U. Greife

The DRAGON facility for nuclear astrophysics at TRIUMF-ISAC: design, construction and operation

A facility for measuring cross-sections (resonance strengths) for reactions of astrophysical importance involving short-lived, radioactive reactants has been designed, built and installed at the new TRIUMF-ISAC Radioactive Beams Laboratory in Canada. Named DRAGON (Detector of Recoils And Gamma-rays of Nuclear reactions), it has been successfully commissioned with stable and radioactive heavy ion beams from ISAC. This report presents the main components of the facility, namely, the windowless gas target, the surrounding g detector array, the subsequent electromagnetic recoil mass separator, the focal plane detectors for recoils, the detection system for elastics, and the modular electronics and computer software used for the data acquisition. Examples of the operation of the facility for both stable beam reactions and the first radioactive beam reaction study, 21 Naðp;gÞ 22 Mg are also presented, along with future plans for the program. r 2003 Elsevier Science B.V. All rights reserved. PACS: 29.0

Background identification and suppression for the measurement of (n,γ) reactions with the DANCE array at LANSCE

Abstract In the commissioning phase of the DANCE project (Detector for Advanced Neutron Capture Experiments) measurements have been performed with special emphasis on the identification and suppression of possible backgrounds for the planned (n,γ) experiments. This report describes several background sources, observed in the experiment or anticipated from simulations, which will need to be suppressed in this and in similar detectors that are planned at other facilities. First successes are documented in the suppression of background from scattered neutrons captured in the detector as well as from the internal radiation. Experimental results and simulations using the GEANT code are compared.

Stopping power, electron screening and the astrophysical S(E) factor of d(He-3,p)He-4

Abstract The d( 3 He,p) 4 He cross section has been measured at E =4.2 to 13.8 keV using the LUNA underground accelerator facility. The experiment was performed to determine the magnitude of the atomic screening effect and to establish values for the energy loss used in data reduction. The observed stopping power of the 3 He ions in the D 2 target is in good agreement with the standard compilation. Using these stopping power values the data lead to an electron-screening potential energy U e = 132±9 eV, which is significantly higher than the estimated value of 65 eV from an atomic-physics model.

Charge state studies of low energy heavy ions passing through hydrogen and helium gas

Studies of the charge state distribution of low energy (<1.5 MeV/u), low Z (<13) heavy ions passing through hydrogen and helium gas of varying target pressure have been performed using separate windowless gas target systems at TRIUMF and the University of Naples. Semi-empirical relationships have been deduced to estimate the equilibrium charge state distributions as a function of beam energy. From these distributions, cross-sections for the relevant charge changing reactions have been deduced.

New constraints on the 18F(p,α) 15O rate in novae from the (d, p) reaction

The degree to which the (p,gamma) and (p,alpha) reactions destroy 18F at temperatures 1-4x10^8 K is important for understanding the synthesis of nuclei in nova explosions and for using the long-lived radionuclide 18F, a target of gamma-ray astronomy, as a diagnostic of nova mechanisms. The reactions are dominated by low-lying proton resonances near the 18F+p threshold (E_x=6.411 MeV in 19Ne). To gain further information about these resonances, we have used a radioactive 18F beam from the Holifield Radioactive Ion Beam Facility to selectively populate corresponding mirror states in 19F via the inverse d(18F,p)19F neutron transfer reaction. Neutron spectroscopic factors were measured for states in 19F in the excitation energy range 0-9 MeV. Widths for corresponding proton resonances in 19Ne were calculated using a Woods-Saxon potential. The results imply significantly lower 18F(p,gamma)19Ne and 18F(p,alpha)15O reaction rates than reported previously, thereby increasing the prospect of observing the 511-keV annihilation radiation associated with the decay of 18F in the ashes ejected from novae.

Off-line production of a 7Be radioactive ion beam

Abstract A 7 Be ion beam of several particle pA at 8 MeV has been produced at the TTT3 tandem of the University “Federico II” in Naples. The 7 Be nuclides were formed via the 7 Li(p,n) 7 Be reaction using a metallic Li target and an 11.4 MeV proton beam of 20 μA intensity, delivered by the cyclotron in Debrecen. Methods of hot chemistry were used to extract the 7 Be nuclides from the Li matrix and to prepare the 7 Be cathodes for the ion sputter source of the tandem. Examples of 7 Be beam applications are given.

Constraining nova observables: direct measurements of resonance strengths in 33S(p,\gamma)34Cl

The 33S(p,\gamma)34Cl reaction is important for constraining predictions of certain isotopic abundances in oxygen-neon novae. Models currently predict as much as 150 times the solar abundance of 33S in oxygen-neon nova ejecta. This overproduction factor may, however, vary by orders of magnitude due to uncertainties in the 33S(p,\gamma)34Cl reaction rate at nova peak temperatures. Depending on this rate, 33S could potentially be used as a diagnostic tool for classifying certain types of presolar grains. Better knowledge of the 33S(p,\gamma)34Cl rate would also aid in interpreting nova observations over the S-Ca mass region and contribute to the firm establishment of the maximum endpoint of nova nucleosynthesis. Additionally, the total S elemental abundance which is affected by this reaction has been proposed as a thermometer to study the peak temperatures of novae. Previously, the 33S(p,\gamma)34Cl reaction rate had only been studied directly down to resonance energies of 432 keV. However, for nova peak temperatures of 0.2-0.4 GK there are 7 known states in 34Cl both below the 432 keV resonance and within the Gamow window that could play a dominant role. Direct measurements of the resonance strengths of these states were performed using the DRAGON recoil separator at TRIUMF. Additionally two new states within this energy region are reported. Several hydrodynamic simulations have been performed, using all available experimental information for the 33S(p,\gamma)34Cl rate, to explore the impact of the remaining uncertainty in this rate on nucleosynthesis in nova explosions. These calculations give a range of ~ 20-150 for the expected 33S overproduction factor, and a range of ~ 100-450 for the 32S/33S ratio expected in ONe novae.

Design of a New Recoil Separator for Measurements of Radiative Capture Reactions in Astrophysics

The rates of proton‐ and alpha‐capture reactions on unstable proton‐rich nuclei are needed to understand the energy generation and element synthesis occurring in novae, X‐ray bursts, and other explosions. Direct measurements of the cross sections of some of these reactions are now possible with radioactive beams and a recoil separator. A new device for such measurements, the Separator for CApture Reactions [SECAR], is being designed for use at the Facility for Rare Isotope Beams (FRIB). The specifications and preliminary conceptual design will be discussed along with plans for the first set of measurements.

Boron-Rich Benzene and Pyrene Derivatives for the Detection of Thermal Neutrons

A synthetic methodology is developed to generate boron rich aromatic small molecules based on benzene and pyrene moieties for the detection of thermal neutrons. The prepared aromatic compounds have a relatively high boron content up to 7.4 wt%, which is important for application in neutron detection as 10B (20% of natural abundance boron) has a large neutron induced reaction cross-section. This is demonstrated by preparing blends of the synthesized molecules with fluorescent dopants in poly(vinyltoluene) matrices resulting in comparable scintillation light output and neutron capture as state-of-the art commercial scintillators, but with the advantage of much lower cost. The boron-rich benzene and pyrene derivatives are prepared by Suzuki conditions using both microwave and traditional heating, affording yields of 40–93%. This new procedure is simple and straightforward, and has the potential to be scaled up.

A gas jet target for radioactive ion beam experiments

New radioactive ion beam (RIB) facilities, like FRIB in the US or FAIR in Europe, will push further away from stability and enable the next generation of nuclear physics experiments. Thus, the need for improved RIB targets is more crucial than ever: developments in exotic beams should coincide with developments in targets for use with those beams, in order for nuclear physics to remain on the cutting edge. Of great importance to the future of RIB physics are scattering, transfer and capture reaction measurements of rare, exotic, and unstable nuclei on light targets such as hydrogen and helium. These measurements require targets that are dense, highly localized, and pure, and conventional targets often suffer too many drawbacks to allow for such experimental designs. Targets must also accommodate the use of large area, highly-segmented silicon detector arrays, high-efficiency gamma arrays, and novel heavy ion detectors to efficiently measure the reaction products. To address this issue, the Jet Experiments...