Timo Gissibl

Linear refractive index and absorption measurements of nonlinear optical liquids in the visible and near-infrared spectral region

Liquid-filled photonic crystal fibers and optofluidic devices require infiltration with a variety of liquids whose linear optical properties are still not well known over a broad spectral range, particularly in the near infrared. Hence, dispersion and absorption properties in the visible and near-infrared wavelength region have been determined for distilled water, heavy water, chloroform, carbon tetrachloride, toluene, ethanol, carbon disulfide, and nitrobenzene at a temperature of 20 °C. For the refractive index measurement a standard Abbe refractometer in combination with a white light laser and a technique to calculate correction terms to compensate for the dispersion of the glass prism has been used. New refractive index data and derived dispersion formulas between a wavelength of 500 nm and 1600 nm are presented in good agreement with sparsely existing reference data in this wavelength range. The absorption coefficient has been deduced from the difference of the losses of several identically prepared liquid filled glass cells or tubes of different lengths. We present absorption data in the wavelength region between 500 nm and 1750 nm.

Ultrafast nonlinear optofluidics in selectively liquid-filled photonic crystal fibers

Selective filling of photonic crystal fibers with different media enables a plethora of possibilities in linear and nonlinear optics. Using two-photon direct-laser writing we demonstrate full flexibility of individual closing of holes and subsequent filling of photonic crystal fibers with highly nonlinear liquids. We experimentally demonstrate solitonic supercontinuum generation over 600 nm bandwidth using a compact femtosecond oscillator as pump source. Encapsulating our fibers at the ends we realize a compact ultrafast nonlinear optofluidic device. Our work is fundamentally important to the field of nonlinear optics as it provides a new platform for investigations of spatio-temporal nonlinear effects and underpins new applications in sensing and communications. Selective filling of different linear and nonlinear liquids, metals, gases, gain media, and liquid crystals into photonic crystal fibers will be the basis of new reconfigurable and versatile optical fiber devices with unprecedented performance. Control over both temporal and spatial dispersion as well as linear and nonlinear coupling will lead to the generation of spatial-temporal solitons, so-called optical bullets.

Sub-micrometre accurate free-form optics by three-dimensional printing on single-mode fibres

Micro-optics are widely used in numerous applications, such as beam shaping, collimation, focusing and imaging. We use femtosecond 3D printing to manufacture free-form micro-optical elements. Our method gives sub-micrometre accuracy so that direct manufacturing even on single-mode fibres is possible. We demonstrate the potential of our method by writing different collimation optics, toric lenses, free-form surfaces with polynomials of up to 10th order for intensity beam shaping, as well as chiral photonic crystals for circular polarization filtering, all aligned onto the core of the single-mode fibres. We determine the accuracy of our optics by analysing the output patterns as well as interferometrically characterizing the surfaces. We find excellent agreement with numerical calculations. 3D printing of microoptics can achieve sufficient performance that will allow for rapid prototyping and production of beam-shaping and imaging devices.

3D-printed eagle eye: Compound microlens system for foveated imaging

A highly miniaturized vision system is realized by directly 3D-printing different multilens objectives onto a CMOS image sensor. We present a highly miniaturized camera, mimicking the natural vision of predators, by 3D-printing different multilens objectives directly onto a complementary metal-oxide semiconductor (CMOS) image sensor. Our system combines four printed doublet lenses with different focal lengths (equivalent to f = 31 to 123 mm for a 35-mm film) in a 2 × 2 arrangement to achieve a full field of view of 70° with an increasing angular resolution of up to 2 cycles/deg field of view in the center of the image. The footprint of the optics on the chip is below 300 μm × 300 μm, whereas their height is <200 μm. Because the four lenses are printed in one single step without the necessity for any further assembling or alignment, this approach allows for fast design iterations and can lead to a plethora of different miniaturized multiaperture imaging systems with applications in fields such as endoscopy, optical metrology, optical sensing, surveillance drones, or security.

Spatial beam intensity shaping using phase masks on single-mode optical fibers fabricated by femtosecond direct laser writing

Submicrometer dielectric phase masks allow for the realization of the miniaturization of high-quality optical elements. In this Letter we demonstrate spatial intensity beam shaping using phase masks attached to optical single-mode fibers. The phase masks are directly fabricated onto the end facet of optical fibers using femtosecond two-photon direct laser writing, achieving, therefore, submicrometer alignment accuracy. We observe high-quality intensity patterns and find excellent agreement with simulations. Our results prove that 3D printing of diffractive micro-optics can achieve sufficient performance to enable compact devices.

Large-area fabrication of TiN nanoantenna arrays for refractory plasmonics in the mid-infrared by femtosecond direct laser writing and interference lithography [Invited]

Robust plasmonic nanoantennas at mid-infrared wavelengths are essential components for a variety of nanophotonic applications ranging from thermography to energy conversion. Titanium nitride (TiN) is a promising candidate for such cases due to its high thermal stability and metallic character. Here, we employ direct laser writing as well as interference lithography to fabricate large-area nanoantenna arrays of TiN on sapphire and silicon substrates. Our lithographic tools allow for fast and homogeneous preparation of nanoantenna geometries on a polymer layer, which is then selectively transferred to TiN by subsequent argon ion beam etching followed by a chemical wet etching process. The antennas are protected by an additional Al2O3 layer which allows for high-temperature annealing in argon flow without loss of the plasmonic properties. Tailoring of the TiN antenna geometry enables precise tuning of the plasmon resonances from the near to the mid-infrared spectral range. Due to the advantageous properties of TiN combined with our versatile large-area and low-cost fabrication process, such refractory nanoantennas will enable a multitude of high-temperature plasmonic applications such as thermophotovoltaics in the future.

Towards integration of a liquid-filled fiber capillary for supercontinuum generation in the 1.2–2.4 μm range

We demonstrate supercontinuum generation in unspliced as well as in integrated CS(2)-filled capillary fibers at different pump wavelengths of 1030 nm, 1510 nm, and 1685 nm. A novel method for splicing a liquid-filled capillary fiber to a standard single-mode optical fiber is presented. This method is based on mechanical splicing using a direct-laser written polymer ferrule using a femtosecond two-photon polymerization process. We maintain mostly single-mode operation despite the multi-mode capability of the liquid-filled capillaries. The generated supercontinua exhibit a spectral width of over 1200 nm and 1000 nm for core diameters of 5 μm and 10 μm, respectively. This is an increase of more than 50 percent compared to previously reported values in the literature due to improved dispersion properties of the capillaries.

Ultra-compact on-chip LED collimation optics by 3D femtosecond direct laser writing.

By using two-photon lithographic 3D printing, we demonstrate additive manufacturing of a dielectric concentrator directly on a LED chip. With a size of below 200 μm in diameter and length, light output is increased by a factor of 6.2 in collimation direction, while the emission half-angle is reduced by 50%. We measure excellent form fidelity and irradiance patterns close to simulation. Additionally, a more complex shape design is presented, which exhibits a nonconventional triangular illumination pattern. The introduced method features exceptional design freedoms which can be used to tailor high-quality miniature illumination optics for specific lighting tasks, for example, endoscopy.

Spatial solitons in optofluidic waveguide arrays with focusing ultrafast Kerr nonlinearity

We present an optofluidic nonlinear waveguide array that is fabricated by selectively filling several strands of a photonic crystal fiber with the liquid CCl(4), which exhibits a large focusing ultrafast Kerr nonlinearity. We demonstrate a power dependent formation of a spatial soliton in this novel optofluidic device. The large thermo-optical effect of liquids enables us to control the characteristics of the spatial soliton formation in these nonlinear structures. This opens the road toward flexible designs and the realization of a new class of optofluidic devices with complex nonlinear landscapes and novel effects.

Refractive index measurements of photo-resists for three-dimensional direct laser writing

Femtosecond 3D printing is an important technology for manufacturing of nano- and microscopic devices and elements. Crucial for the design of such structures is the detailed knowledge of the refractive index in the visible and near-infrared spectral range and its dispersion. Here, we characterize 5 photoresists that are used with femtosecond 3D direct laser writers, namely IP-S, IP-Dip, IP-L, IP-G, and OrmoComp with a modified and automized Pulfrich refractometer setup, utilizing critical angles of total internal reflection. We achieve an accuracy of 5⋅10−4 and reference our values to a BK-7 glass plate. We also give Abbe numbers and Schott Catalog numbers of the different resists. Their refractive indices are in the 1.49-1.57 range, while their Abbe numbers are in the range between 35 and 51.