Y. Tanimura

Development of the Neutron Calibration Fields using Accelerators at FRS and TIARA of JAEA

The neutron calibration fields using accelerators have been developed at the Facility of Radiation Standards (FRS) of JAEA-Tokai for neutrons below 20 MeV and at Takasaki Ion Accelerators for Advanced Radiation Application (TIARA) of JAEA-Takasaki for those over 20 MeV. At FRS, monoenergetic neutrons are generated by using proton or deuteron beam from a 4 MV Van-de-Graaff (Pelletron) accelerator. Up until the present, developments of the 8, 144, 250, 565 keV, 5.0 and 14.8 MeV fields have been completed. As procedure for the development, measurement of neutron energy spectrum, peak energy and reference fluence, development of monitoring scheme for neutron fluence and establishment of the traceability on neutron fluence to the primary standards were achieved. At TIARA, three neutron fields of 45, 60 and 75 MeV are planned to be established. Quasi-monoenergetic neutrons are generated from 7Li(p,n)7Be reaction by using proton beam from an AVF cyclotron, and led into an irradiation room through a cylindrical collimator, 3 m in thickness. Evaluation of the characteristics of the fields needed for the development as the standard calibration fields is in progress now.

Response Functions of Phoswich-Type Neutron Detector for High-Energy Cosmic Ray Neutron Measurement

A phoswich-type neutron detector was developed in order to measure high-energy cosmic ray neutron spectra in aircraft. The neutron detector consists of an EJ309 organic liquid scintillator that is 121.7mm in diameter and 121.7mm in length and is covered with a 15mm thick EJ299-13 outer plastic scintillator. The neutron response functions of the detector are required for the unfolding method to obtain the energy spectrum. The neutron response functions were created based on MCNPX simulations using an anticoincidence mode with the experimental light-output correlations with particle energies, uniformity of light collection and energy resolutions. The light-output correlation with particle energy, the uniformity of light collection and the energy resolutions were evaluated based on experiments. Measurements of neutron response functions were performed using four quasi-monoenergetic neutron beams from 40 to 80 MeV p-Li reactions to verify the calculated results. The calculated response functions show good agreement with the measurements. The angular response of the phoswich detector was confirmed to be isotropic from the calculation. The photon response functions of the detector were also calculated and agreed well with the measurements for 6.129MeV photons. Neutron and photon response matrices were created up to 300 and 50 MeV, respectively, over a wide energy range for experimental flights.

Time-of-Flight Measurements for Low-Energy Components of 45-MeV Quasi-Monoenergetic High-Energy Neutron Field from

A quasi-monoenergetic neutron field generated in the 7Li(p, n) reaction consists of a high-energy monoenergetic peak and a continuum to the low-energy region. In this study, the spectral fluence of the continuum was measured with the time-of-flight (TOF) method using a 6Li-glass scintillation detector and an organic liquid scintillation detector for the keV and MeV region, respectively. The neutron spectral fluence was determined down to the keV region by implementing a new beam chopping system and the results showed that the neutrons that came directly from the target had a lower energy limit about 100 keV. Discussions were made also on the effect of the time-independent neutrons which are assumed to be room-scattered neutrons. The obtained information is expected to contribute to understanding the quasi-monoenergetic high-energy neutron field and improvements of calibrating neutron detectors in the field.

{^7{\rm Li}({\rm p}, {\rm n})}

A portable, light-weight long counter (LC) with small dimensions was developed. This LC consists of a (3)He thermal neutron counter, a cylindrical moderator and outer shields. It was designed to have an almost flat response in a neutron energy range of 0.4 eV to 5 MeV. The portable LC has a radius of 11 cm and a length of 39 cm. Its weight was successfully reduced to 15 kg. Polystyrene was employed instead of polyethylene for the front part of the moderator in order to increase the sensitivity to low-energy neutrons. The response function calculated using the MCNP code was consistent with the results of experiments using monoenergetic neutron calibration fields.

Reaction

The 6- to 7-MeV high-energy gamma-ray calibration field by the (19)F(p, αγ)(16)O reaction is to be served at the Japan Atomic Energy Agency. For the determination of air kerma rates using an ionisation chamber in the 6- to 7-MeV high-energy gamma-ray field, the establishment of the charged particle equilibrium must be achieved during measurement. In addition to measurement of air kerma rates by the ionisation chamber with a thick build-up cap, measurement using the ionisation chamber and a build-up plate (BUP) was attempted, in order to directly determine air kerma rates under the condition of regular calibration for ordinary survey meters and personal dosemeters. Before measurements, Monte Carlo calculations were made to find the optimum arrangement of BUP in front of the ionisation chamber so that the charged particle equilibrium could be well established. Measured results imply that air kerma rates for the 6- to 7-MeV high-energy gamma-ray field could be directly determined under the appropriate condition using an ionisation chamber coupled with build-up materials.

Development of portable long counter with two different moderator materials

A compact single ion irradiation system has been developed to examine energetic particle effects on materials and devices. The system has been constructed by use of commercially available and inexpensive standard components and can be easily recomposed according to beam requirements for various irradiation experiments. The beam adjustment was automatically performed in obedience to a computer program based on a modified SIMPLEX method. The beam performances of the system, i.e., pulse width, the number of ions included in one pulse and beam size were examined by use of a microchannel plate, a SI-SSD, a CCD image sensor and a CR-39 track detector, respectively. A beam of a single ion, 1 nsec in pulse width and several /spl mu/m in diameter has been successfully produced by this system.

Measurement of air kerma rates for 6- to 7-MeV high-energy gamma-ray field by ionisation chamber and build-up plate

ABSTRACT In this study, we developed a 45 MeV neutron fluence rate standard of Japan. Quasi-monoenergetic neutrons with a peak energy of 45 MeV in the neutron standard field were produced by the 7Li(p,n)7Be reaction using a 50-MeV proton beam from an azimuthally varying field (AVF) cyclotron of the Takasaki Ion Accelerators for Advanced Radiation Application (TIARA). The neutron energy spectrum was measured using an organic liquid scintillation detector and a 6Li-glass scintillation detector by the time-of-flight method, and using a Bonner sphere spectrometer by the unfolding method. The absolute neutron fluence was determined using a proton recoil telescope (PRT) composed of the liquid scintillation detector and a Si(Li) detector that was newly developed in the present study. The detection efficiency of the PRT was obtained using the MCNPX code. The peak neutron production cross section for the 7Li(p,n)7Be reaction was also derived from the neutron fluence in order to confirm the neutron fluence of the TIARA high-energy neutron field. The peak neutron production cross section obtained in the present study was in good agreement with those of previous studies. The characteristics of the 45-MeV neutron field in TIARA were successfully evaluated in order to calibrate high-energy neutron detectors and high-energy neutron dosimeters.

Development of a compact single ion irradiation system

A quasi-monoenergetic high-energy neutron field produced via 7Li(p,n) reaction consists of a high-energy peak and a continuum down to the low-energy region. The continuum is a background for the measurement for the peak neutrons. Spectral information is necessary to estimate the effect of it. Using a new beam chopping system, the spectral neutron fluence above ~150 keV was measured by the TOF method. The lower-energy neutrons are time-independent and the unfolding method using the Bonner sphere spectrometer (BSS) is suitable to measure them. However, the common BSS with a 3He or BF3 proportional counter has difficulties in this case: signals caused by high-energy-charged particle are mixed in with the genuine signals caused by thermalized neutrons and the dead-time corrections are difficult in experiments with the pulsed-neutron beam. The gold foil is therefore adopted as a detector element for the BSS. Response matrix of the gold-activation BSS is evaluated by Monte Carlo calculations and response calibrations at a neutron standard facility of the AIST. Measurements for the quasi-monoenergetic high-energy neutron field was performed at the AVF cyclotron facility of TIARA, at the peak neutron energy of 45 MeV.

Development of the high-energy neutron fluence rate standard field in Japan with a peak energy of 45 MeV using the 7Li(p,n)7Be reaction at TIARA

An attempt to decrease the anisotropic emissions of neutrons from a cylindrical (241)Am-Be-encapsulated X3 source was conducted with Monte Carlo calculations and experiments. The influence of metal materials and shapes of the external casing to the anisotropy factor were focussed on. Results obtained by calculations using MCNP4C implied that a light and spherical-shaped external casing decreases the anisotropic emission of neutrons. Experimental results using the spherical-shaped aluminium protection case also revealed that the anisotropy factor was close to 1.0 with wide zenith angle ranges.

Development and evaluation of activation neutron detectors for spectrum measurements of quasi-monoenergetic high-energy neutron fields

A high-efficiency proton recoil telescope was developed to determine neutron fluences in neutron fields using the 3H(d,n)4He reaction. A 2-mm thick plastic scintillation detector was employed as a radiator to increase the detection efficiency and compensate for the energy loss of the recoil proton within. Two silicon detectors were employed as the ΔE and E detectors. The distance between the radiator and the E detector was varied between 50 and 150 mm. The telescope had detection efficiencies of 3.5 × 10-3 and 7.1 × 10-4 cm2 for distances of 50 and 100 mm, respectively, which were high enough to determine the neutron fluence in 14.8-MeV neutron fields, with a few thousand cm-2 s-1 fluence rate, within a few hours.