Victoria E. Cachorro

A long Saharan dust event over the western Mediterranean: Lidar, Sun photometer observations, and regional dust modeling

A long Saharan dust event affected the western Mediterranean in the period 12– 28 June 2002. Dust was present mainly between 1- and 5-km height affecting most parts of the Iberian Peninsula and reaching western/central Europe. Intensive backscatter lidar observations over Barcelona (Spain) and Sun photometer data from two stations (El Arenosillo, Spain, and Avignon, France) are used to evaluate different configurations the Dust Regional Atmospheric Modeling (DREAM) system. DREAM currently operates dust forecasts over the Mediterranean region (http://www.bsc.es/projects/earthscience/ DREAM/) considering four particle size bins while only the first two are relevant for long-range transport analysis since their life time is larger than 12 hours. A more detailed bin method is implemented, and two different dust distributions at sources are compared to the operational version. Evaluations are performed at two wavelengths (532 and 1064 nm). The dust horizontal and vertical structure simulated by DREAM shows very good qualitative agreement when compared to SeaWIFS satellite images and lidar height-time displays over Barcelona. When evaluating the modeled aerosol optical depth (AOD) against Sun photometer data, significant improvements are achieved with the use of the new detailed bin method. In general, the model underpredicts the AOD for increasing A ° ngstro¨m exponents because of the influence of anthropogenic pollution in the boundary layer. In fact, the modeled AOD is highly anticorrelated with the observed A ° ngstro¨m exponents. Avignon shows higher influence of small anthropogenic aerosols which explains the better results of the model at the wavelength of 1064 nm over this location. The uncertainties of backscatter lidar inversions (20–30%) are in the same order of magnitude as the differences between the model experiments. Better model results are obtained when comparing to lidar because most of the anthropogenic effect is removed.

Aerosols in polar regions: A historical overview based on optical depth and in situ observations

Large sets of filtered actinometer, filtered pyrheliometer and Sun photometer measurements have been carried out over the past 30 years by various groups at different Arctic and Antarctic sites and ...

Determination of the Angstrom turbidity parameters

We have analyzed the dependence of the Angstrom turbidity parameters on wavelength throughout the visible range by three different methods. We have obtained significant results about the ability of these parameters to represent the turbidity of the atmosphere. An important variation of these coefficients with the wavelength is shown, depending on the method used and the spectral resolution of the data. The log-log plot of aerosol optical thickness vs wavelength appears as an adequate method of obtaining the Angstrom parameters to represent the turbidity of the atmosphere and to model the effect of aerosols on solar radiation.

Airmass Classification and Analysis of Aerosol Types at El Arenosillo (Spain)

Abstract The Aerosol Robotic Network (AERONET) site “El Arenosillo,” equipped with a Cimel sun photometer, has been in operation since 2000. The data collected there are analyzed to establish an aerosol synoptic climatological description that is representative of the region. Different air masses and aerosol types are present over the site depending on the synoptic conditions. The frequent intrusion of dust from the Sahara Desert at El Arenosillo suggested the use of back trajectories to determine the airmass origins of other types of aerosol observed there. The focus of this study is to classify the air masses arriving at El Arenosillo by means of back-trajectory analyses and to characterize the aerosol within each type by means of the aerosol optical depth (AOD) and its spectral signature, given as the Angstrom exponent (AE). The goal is to determine how aerosols observed over the station (receptor site) differ depending on source region and transport pathways. Two classification methods are used, one b...

The strongest desert dust intrusion mixed with smoke over the Iberian Peninsula registered with Sun photometry

[1] We present the analysis of the strongest North African desert dust (DD) intrusion that occurred over the Iberian Peninsula (IP) during the last decade, as registered by modern remote sensing techniques like Sun photometry. This event took place from 22 July to 3 August 2004. The most relevant features of this exceptional event, originated over the Saharan desert, were its great intensity and duration. We focus on the columnar aerosol properties measured by the AERONET-Cimel photometers at El Arenosillo (southwest) and Palencia (north-center) stations. Aerosol optical depth (AOD) reached a maximum of 2.7 at El Arenosillo during 22 July and 1.3 at Palencia on 23 July, with the Ansgtrom exponent values near zero during the AOD peaks. In addition, PM10 concentration levels are also reported at various sites of the IP in order to establish the impact of this intrusion, reaching daily values as high as 200 μg/m 3 and peaks near 600 μg/m 3 in an hourly basis. The interest of this special event is increased because of the mixing with smoke particles from concurrent forest fires in the IP. Features of the columnar volume particle size distribution and derived microphysical parameters, the single scattering albedo, and a reliable estimation of the radiative forcing under these extreme conditions are also reported. Complementary information, as air mass back trajectories, synoptic charts, images, and AOD maps of satellite sensors (SeaWIFS, MODIS) together with NAAPS prognostic model, is used in the analysis in order to draw a detailed scenario of this dust-smoke event over the IP.

Modified calibration procedures for a Yankee Environmental System UVB-1 biometer based on spectral measurements with a brewer spectrophotometer.

Abstract The calibration of the erythemal irradiance measured by a Yankee Environmental System (YES) UVB-1 biometer is presented using two methods of calibration with a wide range of experimental solar zenith angles (SZAs) and ozone values. The calibration is performed through simultaneous spectral measurements by a calibrated double-monochromator Brewer MK-III spectrophotometer at “El Arenosillo” station, located in southwestern Spain. Because the range of spectral measurements of the Brewer spectrophotometer is 290–363 nm, a previously validated radiative transfer model was used to account for the erythemal contribution between 363 and 400 nm. Both methods are recommended by the World Meteorological Organization and we present and discuss here a wide range of results and features given by modified procedures applied to these two general methods. As is well established, the calibration factor for this type of radiometric system is dependent on atmospheric conditions, the most important of which are the ozone content and the SZA. Although the first method is insensitive to these two factors, we analyze this behavior in terms of the range used for the SZA and the use of two different mathematical approaches for its determination. The second method shows the dependence on SZA and ozone content and, thus, a polynomial as a function of SZA or a matrix including SZA and ozone content were determined as general calibration factors for the UV radiometric system. We must note that the angular responses of the YES radiometer and Brewer spectroradiometer have not been considered, because of the difficulty in correcting them. The results show in detail the advantages and drawbacks (and the corresponding associated error) given by the different approaches used for the determination of these calibration coefficients.

Comparison of UV irradiances from Aura/Ozone Monitoring Instrument (OMI) with Brewer measurements at El Arenosillo (Spain) – Part 2: Analysis of site aerosol influence

Several validation studies have shown a notable overestimation of the clear sky ultraviolet (UV) irradiance at the Earth’s surface derived from satellite sensors such as the Total Ozone Mapping Spectrometer (TOMS) and the Ozone Monitoring Instrument (OMI) with respect to groundbased UV data at many locations. Most of this positive bias is attributed to boundary layer aerosol absorption that is not accounted for in the TOMS/OMI operational UV algorithm. Therefore, the main objective of this study is to analyse the aerosol effect on the bias between OMI erythemal UV irradiance (UVER) and spectral UV (305 nm, 310 nm and 324 nm) surface irradiances and ground-based Brewer spectroradiometer measurements from October 2004 to December 2008 at El Arenosillo station (37.1 ◦ N, 6.7 W, 20 m a.s.l.), with meteorological conditions representative of the South-West of Spain. The effects of other factors as clouds, ozone and the solar elevation over this intercomparison were analysed in detail in a companion paper (Ant ón et al., 2010). In that paper the aerosol effects were studied making only a rough evaluation based on aerosol optical depth (AOD) information at 440 nm wavelength (visible range) without applying any correction. We have used the precise information given by single scattering albedo (SSA) from AERONET for the determination of Correspondence to: V. E. Cachorro (chiqui@goa.uva.es) absorbing aerosols which has allowed the correction of the OMI UV data. An aerosol correction expression was applied to the OMI operational UV data using two approaches to estimate the UV absorption aerosol optical depth, AAOD. The first approach was based on an assumption of constant SSA value of 0.91. This approach reduces the OMI UVER bias against the reference Brewer data from 13.4% to 8.4%. Second approach uses daily AERONET SSA values reducing the bias only to 11.6%. Therefore we have obtained a 37% and 12% of improvement respectively. For the spectral irradiance at 324 nm, the OMI bias is reduced from 10.5% to 6.98% for constant SSA and to 9.03% for variable SSA. Similar results were obtained for spectral irradiances at 305 nm, and 310 nm. Contrary to what was expected, the constant SSA approach has a greater bias reduction than variable SSA, but this is a reasonable result according to the discussion about the reliability of SSA values. Our results reflect the level of accuracy that may be reached at the present time in this type of comparison, which may be considered as satisfactory taking into account the remaining dependence on other factors. Nevertheless, improvements must be accomplished to determine reliable absorbing aerosol properties, which appear as a limiting factor for improving OMI retrievals. Published by Copernicus Publications on behalf of the European Geosciences Union. 11868 V. E. Cachorro et al.: Part 2: Analysis of site aerosol influence

Fitting ångström's formula to spectrally resolved aerosol optical thickness

Abstract The ability of the Angstrom equation to represent the spectral behavior of the aerosol optical thickness is analyzed for various atmospheric turbidity conditions. This analysis is carried out by means of the spectral values of the aerosol optical thickness obtained by experimental spectral direct solar irradiance data.

Intercomparison of aerosol optical depth measurements in the UVB using Brewer spectrophotometers and a Li-Cor spectrophotometer

The first Iberian UV radiation intercomparison was held at “El Arenosillo”-Huelva station of the Instituto Nacional de Tecnica Aeroespatial (INTA) from September 1 to 10, 1999. During this campaign, seven Brewer spectrophotometers and one Li-Cor spectrophotometer measured the total column aerosol optical depth (AOD) at 306, 310, 313.5, 316.75 and 320 nm. The AOD calibration of one Brewer was transferred to all other Brewers using one day of intensive measurements. The remaining days were used to observe the stability and reproducibility of the AOD measurements by the different instruments. All Brewer spectrophotometers agreed to within an AOD of 0.03 during the whole measurement campaign. The differences in AOD between the Li-Cor spectrophotometer and the Brewer spectrophotometers were between −0.07 and +0.02 at 313.5, 316.75, and 320 nm. This investigation demonstrates the possibility of using the existing worldwide Brewer network as a global UV aerosol network for AOD monitoring.

Quantifying the respective roles of aerosols and clouds in the strong brightening since the early 2000s over the Iberian Peninsula

The contribution of clouds and aerosols to the decadal variations of downward surface shortwave radiation (SSR) is a current controversial topic. This study proposes a method, which is based on surface-based SSR measurements, aerosol observations, and radiative transfer simulations (in cloud-free and cloud- and aerosol-free scenarios), to evaluate cloud-aerosol (CARE), cloud (CRE), and aerosol (ARE) radiative effects. This method is applied to quantify the role played by, separately, clouds and aerosols on the intense brightening of the SSR observed in the Iberian Peninsula. Clouds and Earths Radiation Energy Budget System (CERES) and surface-based data exhibit an increase in SSR between 2003 and 2012, exceeding +10 W m−2 over this period for some areas of the peninsula. The calculations are performed for three surface-based sites: Barcelona and Valladolid (Spain), and Evora (Portugal). Ranges in monthly values of CARE, CRE, and ARE are (−80, −20), (−60, −20), and (−30, 0), respectively (in W m−2). The average trends for the analyzed period of CARE, CRE, and ARE are +7, +5, and +2 W m−2 per decade, respectively. Overall, three fourths of the SSR trend is explained by clouds, while the other one fourth is related to aerosol changes. The SSR trends explained by the clouds and aerosol radiative effects are in line with the observed reductions in total cloud cover and aerosol load (both at the surface and in the whole atmospheric column). Furthermore, the CRE values are compared against CERES data showing good agreement between both data series, although some discrepancies are observed in their trends.