Virginia O. Lorenz

Quantifying interface and bulk contributions to spin–orbit torque in magnetic bilayers

Spin-orbit interaction-driven phenomena such as the spin Hall and Rashba effect in ferromagnetic/heavy metal bilayers enables efficient manipulation of the magnetization via electric current. However, the underlying mechanism for the spin-orbit interaction-driven phenomena remains unsettled. Here we develop a sensitive spin-orbit torque magnetometer based on the magneto-optic Kerr effect that measures the spin-orbit torque vectors for cobalt iron boron/platinum bilayers over a wide thickness range. We observe that the Slonczewski-like torque inversely scales with the ferromagnet thickness, and the field-like torque has a threshold effect that appears only when the ferromagnetic layer is thinner than 1 nm. Through a thickness-dependence study with an additional copper insertion layer at the interface, we conclude that the dominant mechanism for the spin-orbit interaction-driven phenomena in this system is the spin Hall effect. However, there is also a distinct interface contribution, which may be because of the Rashba effect.

Multimode memories in atomic ensembles

The ability to store multiple optical modes in a quantum memory allows for increased efficiency of quantum communication and computation. Here we compute the multimode capacity of a variety of quantum memory protocols based on light storage in ensembles of atoms. We find that adding a controlled inhomogeneous broadening improves this capacity significantly.

Fast and highly resolved capture of the joint spectral density of photon pairs

Controlling the spatial and spectral–temporal properties of photon pairs produced in artificially structured materials is fundamental to the realization of numerous photonic quantum information applications. Tailoring the joint spectral properties of photon pairs is of particular importance for applications relying on time–energy entanglement, high-visibility interference, and heralding. Yet measuring the joint spectral properties is a time-consuming task requiring coincidence counting, typically resulting in low-resolution spectra with a poor signal-to-noise ratio. In this work we capture the joint spectral correlations of photon pairs that would be produced in optical fibers with unprecedented speed, resolution, and signal-to-noise ratio, using a scheme based on stimulated four-wave mixing. We also illustrate that this technique can be used in engineering joint spectral correlations, making it a powerful tool for studying quantum states.

State engineering of photon pairs produced through dual-pump spontaneous four-wave mixing

We study theoretically the joint spectral properties of photon-pairs produced through spontaneous four-wave mixing (SFWM) with two spectrally distinct pump pulses in optical fibers. We show that, due to the group velocity difference between the pulses, the signature of the interaction can be significantly different from spontaneous parametric down-conversion or SFWM with a single pump pulse. Specifically, we study the case where temporal walk-off between the pumps enables a gradual turn-on and turn-off of the interaction. By utilizing this property, we develop a new approach towards tailoring the spectral correlations within the generated photon pairs, demonstrating the ability to produce factorable photon-pair states, and hence heralded single photons in a pure wave-packet. We show that the use of two pumps is advantageous over single-pump SFWM approaches towards this goal: the usage of the dual-pump configuration enables, in principle, the creation of completely factorable states without any spectral filtering, even in media for which single-pump SFWM tailoring techniques are unsatisfactory, such as standard polarization-maintaining fiber.

Polarization-entangled photon-pair generation in commercial-grade polarization-maintaining fiber

We demonstrate a fiber-based source of polarization-entangled photon pairs at visible wavelengths suitable for integration with local quantum-processing schemes. The photons are created through birefringent phase-matching in spontaneous four-wave mixing inside a Sagnac interferometer. We address entanglement due to temporal distinguishability of the photons to enable the generation of a spectrally unfiltered polarization-entangled photon-pair state with 95.86±0.10% fidelity to a maximally entangled Bell state, evaluated with a tomographic state reconstruction without applying any corrections or background subtractions. Owing to the large birefringence of the fiber, photons are created far detuned from the pump, where Raman contamination is negligible. This source’s spatial mode and ability to produce spectrally uncorrelated photons make it suitable for implementing quantum information protocols over free-space and fiber-based networks.

Efficient spatially resolved multimode quantum memory

Light storage in atomic ensembles has been implemented successfully, but the retrieval efficiency can be low. We propose to improve this efficiency with appropriately phase-matched backward propagating retrieval. This method allows for easy spatial filtering of the retrieved light; in addition, multiple optical modes can be stored in the transverse momentum of the ensemble. We model walk-off effects with a full numerical simulation, and confirm the applicability of the scheme.

High-density, high-temperature alkali vapor cell

We present a vapor cell design that enables resonant optical spectroscopy in high-density, high-temperature alkali metal vapors. Optical access is provided via reflection from the interface between the vapor and a sapphire window. The cell resists corrosion from the highly reactive alkali vapors, in our case, potassium, up to 800 degrees C (number densities up to 10(19) cm(-3)). The cells maintain their integrity for an average of 100 h above 500 degrees C with about 10 heating/cooling cycles.

All-optical vector measurement of spin-orbit-induced torques using both polar and quadratic magneto-optic Kerr effects

We demonstrate that the magneto-optic-Kerr effect with normal light incidence can be used to obtain quantitative optical measurements of both components of spin-orbit-induced torque (both the antidamping and effective-field components) in heavy-metal/ferromagnet bilayers. This is achieved by analyzing the quadratic Kerr effect as well as the polar Kerr effect. The two effects can be distinguished by properly selecting the polarization of the incident light. We use this all-optical technique to determine the spin-orbit torques generated by a series of Pt/Permalloy samples, finding values in excellent agreement with spin-torque ferromagnetic resonance measurements.

Large spin Hall angle in vanadium film

We report a large spin Hall angle observed in vanadium films sputter-grown at room temperature, which have small grain size and consist of a mixture of body centered tetragonal (bct) and body centered cubic (bcc) structures. The spin Hall angle is as large as θV = −0.071 ± 0.003, comparable to that of platinum, θPt = 0.076 ± 0.007, and is much larger than that of bcc V film grown at 400 °C, θV_bcc = −0.012 ± 0.002. Similar to β-tantalum and β-tungsten, the sputter-grown V films also have a high resistivity of more than 200 μΩ∙cm. Surprisingly, the spin diffusion length is still long at 16.3 nm. This finding not only indicates that specific crystalline structure can lead to a large spin Hall effect but also suggests 3d light metals should not be ruled out in the search for materials with large spin Hall angle.

Multidimensional characterization of an entangled photon-pair source via stimulated emission tomography

Using stimulated emission tomography, we characterize an entangled photon-pair source in the energy and polarization degrees of freedom, with a precision far exceeding what could be obtained by quantum state tomography. Through this multidimensional tomography we find that energy-polarization correlations are a cause of polarization-entanglement degradation, demonstrating that this technique provides useful information for source engineering and can accelerate the development of quantum information processing systems dependent on many degrees of freedom.