W.A. MacFarlane

Ultrasound attenuation in Sr(2)RuO(4): an angle-resolved study of the superconducting gap function.

We present a study of the electronic ultrasound attenuation alpha in the unconventional superconductor Sr(2)RuO(4). The power law behavior of alpha at temperatures down to T(c)/30 clearly indicates the presence of nodes in the gap. In the normal state, we find an enormous anisotropy of alpha in the basal plane of the tetragonal structure. In the superconducting state, the temperature dependence of alpha also exhibits significant anisotropy. We discuss these results in relation to possible gap functions.

Local magnetic properties of a monolayer of Mn12 single molecule magnets.

The magnetic properties of a monolayer of Mn12 single molecule magnets grafted onto a silicon (Si) substrate have been investigated using depth-controlled beta-detected nuclear magnetic resonance. A low-energy beam of spin-polarized radioactive 8Li was used to probe the local static magnetic field distribution near the Mn12 monolayer in the Si substrate. The resonance line width varies strongly as a function of implantation depth as a result of the magnetic dipolar fields generated by the Mn12 electronic magnetic moments. The temperature dependence of the line width indicates that the magnetic properties of the Mn12 moments in this low-dimensional configuration differ from bulk Mn12.

Persistence of Li Induced Kondo Moments in the Superconducting State of Cuprates

Using 7Li NMR shift data, the anomalous local moment induced by spinless Li impurities persists below T(c) in YBa 2Cu 3O6+y. In the underdoped regime, the moments retain their Curie law below Tc. In contrast, near optimal doping, the large Kondo screening observed above Tc (TK = 135 K) is strongly reduced below Tc as expected theoretically when the superconducting gap develops. The limited spatial extent of the induced moment (on first near neighbor Cu) is not drastically modified below Tc, which allows a comparison with STM determination of the local density of states. Our results constrain theoretical models of the impurity electronic properties.

Nature of weak magnetism in SrTiO3/LaAlO3 multilayers.

We report the observation of weak magnetism in superlattices of LaAlO(3)/SrTiO(3) using β-detected nuclear magnetic resonance. The spin lattice relaxation rate of ^{8}Li in superlattices with a spacer layers of 8 and 6 unit cells of LaAlO(3) exhibits a strong peak near ~35 K, whereas no such peak is observed in a superlattice with spacer layer thickness of 3 unit cells. We attribute the observed temperature dependence to slowing down of weakly coupled electronic moments at the LaAlO(3)/SrTiO(3) interface. These results show that the magnetism at the interface depends strongly on the thickness of the spacer layer, and that a minimal thickness of ~4-6 unit cells is required for the appearance of magnetism. A simple model is used to determine that the observed relaxation is due to small fluctuating moments (~0.002μ(B)) in the two samples with a larger LaAlO(3) spacer thickness.

Near-Surface Structural Phase Transition of SrTiO~3 Studied with Zero-Field beta-Detected Nuclear Spin Relaxation and Resonance

We demonstrate that zero-field beta-detected nuclear quadrupole resonance and spin relaxation of low energy (8)Li can be used as a sensitive local probe of structural phase transitions near a surface. We find that the transition near the surface of a SrTiO(3) single crystal occurs at T(c) approximately 150K, i.e., approximately 45K higher than T(c)bulk, and that the tetragonal domains formed below T(c) are randomly oriented.

Muon spin relaxation investigation of the spin dynamics of geometrically frustrated antiferromagnets Y2Mo2O7 and Tb2Mo2O7.

The spin dynamics of geometrically frustrated pyrochlore antiferromagnets Y2Mo2O7 and Tb2Mo2O7 have been investigated using muon spin relaxation. A dramatic slowing down of the moment fluctuations occurs as one approaches the spin freezing temperatures (TF=22 K and 25 K respectively) from above. Below TF there is a disordered magnetic state similar to that found in a spin glass but with a residual muon spin relaxation rate at low temperatures. These results show that there is a large density of states for magnetic excitations in these systems near zero energy.

Muon-Spin Rotation Measurements of the Magnetic Field Dependence of the Vortex-Core Radius and Magnetic Penetration Depth in NbSe{sub 2}

Muon-spin rotation spectroscopy ({mu}SR) has been used to measure the internal magnetic field distribution in NbSe{sub 2} for H{sub c1}{lt}H{lt}0.25H{sub c2} . The deduced profiles of the supercurrent density J{sub s} indicate that the vortex-core radius {rho}{sub 0} in the bulk decreases sharply with increasing magnetic field. This effect, which is attributed to increased vortex-vortex interactions, does not agree with the dirty-limit microscopic theory. A simple phenomenological equation in which {rho}{sub 0} depends on the intervortex spacing is used to model this behavior. In addition, we find for the first time that the in-plane magnetic penetration depth {lambda}{sub ab} increases linearly with H in the vortex state of a conventional superconductor. {copyright} {ital 1997} {ital The American Physical Society}

Low-energy spin-polarized radioactive beams as a nano-scale probe of matter

Abstract We have commissioned a polarized low-energy 8 Li ion beam line, which together with a high-field β-NMR spectrometer, can act as sensitive new probe of thin films and interfaces. The implantation energy can be continuously adjusted from 1 to 90 keV and the maximum polarization achieved thus far is 80%. This instrument opens up new applications for β-NMR which parallel and complement efforts with low-energy muons. For example, it is possible to probe the magnetic field distribution near the surface of a material by stopping a polarized 8 Li beam in a thin overlayer of Ag. Since the 8 Li adopts a site with cubic symmetry in Ag there is no quadrupolar splitting of the resonance, and the 8 Li acts as a purely magnetic sensor.

Magnetic-field effects on the size of vortices below the surface of NbSe2 detected using low energy beta-NMR.

A low energy radioactive beam of polarized

MEASUREMENT OF THE FUNDAMENTAL LENGTH SCALES IN THE VORTEX STATE OF YBA2CU3O6.60

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