Yoshiharu Urata

Difference-frequency terahertz-wave generation from 4-dimethylamino-N-methyl-4-stilbazolium-tosylate by use of an electronically tuned Ti:sapphire laser

Among nonlinear materials, the organic ionic salt crystal 4-dimethylamino- N -methyl-4-stilbazolium-tosylate (DAST) is known for its large nonlinearity. We generated a coherent terahertz (THz) wave, using DAST, from the difference frequency between two oscillating wavelengths of an electronically tuned Ti:sapphire laser. In LiNbO(3), LiTaO(3), KTiOPO(4), and GaP crystals, THz-wave generation was not observed under the same experimental conditions. This result proves the high efficiency of DAST crystals for generation of difference-frequency THz waves.

Thermal conductivity/diffusivity of Nd3+ doped GdVO4, YVO4, LuVO4, and Y3Al5O12 by temperature wave analysis

Thermal diffusivity and thermal conductivity of single crystals of Nd3+ doped GdVO4, YVO4, LuVO4, and Y3Al5O12 are precisely measured over a wide range of doping concentration from 0.5to15at.% by temperature wave analysis. Thermal diffusivity serves as the most sensitive parameter to detect the effect of doping on thermal properties, where Nd3+ doped GdVO4 exhibits a decrease in thermal diffusivity (it has changed about 20% in their values in the c axis) but an increase in heat capacity (only 1.7%). It has long been understood that the thermal conductivity of YVO4 is inferior to that of Y3Al5O12; however, the thermal conductivity of YVO4 in the c axis shows the highest value in all four crystals compared at 1at.% of Nd3+ doping concentration. Thermal conductivity exhibits a decrease (∝e−1∕2, e: mass variance) with an increase of doping concentration, that is characteristic of Klemens’ point defect model for the phonon scattering. In the numerical fitting, the anisotropic decrease of thermal conductivity i...

Efficient laser performance of N:dGdVO 4 crystals grown by the floating zone method

Efficient laser performance is demonstrated with Nd:GdVO4 crystals grown by the floating zone method. With a 2-at. % Nd-doped crystal a slope efficiency of 67% is achieved with pumping at 808 nm. We also find that pumping at 879 nm with a bandwidth of 1.8 nm is practical for laser diode pumping. With this pumping level the slope efficiency reaches 78%. High-quality Nd:GdVO4 crystals are successfully grown with as much as 15-at.% Nd concentration by the floating zone method without inclusions or macroscopic defects. Homogeneity and high reproducibility of crystal growth are confirmed.

808-nm diode-pumped continuous-wave Tm:GdVO4 laser at room temperature.

A high-quality gadolinium vanadate (GdVO4) crystal with 7-at. % thulium as the starting material was grown by the Czochralski technique. The measured absorption spectra exhibited sufficient absorption coefficients for laser diodes (LDs) for neodymium laser pumping: 6.0 cm(-1) for pi polarization and 6.2 cm(-1) for sigma polarization at 808 nm. Laser oscillation was carried out with single-stripe 808-nm LDs in an end-pumping configuration. A slope efficiency of 28% and a threshold of 750 mW were exhibited with respect to the absorbed pump power. An output power of 420 mW was achieved at an absorbed power of 2.4 W. It was demonstrated that Tm:GdVO4 is a useful material for 2-microm lasers, particularly in a compact LD-pumped system.

Fiber-like lanthanum tungstate crystal for efficient stimulated Raman scattering

A solid-state Raman material, fiber-shaped single crystal lanthanum tungstate (LWO) has been successfully grown by the micro-pulling-down method. The fiber-shaped LWO crystals yielded intense Stokes pulses with an energy shift of 940 cm−1. In stimulated Raman conversion, a conversion efficiency of 6.8% (internal efficiency of 37%) to the first Stokes wave was achieved.

Laser performance of highly neodymium-doped yttrium aluminum garnet crystals

The laser performance of highly neodymium-doped yttrium aluminum garnet (YAG) crystals is reported. In cw laser-diode pumping, a slope efficiency of 54% was achieved for a 2-at. %-doped sample, which was comparable with the slope efficiency of 55% of YVO(4) . The crystal also exhibited a slope efficiency of 64% under pulsed Ti:sapphire pumping. Such a high efficiency suggests a total cavity loss of ~1% , which is as low as that of commercially available 1-at. % YAG crystal. The excellent performance of the neodymium-doped YAG crystals indicates their high optical quality.

Numerical simulation and optimization of Q-switched 2 μm Tm,Ho:YLF laser

Numerical simulation suggests that for obtaining a giant (G) pulse from a 2.06 mum solid state Tm,Ho:YLF laser by the active Q-switching technique, the optimal Ho concentration will be higher than that used in normal operation. In simulations of 500 ns G-pulse generation maximal efficiency occurred at 6 % Tm and 1.0 % Ho, in contrast with 0.4% Ho found to be optimal for the normal pulse generation. Maximal energy output from Tm,Ho:YLF lasers can be achieved by incorporating a delay of about 0.7 ms between 0.5 ms 780 nm LD pulsed pumping and the start of Q-switched G-pulse operation.

Laser Performance of Neodymium-Doped Lanthanum Tungstate Crystals

We demonstrated the laser oscillation at 1.06 µm with neodymium-doped lanthanum tungstate crystals under pulsed-laser pumping at 802 nm. Fiber-shaped crystals with Nd concentration of up to 20 at.% were grown using the micro-pulling-down method. A maximum slope efficiency of 35% was achieved for a 3.2 at.%-doped sample at 1059 nm.

Thermo-optical modeling of high power operation of 2 μm codoped Tm,Ho solid-state lasers

The results of coupled thermo-optical modeling of Tm,Ho solid-state laser operation are reported. A rate dynamics model integrated together with a TEM00 distribution for the total number of stimulated photons is coupled with a two-dimensional time-dependent heat transfer model. The heat transfer model includes absorption, heat release, and transfer inside the crystal as well as the thermal effect of the spontaneously emitted infrared radiation. In water cooled crystal operation this radiation is shown to be absorbed within the water boundary layer, producing significant inhibition of dissipation of the heat released inside the crystal. This effect leads to crystal superheating and significant inhibition of laser energy output. Absorption loss, in particular, due to water vapor present in the cavity is found to decrease significantly laser pulse energy. Numerical results are compared to previous (Tm,Ho:yttrium lithium fluoride) and new (Tm,Ho:ceramic yttrium aluminum garnet) experimental data and discussed...

WIDELY TUNABLE, NARROW-LINEWIDTH, SUBNANOSECOND PULSE GENERATION IN AN ELECTRONICALLY TUNED TI:SAPPHIRE LASER

Widely tunable subnanosecond Ti:sapphire laser radiation pumped with a cw Q -switched laser-diode-pumped Nd:YAG laser has been demonstrated in a simple laser system with a configuration of variable cavity length. Laser wavelengths can be continuously tuned by adjustment of the rf of an intracavity acousto-optic tunable filter with a computer through the whole range of the laser gain. During tuning of the whole spectral range, there is no need to realign any optics in the laser, except for moving the mirror to track the change of the rf. The peak powers of the output pulses at a pump level of 300 mW are comparable with those of conventional tunable picosecond Ti:sapphire lasers at a cw pump level of almost 10 W.