Wonkeun Chang

Ultrafast nonlinear optics in gas-filled hollow-core photonic crystal fibers [Invited]

We review the use of hollow-core photonic crystal fibers (PCFs) in the field of ultrafast gas-based nonlinear optics, including recent experiments, numerical modeling, and a discussion of future prospects. Concentrating on broadband guiding kagome-style hollow-core PCF, we describe its potential for moving conventional nonlinear fiber optics both into extreme regimes—such as few-cycle pulse compression and efficient deep ultraviolet wavelength generation—and into regimes hitherto inaccessible, such as single-mode guidance in a photoionized plasma and high-harmonic generation in fiber.

Dissipative soliton resonances in laser models with parameter management

Dissipative soliton resonance (DSR) is a phenomenon where the energy of a soliton in a dissipative system increases without limit at certain values of the system parameters. We have found that the DSR phenomenon is robust and does not disappear when perturbations are introduced into the model. In particular, parameter management is benign to DSR: the resonance property remains intact even when a pulse experiences periodic changes of system parameters in a laser cavity. We also show that high energy pulses emerging from a laser cavity can be compressed to shorter durations with the help of linear dispersive devices.

Ultrafast nonlinear dynamics of surface plasmon polaritons in gold nanowires due to the intrinsic nonlinearity of metals

Starting from first principles, we theoretically model the nonlinear temporal dynamics of gold-based plasmonic devices resulting from the heating of their metallic components. At optical frequencies, the gold susceptibility is determined by the interband transitions around the X, L points in the first Brillouin zone, and thermo-modulational effects ensue from Fermi smearing of the electronic energy distribution in the conduction band. As a consequence of light-induced heating of the conduction electrons, the optical susceptibility becomes nonlinear. In this paper we describe, for the first time to our knowledge, the effects of the thermo-modulational nonlinearity of gold on the propagation of surface plasmon polaritons guided on gold nanowires. We introduce a novel nonlinear Schr¨ odinger-like equation to describe pulse propagation in such nanowires, and we predict the appearance of an intense spectral red-shift caused by the delayed thermal response.

Midinfrared frequency combs from coherent supercontinuum in chalcogenide and optical parametric oscillation

We observe the coherence of the supercontinuum generated in a nanospike chalcogenide-silica hybrid waveguide pumped at 2 μm. The supercontinuum is shown to be coherent with the pump by interfering it with a doubly resonant optical parametric oscillator (OPO) that is itself coherent with the shared pump laser. This enables coherent locking of the OPO to the optically referenced pump frequency comb, resulting in a composite frequency comb with wavelengths from 1 to 6 μm.

Influence of ionization on ultrafast gas-based nonlinear fiber optics

We numerically investigate the effect of ionization on ultrashort high-energy pulses propagating in gas-filled kagomé-lattice hollow-core photonic crystal fibers by solving an established uni-directional field equation. We consider the dynamics of two distinct regimes: ionization induced blue-shift and resonant dispersive wave emission in the deep-UV. We illustrate how the system evolves between these regimes and the changing influence of ionization. Finally, we consider the effect of higher ionization stages.

Combined soliton pulse compression and plasma-related frequency upconversion in gas-filled photonic crystal fiber

We numerically investigate self-frequency blueshifting of a fundamental soliton in a gas-filled hollow-core photonic crystal fiber. Because of the changing underlying soliton parameters, the blueshift gives rise to adiabatic soliton compression. Based on these features, we propose a device that enables frequency shifting over an octave and pulse compression from 30 fs down to 2.3 fs.

Positive and negative curvatures nested in an antiresonant hollow-core fiber

We propose a negative curvature hollow-core fiber that has a nested elliptical element in the antiresonant tubes. The additional elliptical element effectively adds two curvatures, namely, a positive and a negative curvature. Our numerical study shows that it enhances the confinement of the light in the core. Moreover, the nested elements provided an extra degree of freedom that can be exploited to suppress higher-order modes through the change of the ellipticity. The resulting low confinement loss and single-mode guidance properties of the proposed fiber make it a suitable candidate for applications in ultrashort pulse delivery and gas-based nonlinear systems.

Influence of timing jitter on nonlinear dynamics of a photonic crystal fiber ring cavity

We demonstrate that timing jitter has a strong influence on supercontinua generated in a photonic crystal fiber ring cavity synchronously pumped by 140 fs pulses. The global dynamics with respect to cavity detuning is analyzed both numerically and experimentally by tracking the cavity pulse energy. The results show that low-frequency timing jitter, induced by both the pump oscillator and the external cavity, masks the fine underlying bifurcation structure of the system. Numerical simulations in the absence of timing jitter reveal that the system dynamics fall into four qualitatively different regimes. The existence of these regimes is experimentally observed in first-return diagrams.

Observation of Coexisting Dissipative Solitons in a Mode-Locked Fiber Laser.

We show, experimentally and numerically, that a mode-locked fiber laser can operate in a regime where two dissipative soliton solutions coexist and the laser will periodically switch between the solutions. The two dissipative solitons differ in their pulse energy and spectrum. The switching can be controlled by an external perturbation and triggered even when switching does not occur spontaneously. Numerical simulations unveil the importance of the double-minima loss spectrum and nonlinear gain to the switching dynamics.

Raman-free nonlinear optical effects in high pressure gas-filled hollow core PCF

The effective Kerr nonlinearity of hollow-core kagomé-style photonic crystal fiber (PCF) filled with argon gas increases to ~15% of that of bulk silica glass when the pressure is increased from 1 to 150 bar, while the zero dispersion wavelength shifts from 300 to 900 nm. The group velocity dispersion of the system is uniquely pressure-tunable over a wide range while avoiding Raman scattering-absent in noble gases-and having an extremely high optical damage threshold. As a result, detailed and well-controlled studies of nonlinear effects can be performed, in both normal and anomalous dispersion regimes, using only a fixed-frequency pump laser. For example, the absence of Raman scattering permits clean observation, at high powers, of the interaction between a modulational instability side-band and a soliton-created dispersive wave. Excellent agreement is obtained between numerical simulations and experimental results. The system has great potential for the realization of reconfigurable supercontinuum sources, wavelength convertors and short-pulse laser systems.