Tim Hellwig

On-chip visible-to-infrared supercontinuum generation with more than 495 THz spectral bandwidth

We report ultra-broadband supercontinuum generation in high-confinement Si3N4 integrated optical waveguides. The spectrum extends through the visible (from 470 nm) to the infrared spectral range (2130 nm) comprising a spectral bandwidth wider than 495 THz, which is the widest supercontinuum spectrum generated on a chip.

Optical repetition rate stabilization of a mode-locked all-fiber laser

We designed an all-fiber mode-locked Erbium laser with optically stabilized repetition rate of 31.4 MHz. The stabilization was achieved by changing the refractive index of an Ytterbium-doped fiber in the resonator via optical pumping at a wavelength of 978 nm; and for long-term stability the local temperature of the fiber was additionally controlled with a thermo-electric element. The repetition rate was stabilized over 12 hours, and an Allan deviation of 2.5 × 10⁻¹² for an averaging time of 1 s could be achieved.

Two-octave spanning supercontinuum generation in stoichiometric silicon nitride waveguides pumped at telecom wavelengths

We demonstrate supercontinuum generation in stoichiometric silicon nitride (Si3N4 in SiO2) integrated optical waveguides, pumped at telecommunication wavelengths. The pump laser is a mode-locked erbium fiber laser at a wavelength of 1.56 µm with a pulse duration of 120 fs. With a waveguide-internal pulse energy of 1.4 nJ and a waveguide with 1.0 µm × 0.9 µm cross section, designed for anomalous dispersion across the 1500 nm telecommunication range, the output spectrum extends from the visible, at around 526 nm, up to the mid-infrared, at least to 2.6 µm, the instrumental limit of our detection. This output spans more than 2.2 octaves (454 THz at the -30 dB level). The measured output spectra agree well with theoretical modeling based on the generalized nonlinear Schrödinger equation. The infrared part of the supercontinuum spectra shifts progressively towards the mid-infrared, well beyond 2.6 µm, by increasing the width of the waveguides.

Near-infrared photoswitching of cyclodextrin–guest complexes using lanthanide-doped LiYF4 upconversion nanoparticles

This communication reports a new type of supramolecular cyclodextrin-guest complexes using cyclodextrin coated upconversion nanoparticles as hosts and monovalent and divalent azobenzenes and arylazopyrazoles as guests. A potentially biocompatible photocontrol of the interaction by isomerization of the azobenzene or arylazopyrazole was achieved by laser irradiation at 980 nm and a very low light intensity of 0.22 W cm-2.

Stabilization of High Oxidation State Upconversion Nanoparticles by N-Heterocyclic Carbenes

The stabilization of high oxidation state nanoparticles by N-heterocyclic carbenes is reported. Such nanoparticles represent an important subset in the field of nanoparticles, with different and more challenging requirements for suitable ligands compared to elemental metal nanoparticles. N-Heterocyclic carbene coated NaYF4 :Yb,Tm upconversion nanoparticles were synthesized by a ligand-exchange reaction from a well-defined precursor. This new photoactive material was characterized in detail and employed in the activation of photoresponsive molecules by low-intensity near-infrared light (λ=980 nm).

Experimental realization of femtosecond transverse mode conversion using optically induced transient long-period gratings

We present the experimental realization of transverse mode conversion in an optical fiber via an optically induced long-period grating. The transient gratings are generated by femtosecond laser pulses, exploiting the Kerr effect to translate intensity patterns emerging from multimode interference into a spatial refractive index modulation. Since these modulations exist only while the pump beam is present, they can be used for optical switching of transverse modes. As only a localized part of the grating was written at a time and the probe beam was co-propagating with the pump beam the required pulse energies could be reduced to 120 nJ which is about a factor of 600 lower than in previous quasi-continuous-wave experiments. Accompanying numerical simulations allow a better understanding of the involved effects and show excellent agreement to the experimental results.

Ultrafast, low-power, all-optical switching via birefringent phase-matched transverse mode conversion in integrated waveguides

We demonstrate the potential of birefringence-based, all-optical, ultrafast conversion between the transverse modes in integrated optical waveguides by modelling the conversion process by numerically solving the multi-mode coupled nonlinear Schroedinger equations. The observed conversion is induced by a control beam and due to the Kerr effect, resulting in a transient index grating which coherently scatters probe light from one transverse waveguide mode into another. We introduce birefringent phase matching to enable efficient all-optically induced mode conversion at different wavelengths of the control and probe beam. It is shown that tailoring the waveguide geometry can be exploited to explicitly minimize intermodal group delay as well as to maximize the nonlinear coefficient, under the constraint of a phase matching condition. The waveguide geometries investigated here, allow for mode conversion with over two orders of magnitude reduced control pulse energy compared to previous schemes and thereby promise nonlinear mode switching exceeding efficiencies of 90% at switching energies below 1 nJ.

Ultrafast, all-optical control of modal phases in a few-mode fiber for all-optical switching

The phase differences between the transverse modes of an optical fiber can be altered all-optically by intermodal cross-phase modulation. In this Letter, we experimentally demonstrate this effect with ultrashort laser pulses. An ultrashort probe pulse, guided in both modes of a two-mode fiber, is co-propagating and temporally overlapping with an ultrashort control pulse, guided in the fundamental mode only and centered at a separate wavelength. The use of ultrashort pulses allows for a notable phase shift at a 33-fold reduced control pulse energy and a 173-fold reduced fiber length, compared to previous experiments. A total phase shift of 0.285π between the two probe modes was achieved at a 9 nJ control pulse energy in a 19 cm long two-mode graded-index fiber. Additionally, the capability of this scheme to switch ultrashort pulses in an all-optical manner was investigated. A modulation depth of 50% was achieved, limited by temporal nonlinear effects.

Toward an all-optically stabilized frequency comb based on a mode-locked fiber laser

We present an erbium-doped mode-locked fiber laser comprising two all-optical control mechanisms acting on the carrier envelope offset (CEO)-frequency as well as the repetition frequency. The lasers repetition frequency is stabilized via optically pumping a distinct ytterbium-doped fiber module. By proving that additionally controlling the pump power of the erbium-doped gain fiber acts sufficiently complementary on the lasers CEO-frequency compared with repetition frequency stabilization, we demonstrate the feasibility of this concept for an all-optically controlled frequency comb in an all-fiber setup.

Spectrally resolving single-shot polarimeter.

We demonstrate a spectrally resolving single-shot polarimeter. The system consists of a commercial imaging spectrograph, modified by a birefringent wedge and a segmented polarizer. The physical operating principle and limitations of the apparatus as well as preliminary polarimetric measurements on the emission of random lasers are reported.