosecond pulses.

Two-dimensional periodic nanostructures on ZnO crystal surface were fabricated by two-beam interference of 790 nm femtosecond laser. The long period is, as usually reported, determined by the interference pattern of two laser beams. Surprisingly, there is another short periodic nanostructures with periods of 220-270 nm embedding in the long periodic structures. We studied the periods, orientation, and the evolution of the short periodic nanostructures, and found them analogous to the self-organized nanostructures induced by single fs laser beam.

Complex periodic micro/nanostructures on 6H-SiC crystal induced by the interference of three femtosecond laser beams

We reported three types of complex micro/nanostructures on 6H-SiC crystal induced by the interferences of three femtosecond laser beams by arranging three types of laser polarization combinations. The micro/nanostructures are composed of two parts: two-dimensional long-periodic micropatterns determined by the interferential intensity pattern and short-periodic nanopatterns determined by the interferential polarization pattern. Theoretical calculation indicates that the different polarization combinations will lead to a distinct complex interferential polarization pattern and intensity pattern, and they accord well with the experimental results.

Fine tunable red-green upconversion luminescence from glass ceramic containing 5%Er3+:NaYF4 nanocrystals under excitation of two near infrared femtosecond lasers

In this paper, we report fine tunable red-green upconversion luminescence of glass ceramic containing 5%Er3+: NaYF4 nanocrystals excited simultaneously by two near infrared femtosecond lasers. When the glass ceramic was irradiated by 800 nm femtosecond laser, weak red emission centered at 670 nm was detected. Bright red light was observed when the fs laser wavelength was tuned to 1490 nm. However, when excited by the two fs lasers simultaneously, the sample emitted bright green light centered at 550 nm, while the red light kept the same intensity. The dependences of the red and the green light intensities on the two pump lasers are much different, which enables us to manipulate the color emission by adjusting the two pump laser intensities, respectively. We present a theoretical model of Er3+ ions interacting with two fs laser fields, and explain well the experimental results.

A uniform 290 nm periodic square structure on ZnO fabricated by two-beam femtosecond laser ablation

A uniform submicron periodic square structure was fabricated on the surface of ZnO by a technique of two linearly polarized femtosecond laser beams with orthogonal polarizations ablating material alternately. The formed two-dimensional ordering submicron structure consists of close-packed submicron squares with a spacial periodicity of 290 nm, which arises from the intercrossing of two orthogonal submicron ripple structures induced by the two beams respectively. The result demonstrates a noninterference effect of two-beam ablation based on the alternate technique, which should come from the polarization-dependent enhancement of the subwavelength ripple structure and the large interval of two alternate pulses. This two-beam alternate ablation technique is expected to open up prospects for the submicron fabrication of wide-bandgap materials.

Dipole, quadrupole and octupole plasmon resonance modes in non-concentric nanocrescent/nanodisk structure: local field enhancement in the visible and near infrared regions

By deviating the nanodisk from the center in the silver nanocrescent/nanodisk structure, we find that the dipole, quadrupole and octupole modes can all induce very high local electric field enhancement (LFE, more than 750) for the coupling of nanocrescent and crescent gap modes, which makes the resonant wavelengths of the non-concentric nanostructures change from the visible to near infrared regions. In addition, the LFE factor of the quadrupole mode is more than 1000, which is suitable for single molecular detection by local surface enhanced spectroscopy.

Quadrupole plasmon resonance mode in nanocrescent/nanodisk structure:Local field enhancement and tunability in the visible light region

We propose a metallic nanostructure consisting of a nanodisk in a nanocrescent. At the quadrupole plasmon resonance wavelengths of the nanocrescent/nanodisk structures, the local electric field amplitudes at the crescent tips are 15 times higher than those of the single nanocrescents. In addition, the quadrupole resonance wavelengths are tunable in the visible region while the peak widths keep less than 5 nm. We study the mechanisms of the local field enhancement (LFE), and find that the coupling between the quadrupole resonance modes of the nanogap and the nanocrescent result into the high LFE factor.