Vladimir A. Zenin

Boosting Local Field Enhancement by on-Chip Nanofocusing and Impedance-Matched Plasmonic Antennas

Strongly confined surface plasmon-polariton modes can be used for efficiently delivering the electromagnetic energy to nanosized volumes by reducing the cross sections of propagating modes far beyond the diffraction limit, that is, by nanofocusing. This process results in significant local-field enhancement that can advantageously be exploited in modern optical nanotechnologies, including signal processing, biochemical sensing, imaging, and spectroscopy. Here, we propose, analyze, and experimentally demonstrate on-chip nanofocusing followed by impedance-matched nanowire antenna excitation in the end-fire geometry at telecom wavelengths. Numerical and experimental evidence of the efficient excitation of dipole and quadrupole (dark) antenna modes are provided, revealing underlying physical mechanisms and analogies with the operation of plane-wave Fabry-Pérot interferometers. The unique combination of efficient nanofocusing and nanoantenna resonant excitation realized in our experiments offers a major boost to the field intensity enhancement up to ∼12000, with the enhanced field being evenly distributed over the gap volume of 30 × 30 × 10 nm(3), and promises thereby a variety of useful on-chip functionalities within sensing, nonlinear spectroscopy and signal processing.

Direct Characterization of Plasmonic Slot Waveguides and Nanocouplers

We demonstrate the use of amplitude- and phase-resolved near-field mapping for direct characterization of plasmonic slot waveguide mode propagation and excitation with nanocouplers in the telecom wavelength range. We measure modes propagation length, effective index and field distribution and directly evaluate the relative coupling efficiencies for various couplers configurations. We report 26- and 15-fold improvements in the coupling efficiency with two serially connected dipole and modified bow-tie antennas, respectively, as compared to that of the short-circuited waveguide termination.

Directional coupling in channel plasmon-polariton waveguides

We investigate directional couplers (DCs) formed by channel plasmon-polariton (CPP) waveguides (CPPWs). DCs comprising 5-µm-offset S-bends and 40-µm-long parallel CPPWs with different separations (0.08, 0.25, 0.5 and 2 µm) between V-groove channels are fabricated by using a focused ion-beam (FIB) technique in a 2-μm-thick gold film and characterized at telecom wavelengths (1425-1630 nm) with near-field optical microscopy. Experimental results reveal strong coupling, resulting in approximately equal power splitting between DC-CPPWs, for small CPPW separations (0.08 and 0.25 µm). The coupling gradually deteriorates with the increase of separation between V-grooves and practically vanishes for the separation of 2 µm. The DC-CPPW characteristics observed are found in good agreement with finite-element method (implemented in COMSOL) simulations.

White Light Generation and Anisotropic Damage in Gold Films near Percolation Threshold

Strongly enhanced and confined electromagnetic fields generated in metal nanostructures upon illumination are exploited in many emerging technologies by either fabricating sophisticated nanostructures or synthesizing colloid nanoparticles. Here we study effects driven by field enhancement in vanishingly small gaps between gold islands in thin films near the electrically determined percolation threshold. Optical explorations using two-photon luminescence (TPL) and near-field microscopies reveals supercubic TPL power dependencies with white-light spectra, establishing unequivocally that the strongest TPL signals are generated close to the percolation threshold films, and occurrence of extremely confined (∼30 nm) and strongly enhanced (∼100 times) fields at the illumination wavelength. For linearly polarized and sufficiently powerful light, we observe pronounced optical damage with TPL images being sensitive to both wavelength and polarization of illuminating light. We relate these effects to thermally induc...

Near-field characterization of bound plasmonic modes in metal strip waveguides

Propagation of bound plasmon-polariton modes along 30-nm-thin gold strips on a silica substrate at the free-space wavelength of 1500 nm is investigated both theoretically and experimentally when decreasing the strip width from 1500 nm down to the aspect-ratio limited width of 30 nm, which ensures deep subwavelength mode confinement. The main mode characteristics (effective mode index, propagation length, and mode profile) are determined from the experimental amplitude- and phase-resolved near-field images for various strip widths (from 30 to 1500 nm), and compared to numerical simulations. The mode supported by the narrowest strip is found to be laterally confined within ~ 100 nm at the air side, indicating that the realistic limit for radiation nanofocusing in air using tapered metal strips is ~ λ/15.

Directional coupling in long-range dielectric-loaded plasmonic waveguides.

Directional couplers (DCs) based on long-range dielectric-loaded surface plasmon-polariton waveguides (LR-DLSPPWs) operating at telecom wavelengths are studied both numerically and experimentally. The investigated LR-DLSPPWs are formed by ~1.2-µm-high and 1-µm-wide polymer ridges fabricated atop of 15-nm-thick and 500-nm-wide gold stripes supported by a 288-nm-thick Ormoclear polymer deposited on a low-index (n(s) ≈1.34) layer of Cytop. DC structures consisting of sine-shaped S-bends (having an offset of ~10 µm over a distance of ~20 µm) and ~100-µm-long parallel LR-DLSPPWs with a center-to-center separation of 2 µm are characterized using scanning near-field microscopy. The experimentally obtained values of the propagation length (~400 µm), S-bend loss (~4 dB) and coupling length (~100 µm) are found in good agreement with the numerical simulations, indicating a significant potential of LR-DLSPPWs for the realization of various plasmonic components.

Hybrid plasmonic waveguides formed by metal coating of dielectric ridges

Bound hybrid plasmon-polariton modes supported by waveguides, which are formed by gold coating of ridges etched into a silica substrate, are analyzed using numerical simulations and investigated experimentally using near-field microscopy at telecom wavelengths (1425-1625 nm). Drastic modifications of the fundamental mode profile along with changes in the mode confinement and propagation loss are found when varying the ridge height. The main mode characteristics (effective mode index, propagation length, and mode profile) are determined from the experimental amplitude- and phase-resolved near-field images and compared with the simulations. The possibility of strongly influencing the mode properties along with subwavelength confinement found simultaneously with relatively long propagation can further be exploited in mode shaping and sensing applications.

Direct Amplitude-Phase Near-Field Observation of Higher-Order Anapole States

Anapole states associated with the resonant suppression of electric-dipole scattering exhibit minimized extinction and maximized storage of electromagnetic energy inside a particle. Using numerical simulations, optical extinction spectroscopy, and amplitude-phase near-field mapping of silicon dielectric disks, we demonstrate high-order anapole states in the near-infrared wavelength range (900-1700 nm). We develop the procedure for unambiguously identifying anapole states by monitoring the normal component of the electric near-field and experimentally detect the first two anapole states as verified by far-field extinction spectroscopy and confirmed with the numerical simulations. We demonstrate that higher-order anapole states possess stronger energy concentration and narrower resonances, a remarkable feature that is advantageous for their applications in metasurfaces and nanophotonics components, such as nonlinear higher-harmonic generators and nanoscale lasers.

Direct Characterization of Near-Field Coupling in Gap Plasmon-Based Metasurfaces

Metasurfaces based on gap surface-plasmon resonators allow one to arbitrarily control the phase, amplitude, and polarization of reflected light with high efficiency. However, the performance of densely packed metasurfaces is reduced, often quite significantly, in comparison with simple analytical predictions. We argue that this reduction is mainly because of the near-field coupling between metasurface elements, which results in response from each element being different from the one anticipated by design simulations, which are commonly conducted for each individual element being placed in an artificial periodic arrangement. In order to study the influence of near-field coupling, we fabricate meta-elements of varying sizes arranged in quasi-periodic arrays so that the immediate environment of same size elements is different for those located in the middle and at the border of the arrays. We study the near-field using a phase-resolved scattering-type scanning near-field optical microscopy (s-SNOM) and conducting numerical simulations. By comparing the near-field maps from elements of the same size but different placements we evaluate the near-field coupling strength, which is found to be significant for large and densely packed elements. This technique is quite generic and can be used practically for any metasurface type in order to precisely measure the near-field response from each individual element and identify malfunctioning ones, providing feedback to their design and fabrication, thereby allowing one to improve the efficiency of the whole metasurface.

Near-field phase characterization of gradient gap plasmon-based metasurfaces

Metasurface studies have demonstrated vast applications to control optical properties of light based on the ability to design unit cells with desired phase and reflectivity in 2D subwavelength periodic arrays. The simplified design strategy is only an approximation since the unit cells can be subject to near-field coupling effects due to influence from neighbor unit cells. In this work, we try to investigate this effect by numerically and experimentally studying the near-field response from gold nanobricks of varied length, fabricated in both quasi-periodic and periodic configuration on top of dielectric-coated (SiO2) layer and gold layer at telecommunication wavelength (1500 nm), which is the commonly used gap plasmon configuration for efficient metasurfaces. The experimental near-field investigation is performed using a phase-resolved scattering-type scanning near-field optical microscopy (s-SNOM) in the transmission mode. We demonstrate that near-field coupling becomes significant when edge-to-edge separation between GSP elements goes below ~200-250 nm. We also show that the reflection phase of any GSP element is approximately equal to its doubled near-field phase. Thus, our studies provide a direct explanation of a reduced performance of a densely-packed GSP metasurfaces. This technique can accurately predict the performance of different types of metasurfaces by observing their near-field response in different periodic configurations by considering factors ignored in the design stage, which include fabrication uncertainties, wrong design considerations along with near-field coupling effects.