Yoko Saito-Kokubu

Depositional records of plutonium and 137Cs released from Nagasaki atomic bomb in sediment of Nishiyama reservoir at Nagasaki

In a sediment core of Nishiyama reservoir at Nagasaki city, depth profiles of (240)Pu/(239)Pu isotopic ratio, (239+240)Pu and (137)Cs activities were determined. Sediments containing plutonium and (137)Cs, which were deposited immediately after a detonation of Nagasaki atomic bomb, were identified in the core. Observed below the sediments were macroscopic charcoals, providing evidence for initial deposit of the fallout of the Nagasaki atomic bomb. This is the first entire depositional records of plutonium and (137)Cs released from the Nagasaki atomic bomb together with those from atmospheric nuclear tests.

Seasonal and snowmelt-driven changes in the water-extractable organic carbon dynamics in a cool-temperate Japanese forest soil, estimated using the bomb-14C tracer

Water-extractable organic carbon (WEOC) in soil consists of a mobile and bioavailable portion of the dissolved organic carbon (DOC) pool. WEOC plays an important role in dynamics of soil organic carbon (SOC) and transport of radionuclides in forest soils. Although considerable research has been conducted on the importance of recent litter versus older soil organic matter as WEOC sources in forest soil, a more thorough evaluation of the temporal pattern of WEOC is necessary. We investigated the seasonal variation in WEOC in a Japanese cool-temperate beech forest soil by using the carbon isotopic composition ((14)C and (13)C) of WEOC as a tracer for the carbon sources. Our observations demonstrated that fresh leaf litter DOC significantly contributed to WEOC in May (35-52%) when the spring snowmelt occurred because of the high water flux and low temperature. In the rainy season, increases in the concentration of WEOC and the proportion of hydrophobic compounds were caused by high microbial activity under wetter conditions. From summer to autumn, the WEOC in the mineral soil horizons was also dominated by microbial release from SOC (>90%). These results indicate that the origin and dynamics of WEOC are strongly controlled by seasonal events such as the spring snowmelt and the rainy seasons intense rainfall.

Current R & D Activities in the Study on Geosphere Stability

The Japanese islands are located in a tectonically active zone. The scientific base is required for assessing the geosphere stability for long-term isolation of radioactive waste in Japan. JAEA is promoting the establishment of investigation method for geotectonic events affecting geosphere stability and prediction model for the future changes of geological environments, that is necessary for site selection and safety assessment of the HLW geological disposal. For seismicity and faulting, detection techniques for active faults without topographic surface expression, such as using helium isotope ratios in hot spring gases or detection of hydrogen gas, and studies on the assessment of fault evolution have been developed. For volcanism and geothermal activity, heat sources for anomalous geothermal activity in non-volcanic regions are considered. Detection techniques for high-temperature fluids and magma deep underground, using geophysical and geochemical approaches, were constructed. For uplift, denudation and climatic/sea-level changes, a methodology to predict the future topographic change was developed. Also, for dating techniques as an essential part to proceed on these studies, C-14 and Be-10 dating using AMS and (U-Th)/He dating using QMS and ICP-MS have been developed. We are planning the establishment of assessment methods for geosphere stability including assessment of the activity of faults encountered in underground excavations, development of long-term prediction model of volcanism and hydrothermal activities, and hydrogeological analyses considering topographic change.© 2010 ASME