Xue-Fang Sang
Sun Yat-sen University
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Tellus B | 2011
Guenter Engling; Yi-Nan Zhang; Chuen-Yu Chan; Xue-Fang Sang; Mang Lin; K.F. Ho; Y.S. Li; Chuan-Yao Lin; James J. Lee
The Tibetan Plateau is one of the highest regions in theworld, exerting profound influence on the large-scale atmospheric circulation of Asia and the global climate. Here we report ambient concentrations of black carbon (BC), aerosol mass (PM2.5 and PM10) and associated carbonaceous species and water-soluble inorganic ions from a remote mountain site in the southeastern part of the Tibetan Plateau during spring, in order to characterize the major sources contributing to the ambient aerosol in the background atmosphere of Southeast Asia. Significant build-up of aerosol and BC concentrations was observed during a dry period, accompanied by the occurrence of fires and transport of pollution from the nearby regions of Southeast Asia and the northern part of the Indian Peninsula. The concentrations of BC, PM2.5 and PM10 mass reached maximum hourly values of 1470 ng m-3, 107 and 117 μg m-3, respectively. Organic carbon (OC), elemental carbon (EC) and sulfate were the predominant aerosol components. OC showed strong correlations with EC (R2 = 0.93 for PM2.5 and 0.74 for PM10) and non-sea-salt potassium, especially in fine aerosol (R2 = 0.95). In addition, the relative change rates of K+ against OC reached characteristically high values, highlighting the important contributions of biomass-burning smoke.
Tellus B | 2011
Xue-Fang Sang; Chuen-Yu Chan; Guenter Engling; Lo-Yin Chan; Xuemei Wang; Yi-Nan Zhang; Si Shi; Zhisheng Zhang; Ting Zhang; Ming Hu
An intensive field experiment was conducted at an urban and a rural site in Hong Kong to identify the influence of biomass burning emissions transported from distinct regions on ambient aerosol in coastal southeast China. Watersoluble ionic and carbonaceous species, specifically the biomass burning tracer levoglucosan, were analysed. Elevated levoglucosan concentrations with maxima of 91.5 and 133.7 ng m-3 and overall average concentrations of 30 and 36 ng m-3 were observed at the rural and urban sites, respectively. By combining the analysed meteorological data, backward trajectories, fire counts and Aerosol Index from the Earth Probe satellite, southwest China and the northern Philippines, together with the southeast China coast, were identified for the first time as source regions of the transported biomass burning particles at the surface level in rural Hong Kong. Occasional levoglucosan enhancements observed at urban Hong Kong were attributed to local incense and joss paper burning during the Ching-Ming festival period. The contributions of transported biomass burning emissions, especially from the northern Philippines, were estimated to account for 7.5% and 2.9% of OC and PM2.5, respectively.
Archive | 2011
Chuen-Yu Chan; Guenter Engling; Xue-Fang Sang; Ting Zhang
Biofuels have recently gained much attention, mainly as alternative fuels for applications in energy generation and transportation. The utilization of biofuels in such controlled combustion processes has the great benefit of not further depleting the limited resources of fossil fuels, yet it is associated with emissions of greenhouse gases and smoke particles similar to traditional combustion processes, i.e., those of fossil fuels. On the other hand, a vast amount of biofuels is subject to combustion in small-scale processes, such as for heating and cooking in residential dwellings, as well as in agricultural operations, such as for crop residue removal and land clearing. In addition, large amounts of biomass are consumed annually during forest and savanna fires in many parts of the world. These types of burning processes are typically uncontrolled and unregulated. Consequently, the emissions from such processes may be substantially larger compared to industrial-type operations. Aside from direct effects on human health, especially due to a sizeable fraction of the smoke emissions remaining inside residential homes, the smoke particles and gases released from uncontrolled biofuel combustion impose significant effects on regional and global climate. Estimates have shown the majority of carbonaceous airborne particulate matter to be derived from the combustion of biofuels and biomass. The resulting “clouds” of carbonaceous aerosol particles nowadays span vast areas across the Globe. Aside from the negative health impacts and influence on global climate, these smoke particles affect biogeochemical cycles and regional air quality, which is also associated with severe economic impacts. Whereas emissions from industrial operations and traffic have been fairly well characterized, smoke released during combustion of biofuels is poorly understood in terms of its chemical composition and physical properties. Biofuel combustion generates smoke particles which are predominantly of carbonaceous nature, consisting of an organic carbon (OC) and an elemental carbon (EC) fraction, the latter of which is at times mistakenly referred to as black carbon (BC) or soot. While the OC and EC fractions can be quantified by various methods, there is a large gap in our knowledge regarding the specific composition of OC in biofuel smoke particles. In fact, OC is composed of thousands of individual organic compounds with a wide range of chemical and physical properties. Recent advances in the
Environmental Research Letters | 2010
Ting Zhang; Guenter Engling; Chuen-Yu Chan; Yi-Nan Zhang; Zhisheng Zhang; Mang Lin; Xue-Fang Sang; Youping Li; Y.S. Li
Atmospheric Environment | 2013
Xue-Fang Sang; Zhisheng Zhang; Chuenyu Chan; Guenter Engling
Environmental Science and Pollution Research | 2012
Yi-Nan Zhang; Zhisheng Zhang; Chuen-Yu Chan; Guenter Engling; Xue-Fang Sang; Si Shi; Xuemei Wang
Atmospheric Environment | 2015
Zhisheng Zhang; Jian Gao; Guenter Engling; Jun Tao; Fahe Chai; Leiming Zhang; Renjian Zhang; Xue-Fang Sang; Chuen-Yu Chan; Zejian Lin; Junji Cao
Aerosol and Air Quality Research | 2013
Dalei Wu; Mang Lin; Chuen-Yu Chan; Wei-Zhong Li; Jun Tao; Youping Li; Xue-Fang Sang; Chun-Wei Bu; Nanhai District
Atmospheric Environment | 2011
Yi-Nan Zhang; Y.R. Xiang; Lo-Yin Chan; Chuen-Yu Chan; Xue-Fang Sang; R. Wang; H.X. Fu
Atmospheric Pollution Research | 2014
Xiaocui Chen; Zhisheng Zhang; Guenter Engling; Renjian Zhang; Jun Tao; Mang Lin; Xue-Fang Sang; Chuen-Yu Chan; Shiyu Li; Youping Li