Tijiang Liu

Superconductivity close to magnetic instability in Fe(Se 1-xTex)0.82

We report our study of the evolution of superconductivity and the phase diagram of the ternary Fe(Se1-xTex)0.82 (0≤x≤1.0) system. We discovered a superconducting phase with T c,max=14 K in the 0.3<x<1.0 range. This superconducting phase is suppressed when the sample composition approaches the end member FeTe 0.82, which exhibits an incommensurate antiferromagnetic order. We discuss the relationship between the superconductivity and magnetism of this material system in terms of recent results from neutron-scattering measurements. Our results and analyses suggest that superconductivity in this class of Fe-based compounds is associated with magnetic fluctuations and therefore may be unconventional in nature.

Charge-carrier localization induced by excess Fe in the superconductor Fe1+yTe1−xSex

We have investigated the effect of Fe nonstoichiometry on properties of the Fe1+y(Te, Se) superconductor system by means of resistivity, Hall coefficient, magnetic susceptibility, and specific heat measurements. We find that the excess Fe at interstitial sites of the (Te, Se) layers not only suppresses superconductivity, but also results in a weakly localized electronic state. We argue that these effects originate from the magnetic coupling between the excess Fe and the adjacent Fe square planar sheets, which favors a short-range magnetic order.

From (π,0) magnetic order to superconductivity with (π,π) magnetic resonance in Fe1.02Te1−xSex

The iron chalcogenide Fe(1+y)(Te(1-x)Se(x)) is structurally the simplest of the Fe-based superconductors. Although the Fermi surface is similar to iron pnictides, the parent compound Fe(1+y)Te exhibits antiferromagnetic order with an in-plane magnetic wave vector (pi,0) (ref. 6). This contrasts the pnictide parent compounds where the magnetic order has an in-plane magnetic wave vector (pi,pi) that connects hole and electron parts of the Fermi surface. Despite these differences, both the pnictide and chalcogenide Fe superconductors exhibit a superconducting spin resonance around (pi,pi) (refs 9, 10, 11). A central question in this burgeoning field is therefore how (pi,pi) superconductivity can emerge from a (pi,0) magnetic instability. Here, we report that the magnetic soft mode evolving from the (pi,0)-type magnetic long-range order is associated with weak charge carrier localization. Bulk superconductivity occurs as magnetic correlations at (pi,0) are suppressed and the mode at (pi, pi) becomes dominant for x>0.29. Our results suggest a common magnetic origin for superconductivity in iron chalcogenide and pnictide superconductors.

Calorimetric evidence of strong-coupling multiband superconductivity in Fe(Te0.57Se0.43) single crystal

We have investigated the specific heat of optimally-doped iron chalcogenide superconductor Fe(Te0.57Se0.43) with a high-quality single crystal sample. The electronic specific heat Ce of this sample has been successfully separated from the phonon contribution using the specific heat of a non-superconducting sample (Fe0.90Cu0.10)(Te0.57Se0.43) as a reference. The normal state Sommerfeld coefficient gamma_n of the superconducting sample is found to be ~ 26.6 mJ/mol K^2, indicating intermediate electronic correlation. The temperature dependence of Ce in the superconducting state can be best fitted using a double-gap model with 2Delta_s(0)/kBTc = 3.92 and 2Delta_l(0)/kBTc = 5.84. The large gap magnitudes derived from fitting, as well as the large specific heat jump of Delta_Ce(Tc)/gamma_n*Tc ~ 2.11, indicate strong-coupling superconductivity. Furthermore, the magnetic field dependence of specific heat shows strong evidence for multiband superconductivity.

Friedel-Like Oscillations from Interstitial Iron in Superconducting Fe1+yTe0.62Se0.38

Using polarized and unpolarized neutron scattering, we show that interstitial Fe in superconducting Fe(1+y)Te(1-x)Se(x) induces a magnetic Friedel-like oscillation that diffracts at Q⊥=(1/2 0) and involves >50 neighboring Fe sites. The interstitial >2μ(B) moment is surrounded by compensating ferromagnetic four-spin clusters that may seed double stripe ordering in Fe(1+y)Te. A semimetallic five-band model with (1/2 1/2) Fermi surface nesting and fourfold symmetric superexchange between interstitial Fe and two in-plane nearest neighbors largely accounts for the observed diffraction.

Enhanced spin-triplet superconductivity near dislocations in Sr 2 RuO 4

Superconductors with a chiral p-wave pairing are of great interest because they could support Majorana modes that could enable the development of topological quantum computing technologies that are robust against decoherence. Sr₂RuO₄ is widely believed to be a chiral p-wave superconductor. Yet, the mechanism by which superconductivity emerges in this, and indeed most other unconventional superconductors, remains unclear. Here we show that the local superconducting transition temperature in the vicinity of lattice dislocations in Sr₂RuO₄ can be up to twice that of its bulk. This is all the more surprising for the fact that disorder is known to easily quench superconductivity in this material. With the help of a phenomenological theory that takes into account the crystalline symmetry near a dislocation and the pairing symmetry of Sr₂RuO₄, we predict that a similar enhancement should emerge as a consequence of symmetry reduction in any superconductor with a two-component order parameter.Sr2RuO4 Y. A. Ying, N. E. Staley, Y. Xin, K. Sun, X. Cai, D. Fobes, T. Liu, Z. Q. Mao, and Y. Liu ∗ Department of Physics and Materials Research Institute, The Pennsylvania State University, University Park, Pennsylvania 16802, USA National High Magnetic Field Laboratory, Florida State University, Tallahassee, Florida 32306, USA Condensed Matter Theory Center and Joint Quantum Institute, Department of Physics, University of Maryland, College Park, Maryland 20742, USA Department of Physics, Tulane University, New Orleans, Louisiana 70118, USA (Dated: May 1, 2014)

Unusual heavy-mass nearly ferromagnetic state with a surprisingly large Wilson ratio in the double layered ruthenates (Sr1−xCax)3Ru2O7

We report an unusual nearly ferromagnetic heavy-mass state with a surprisingly large Wilson ratio Rw e.g., Rw 700 for x = 0.2 in double layered ruthenates Sr1�xCax3Ru2O7 with 0.08x 0.4. This state does not evolve into a long-range ferromagnetically ordered state despite considerably strong ferromagnetic correlations, but it freezes into a cluster-spin glass at low temperatures. In addition, evidence of non-Fermi-liquid behavior is observed as the spin-freezing temperature of the cluster-spin glass approaches zero near x 0.1. We discuss the origin of this unique magnetic state from the Fermi-surface information probed by Hall-effect measurements.

Coupling of electronic and magnetic properties in Fe1+y(Te1−xSex)

We have studied the coupling of electronic and magnetic properties in Fe1+y(Te1-xSex) via systematic specific heat, magnetoresistivity, and Hall coefficient measurements on two groups of samples with y = 0.02 and 0.1. In the y = 0.02 series, we find that the 0.09 < x < 0.3 composition region, where superconductivity is suppressed, has large Sommerfeld coefficient Gamma (~55-65 mJ/mol K^2), positive Hall coefficient R_H and negative magnetoresistance MR at low temperature, in sharp contrast with the x=0.4-0.5 region where Gamma drops to ~ 26 mJ/mol K^2 and R_H / MR becomes negative/positive at low temperature. Dramatic changes of Gamma, as well as sign reversal in low-temperature RH and MR, are also observed across the x~0.1 boundary where the long-range antiferromagnetic order is suppressed. However, for the system with rich interstitial excess Fe (y = 0.1), where bulk superconductivity is suppressed even for x=0.4-0.5, the variations of Gamma, R_H and MR with x are distinct from those seen in y = 0.02 system: Gamma is ~40 mJ/mol K^2 for 0.1 < x < 0.3, and drops to ~ 34 mJ/mol K^2 for x = 0.4-0.5; R_H and MR does not show any sign reversal as x is increased above 0.3. We will show that all these results can be understood in light of the evolution of the incoherent magnetic scattering by (pi,0) magnetic fluctuations with Se concentration. In addition, with the suppression of magnetic scattering by magnetic field, we observed the surprising effect of a remarkable increase in the superconducting volume fraction under moderate magnetic fields for x=0.3-0.4 samples in the y = 0.02 system.

Complex electronic states in double-layered ruthenates (Sr1−xCax)3Ru2O7

The magnetic ground state of (Sr

Possible nodal superconducting gap in Fe1+y(Te1−xSex) single crystals from ultralow temperature penetration depth measurements

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