Wei Ruan

Electron interaction-driven insulating ground state in Bi2Se3 topological insulators in the two-dimensional limit

We report a transport study of ultrathin Bi

Characterization of collective ground states in single-layer NbSe2

{}_{2}

Probing the Role of Interlayer Coupling and Coulomb Interactions on Electronic Structure in Few-Layer MoSe2 Nanostructures

Se

Visualizing the atomic-scale electronic structure of the Ca2CuO2Cl2 Mott insulator

{}_{3}

Imaging the coexistence of superconductivity and a charge density modulation in K

topological insulators with thickness from one quintuple layer to six quintuple layers grown on sapphire by molecular beam epitaxy. At low temperatures, the film resistance increases logarithmically with decreasing temperature, revealing an insulating ground state. The insulating behavior becomes more pronounced in thinner films. The sharp increase of resistance with magnetic field, however, indicates the existence of weak antilocalization originated from the topological protection. We show that this unusual insulating ground state in the two-dimensional limit of topological insulators is induced by the combined effect of strong electron interaction and topological delocalization.

_{0.73}

What happens to correlated electronic phases—superconductivity and charge density wave ordering—as a material is thinned? Experiments show that both can remain intact in just a single layer of niobium diselenide.

Fe

Despite the weak nature of interlayer forces in transition metal dichalcogenide (TMD) materials, their properties are highly dependent on the number of layers in the few-layer two-dimensional (2D) limit. Here, we present a combined scanning tunneling microscopy/spectroscopy and GW theoretical study of the electronic structure of high quality single- and few-layer MoSe2 grown on bilayer graphene. We find that the electronic (quasiparticle) bandgap, a fundamental parameter for transport and optical phenomena, decreases by nearly one electronvolt when going from one layer to three due to interlayer coupling and screening effects. Our results paint a clear picture of the evolution of the electronic wave function hybridization in the valleys of both the valence and conduction bands as the number of layers is changed. This demonstrates the importance of layer number and electron–electron interactions on van der Waals heterostructures and helps to clarify how their electronic properties might be tuned in future 2D nanodevices.

_{1.67}

Although the mechanism of superconductivity in the cuprates remains elusive, it is generally agreed that at the heart of the problem is the physics of doped Mott insulators. A crucial step for solving the high temperature superconductivity puzzle is to elucidate the electronic structure of the parent compound and the behaviour of doped charge carriers. Here we use scanning tunnelling microscopy to investigate the atomic-scale electronic structure of the Ca(2)CuO(2)Cl(2) parent Mott insulator of the cuprates. The full electronic spectrum across the Mott-Hubbard gap is uncovered for the first time, which reveals the particle-hole symmetric and spatially uniform Hubbard bands. Defect-induced charge carriers are found to create broad in-gap electronic states that are strongly localized in space. We show that the electronic structure of pristine Mott insulator is consistent with the Zhang-Rice singlet model, but the peculiar features of the doped electronic states require further investigations.

Se

We report scanning tunneling microscopy studies of the local structural and electronic properties of the iron selenide superconductor K0.73Fe1.67Se2 with TC = 32K. On the atomically resolved FeSe surface, we observe well-defined superconducting gap and the microscopic coexistence of a charge density modulation with root2*root2 periodicity with respect to the original Se lattice. We propose that a possible origin of the pattern is the electronic superstructure caused by the block antiferromagnetic ordering of the iron moments. The widely expected iron vacancy ordering is not observed, indicating that it is not a necessary ingredient for superconductivity in the intercalated iron selenides.

_{2}

Although the origin of high temperature superconductivity in the iron pnictides is still under debate, it is widely believed that magnetic interactions or fluctuations have a crucial role in triggering Cooper pairing. A key issue regarding the iron pnictide phase diagram is whether long-range magnetic order can coexist with superconductivity microscopically. Here we use scanning tunnelling microscopy to investigate the local electronic structure of underdoped NaFe1-xCoxAs near the spin density wave and superconducting phase boundary. Spatially resolved spectroscopy directly reveals both the spin density wave and superconducting gaps at the same atomic location, providing compelling evidence for the microscopic coexistence of the two phases. The strengths of the two orders are shown to anti-correlate with each other, indicating the competition between them. This work implies that Cooper pairing in the iron pnictides can occur when portions of the Fermi surface are already gapped by the spin density wave order.