Yanko Todorov

Ultrastrong Light-Matter Coupling Regime with Polariton Dots

The regime of ultrastrong light-matter interaction has been investigated theoretically and experimentally, using zero-dimensional electromagnetic resonators coupled with an electronic transition between two confined states of a semiconductor quantum well. We have measured a splitting between the coupled modes that amounts to 48% of the energy transition, the highest ratio ever observed in a light-matter coupled system. Our analysis, based on a microscopic quantum theory, shows that the nonlinear polariton splitting, a signature of this regime, is a dynamical effect arising from the self-interaction of the collective electronic polarization with its own emitted field.

Optical properties of metal-dielectric-metal microcavities in the THz frequency range

We present an experimental and theoretical study of the optical properties of metal-dielectric-metal structures with patterned top metallic surfaces, in the THz frequency range. When the thickness of the dielectric slab is very small with respect to the wavelength, these structures are able to support strongly localized electromagnetic modes, concentrated in the subwavelength metal-metal regions. We provide a detailed analysis of the physical mechanisms which give rise to these photonic modes. Furthermore, our model quantitatively predicts the resonance positions and their coupling to free space photons. We demonstrate that these structures provide an efficient and controllable way to convert the energy of far field propagating waves into near field energy.

Electrically injected cavity polaritons

We have realised an electroluminescent device in which electron are injected into intersubband polariton branches. We reproduce electroluminescence spectra by using a phenomenological model, in which a voltage dependent injection is taken into account.

Coupling of a surface plasmon with localized subwavelength microcavity modes

Midinfrared photonic modes of a periodically patterned metal-dielectric-metal structure have been investigated theoretically and experimentally. We have observed an anticrossing behavior between cavity modes localized in the double-metal regions and the surface plasmon polariton, signature of a hybridization between the two modes.

Antenna-coupled microcavities for enhanced infrared photo-detection

We demonstrate mid-infrared detectors embedded into an array of double-metal nano-antennas. The antennas act as microcavities that squeeze the electric field into thin semiconductor layers, thus enhancing the detector responsivity. Furthermore, thanks to the ability of the antennas to gather photons from an area larger than the devices physical dimensions, the dark current is reduced without hindering the photo-generation rate. In these devices, the background-limited performance is improved with a consequent increase of the operating temperature. Our results illustrate how the antenna-coupled microcavity concept can be applied to enhance the performances of infrared opto-electronic devices.

Charge-induced coherence between intersubband plasmons in a quantum structure.

In this Letter we investigate a low dimensional semiconductor system, in which the light-matter interaction is enhanced by the cooperative behavior of a large number of dipolar oscillators, at different frequencies, mutually phase locked by Coulomb interaction. We experimentally and theoretically demonstrate that, owing to this phenomenon, the optical response of a semiconductor quantum well with several occupied subbands is a single sharp resonance, associated with the excitation of a bright multisubband plasmon. This effect illustrates how the whole oscillator strength of a two-dimensional system can be concentrated into a single resonance independently from the shape of the confining potential. When this cooperative excitation is tuned in resonance with a cavity mode, their coupling strength can be increased monotonically with the electronic density, allowing the achievement of the ultrastrong coupling regime up to room temperature.

Ultra-strong light–matter coupling for designer Reststrahlen band

The strength of the light–matter interaction depends on the number of dipoles that can couple with the photon trapped in an optical cavity. The coupling strength can thus be maximized by filling the entire cavity volume with an ensemble of interacting dipoles. In this work this is achieved by inserting a highly doped semiconductor layer in a subwavelength plasmonic resonator. In our system the ultra-strong light–matter coupling occurs between a collective electronic excitation and the cavity photon. The measured coupling strength is 73% of the matter excitation energy, the highest ever reported for a light–matter coupled system at room temperature. We experimentally and theoretically demonstrate that such an ultra-strong interaction modifies the optical properties on a very wide spectral range (20–250 meV), and results in the appearance of a photonic gap of 38 meV, independently of the light polarization and angle of incidence. Light–matter ultra-strong coupling can thus be exploited to conceive metasurfaces with an engineered reflectivity band.

Strong near field enhancement in THz nano-antenna arrays

A key issue in modern photonics is the ability to concentrate light into very small volumes, thus enhancing its interaction with quantum objects of sizes much smaller than the wavelength. In the microwave domain, for many years this task has been successfully performed by antennas, built from metals that can be considered almost perfect at these frequencies. Antenna-like concepts have been recently extended into the THz and up to the visible, however metal losses increase and limit their performances. In this work we experimentally study the light coupling properties of dense arrays of subwavelength THz antenna microcavities. We demonstrate that the combination of array layout with subwavelength electromagnetic confinement allows for 104-fold enhancement of the electromagnetic energy density inside the cavities, despite the low quality factor of a single element. This effect is quantitatively described by an analytical model that can be applied for the optimization of any nanoantenna array.

Intersubband Polaritons in the Electrical Dipole Gauge

We provide a theoretical description for the coupling between the intersubband excitations of a bi-dimensional electron gas with the electromagnetic field. This description, based on the electrical dipole gauge, applies to an arbitrary quantum heterostructure embedded in a general multilayered waveguide or a microcavity. We show that the dipole gauge Hamiltonian automatically takes into account the Coulomb interactions in this system. Furthermore, it can be conveniently expressed in terms of the many-body collective plasmon modes, which interact both with each other and with the light field. The dipole gauge therefore provides a suitable framework for the study of solid state Quantum Electrodynamics (QED) phenomena, such as the ultra-strong light-matter interaction regime, occurring at very high electronic densities.

Superradiant Emission from a Collective Excitation in a Semiconductor.

We report an anomalous wide broadening of the emission spectra of an electronic excitation confined in a two-dimensional potential. We attribute these results to an extremely fast radiative decay rate associated with superradiant emission from the ensemble of confined electrons. Lifetimes extracted from the spectra are below 100 fs and, thus, 6 orders of magnitude faster than for single particle transitions at similar wavelength. Moreover, the spontaneous emission rate increases with the electronic density, as expected for superradiant emission. The data, all taken at 300 K, are in excellent agreement with our theoretical model, which takes into account dipole-dipole Coulomb interaction between electronic excitations. Our experimental results demonstrate that the interaction with infrared light, which is usually considered a weak perturbation, can be a very efficient relaxation mechanism for collective electronic excitations in solids.