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Featured researches published by Yaqian Zhao.


Environmental Science and Pollution Research | 2017

Erratum to: Effects of rapid temperature rising on nitrogen removal and microbial community variation of anoxic/aerobic process for ABS resin wastewater treatment

Huilong Luo; Yudong Song; Yuexi Zhou; Liwei Yang; Yaqian Zhao

ABS resin wastewater is a high-temperature nitrogenous organic wastewater. It can be successfully treated with anoxic/aerobic (A/O) process. In this study, the effect of temperature on nitrogen removal and microbial community after quick temperature rise (QTR) was investigated. It was indicated that QTR from 25 to 30xa0°C facilitated the microbial growth and achieved a similar effluent quality as that at 25xa0°C. QTR from 25 to 35xa0°C or 40xa0°C resulted in higher effluent concentration of chemical oxygen demand (COD), biochemical oxygen demand (BOD5), total nitrogen (TN), and total phosphorus (TP). Illumina MiSeq pyrosequencing analysis illustrated that the richness and diversity of the bacterial community was decreased as the temperature was increased. The percentage of many functional groups was changed significantly. QTR from 25 to 40xa0°C also resulted in the inhibition of ammonia oxidation rate and high concentration of free ammonia, which then inhibited the growth of NOB (Nitrospira), and thus resulted in nitrite accumulation. The high temperature above 35xa0°C promoted the growth of a denitrifying bacterial genus, Denitratisoma, which might increase N2O production during the denitrification process.


Geofluids | 2018

Effects of Dissolved Organic Matter on Sorption of Oxytetracycline to Sediments

Zongzhou Wang; Qianli Jiang; Runze Wang; Xiaoyu Yuan; Shengke Yang; Wenke Wang; Yaqian Zhao

The effects of two representative dissolved organic matters (DOMs) (derived from corrupt plants (PDOM) and chicken manure (MDOM)) on sorption characteristic of oxytetracycline to three typical sediments (first terrace (FT), river floodplain (RF), and riverbed (RB) sediments collected from the Weihe River) were investigated. Results showed that both DOMs can make the adsorption equilibrium time advance about 6 hours. The presence of DOMs changed the sorption kinetics model and the spontaneous degree of the reaction but did not change the sorption isotherm models. The adsorption of oxytetracycline (OTC) could be promoted by adding PDOM, and its maximum adsorption amount increased by 23.8% for FT, 38.0% for RB, and 28.3% for RF, respectively, whereas MDOM could inhibit the adsorption and maximum adsorption amount decreased by 23.3% for FT, 11.6% for RB, and 16.1% for RF, respectively. In addition, the DOM concentration also affected the adsorption. Overall, this study suggests that the humus-like DOM can promote the adsorption of OTC while the protein-like DOM can inhibit the adsorption of OTC to sediments, which is determined by the aromaticity, hydrophilicity, and polarity of the DOMs.


Environmental Science & Technology | 2018

Rethinking Intensification of Constructed Wetlands as a Green Eco-Technology for Wastewater Treatment

Shubiao Wu; Tao Lyu; Yaqian Zhao; Jan Vymazal; Carlos A. Arias; Hans Brix

Technology for Wastewater Treatment Shubiao Wu,*,†,‡ Tao Lyu, Yaqian Zhao, Jan Vymazal, Carlos A. Arias, and Hans Brix †College of Engineering, China Agricultural University, Beijing 100083, China ‡Aarhus Institute of Advanced Studies, Aarhus University, Høegh-Guldbergs Gade 6B, DK-8000 Aarhus C, Denmark School of Animal, Rural and Environmental Sciences, Nottingham Trent University, Nottinghamshire NG25 0QF, U.K. Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kymyćka ́ 129, 165 21 Praha 6, Czech Republic Centre for Water Resources Research, School of Civil Engineering, University College Dublin, Belfield, Dublin, 4, Ireland Department of Bioscience, Aarhus University, 8000 Aarhus C, Denmark


applied reconfigurable computing | 2018

An OpenCLTM Implementation of WebP Accelerator on FPGAs

Zhenhua Guo; Baoyu Fan; Yaqian Zhao; Xuelei Li; Shixin Wei; Long Li

With the development of cloud computing, the super-large scale of image data has bring severe challenges for the storage cost and network bandwidth in data centers. In order to alleviate the present situation effectively, WebP has replaced the current mainstream image file format due to its better compression efficiency. In this paper, we provide an OpenCL implementation of WebP accelerator on FPGAs to optimize the performance of WebP Lossy Compression Algorithm. Our accelerator makes use of a heavily-pipelined custom hardware implementation to achieve a high throughput ~450MPixel/s. The performance-per-watt of our OpenCL implementation on Intel’s Arria 10 device is 8.32x better than a highly-tuned CPU implementation on Intel Xeon E5-2690v3 with 24 thread cores. Additionally, the delay time per image can be reduced to ~90% by the data parallelism and macroblock pipelining on FPGAs. Finally, our OpenCLTM implementation of WebP accelerator on FPGAs is more competitive for data centers to achieve higher performance and lower cost.


Materials | 2018

Preparation of Parabolic Superhydrophobic Material for Oil-Water Separation

Xiaoying Qiao; Chunyan Yang; Qian Zhang; Shengke Yang; Yangyang Chen; Dan Zhang; Xiaoyu Yuan; Wenke Wang; Yaqian Zhao

In order to prepare parabolic superhydrophobic materials, copper meshes were used as the substrate and ultrasonic etching and oxidative corrosion were carried out with FeCl3 solution and H2O2 solution, respectively, and then the surface was modified with stearic acid (SA). The topological structure and surface wettability of the prepared mesh were characterized by fluorescence microscope, scanning electron microscopy and contact angle measurement. Finally, the as-prepared copper meshes were applied to oil-water separation. The results showed that the micro-nano-mastoid structure on the surface of the copper mesh was flaky bulges, forming a rough structure similar to a paraboloid. When the oxidative corrosion time of H2O2 was 1 min, it is more beneficial to increase the hydrophobicity of the surface of the copper mesh and increase the contact angle of water droplets on the surface of the membrane. Additionally, based on superhydrophobic materials of the parabolic copper mesh, the static contact angles of the water droplets, engine oil and carbon tetrachloride with the surface were approximately 153.6°, 5° and 0.1°, respectively and the sliding angle of the water droplets with the surface were approximately 4.9°. The parabolic membrane was applied to discuss the separation efficiency of different oils with deionized water and the separation efficiency was obtained as benzene > carbon tetrachloride > oil > machine oil. Therefore, based on the research, the parabolic superhydrophobic material has good efficiency of oil-water separation.


Journal of Hazardous Materials | 2018

Effects of long-lasting nitrogen and organic shock loadings on an engineered biofilter treating matured landfill leachate

Yidong Guan; Jun Zhou; Xiaoru Fu; Yaqian Zhao; Ancheng Luo; Jianqiang Xu; Jie Fu; Dongye Zhao

The decentralized bioreactor is a promising process for landfill leachate (LL) treatment, however, it is often confronted with various forms of shock loadings. To explore the robustness of bioreactors to the long-lasting substrate shocks, a long-term study of over 90 days was carried out to investigate the effects of nitrogen (mainly ammonium nitrogen, NH4-N) and organic (in terms of chemical oxygen demand, COD) shock loading on an engineered zeolite-based biofilter with alternative soil-mixed block (SMB) (EZS-biofilter) for treating matured LL. The low-, mid-, and high-strength intensity of matured LL was theoretical defined mainly according to the content of total nitrogen (TN) and COD. The experiment proved that the EZS-biofilter could effectively absorb the substrate shocks in a range of 104, 408, and 1357u2009mg/L as TN and 178, 590, and 1050u2009mg/L as COD, corresponding to the low-, medium-, and high-strength LL, respectively. A modified sensitivity index reflected that the nitrogen shock loadings exerted much more predominant influence than COD shock due to the great variation of nitrification/denitrification. The provided information in this study are beneficial for the practical engineered operation of biofilters for treating matured LL.


International Journal of Environmental Research and Public Health | 2018

Enhanced Nutrients Removal Using Reeds Straw as Carbon Source in a Laboratory Scale Constructed Wetland

Tong Wang; Haiyan Wang; Yang Chang; Zhaosheng Chu; Yaqian Zhao; Ranbin Liu

The low carbon/nitrogen (C/N) ratio and high nitrate content characteristics of agricultural runoff restricted the nitrogen removal in constructed wetlands (CWs). To resolve such problems, the economically- and easily-obtained Phragmites Australis (reeds) litters were applied and packed in the surface layer of a surface flow CW as external carbon sources. The results demonstrated that the introduction of the reeds straw increased the C concentration as a result of their decomposition during the CW operation, which will help the denitrification in the ensuing operation of an entire 148 days. The total nitrogen (TN) and Chemical Oxygen Demand (COD) () in the effluent reached the peak level of 63.2 mg/L and 83 mg/L at the fourth and the second day, respectively. Subsequently, the pollutants in the CW that were filled with straw decreased rapidly and achieved a stable removal after 13 days of operation. Moreover, the present study showed that the N removal efficiency increased with the increase of the hydraulic retention time (HRT). Under the HRT of four days, the CW presented 74.1 ± 6%, 87.4 ± 6% and 56.0 ± 6% removal for TN, NO3-, and TP, respectively.


International Journal of Environmental Research and Public Health | 2018

Interaction Mechanism between Antibiotics and Humic Acid by UV-Vis Spectrometry

Xiaoyu Yuan; Shengke Yang; Jie Fang; Xueli Wang; Haizhen Ma; Zongzhou Wang; Runze Wang; Yaqian Zhao

In this study, the interaction between the humus and two antibiotics was studied by UV-Vis spectroscopy to describe the interaction mechanism and the effects of different environmental factors on the mechanism. Results showed that humic acid (HA) containing more aromatic groups was easily associated with antibiotics. In the HA-OTC, with the increase of the concentration of OTC, there were obvious absorption peaks in the 230–260 nm and 330–360 nm range, and the absorption band of the HA ultraviolet spectrum underwent a slight blue shift and the absorption intensity increased, demonstrating that a new ground state complex was generated. In the HA-SD, with the increase of SD concentration, an aromatic structure absorption peak appeared in the 190–220 nm range, and the peak value increased and the absorption band underwent a red shift, and the aromatization of HA decreased, which enhanced the interaction between the antibiotics and HA. With the increase of pH, the absorption band of HA, HA-OTC and HA-SD ultraviolet spectrum suffered a blue shift, the degree of polymerization of HA molecules decreased, and the number of adsorption binding sites increased, which resulted in the interaction of HA with antibiotics being enhanced. The absorption band of HA, HA-OTC and HA-SD displayed a red shift with the increase of ionic strength, which indicated that the repulsion within HA particles was weakened, and the molecular polymerization was strengthened and therefore, the interaction between antibiotics and HA was inhibited. The UV characteristics of the HA, HA-OTC and HA-SD systems were insensitive to the temperature. This study lays the foundation for better studying the effect of humus on the distribution of antibiotic residues in the environment.


International Journal of Environmental Research and Public Health | 2018

Concentrations, Distributions, and Risk Assessment of HBCD in Sediment in the Weihe River Basin in Northwest China

Xueli Wang; Xiaoyu Yuan; Shengke Yang; Yaqian Zhao

As one of the most widely used brominated flame retardants, hexabromocyclododecane (HBCD) is found widely in the environmental media. In this study, the content and spatial distribution of HBCD and risk posed by HBCD in surface sediment in the Weihe River Basin in Northwest China were investigated. The HBCD concentration ranged nd–4.04 ng/g dw with the mean was 0.45 ng/g dw. The major source of HBCD in surface sediment was local point discharge. The distribution profiles of α-, β-, γ-HBCD were 24.7–87.9%, 0–42.0%, and 0–67.1%, respectively. Specially, α-HBCD was the dominating isomer in most sample sites. This differed significantly from that in HBCD technical product, which might be attributed to the different degradation rates and inter-transformation of the three HBCD isomers. Risk quotient method was used to assess the potential risk posed by HBCD in sediment. HBCD do not pose strong risks to aquatic algae organisms in the Weihe River Basin.


Environmental Science and Pollution Research | 2018

Achieving an extraordinary high organic and hydraulic loadings with good performance via an alternative operation strategy in a multi-stage constructed wetland system

X. H. Zhao; Yuansheng Hu; Yaqian Zhao; Lordwin Kumar

In this study, a high organic loading rate of 58–146xa0gxa0BOD5/m2xa0day with a hydraulic loading rate (HLR) of 1.63xa0m3/m2xa0day and retention time (RT) of 16xa0h was achieved to maximize the treatment capacity of a four-stage alum sludge-based constructed wetland (CW) system. An alternative operation strategy, i.e., the first stage anaerobic up-flow and the remaining stage tidal flow with effluent recirculation, was investigated to achieve the goal with good treatment performance of 82% COD, 91% BOD5, 92% SS, 94% NH4-N, and 82% TN removal. Two kinetic models, i.e., first-order model and Monod plus continuous stirred-tank reactor (CSTR) flow model, were employed for predicting the removal dynamics. The results showed that the tidal flow strategy enhances oxygen transport and diffusion, thus improving reduction of organics and NH4-N. Effluent recirculation could further increase elimination of organics by extending the interaction time and also benefit the denitrification process. In addition, denitrification could be further enhanced by anaerobic up-flow in the first stage.

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Wenzheng Yu

Imperial College London

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Lei Xu

University College Dublin

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Ranbin Liu

University College Dublin

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