Zhengqian Luo

Graphene-based passively Q-switched dual-wavelength erbium-doped fiber laser

We demonstrate a compact Q-switched dual-wavelength erbium-doped fiber (EDF) laser based on graphene as a saturable absorber (SA). By optically driven deposition of graphene on a fiber core, the SA is constructed and inserted into a diode-pumped EDF laser cavity. Also benefiting from the strong third-order optical nonlinearity of graphene to suppress the mode competition of EDF, a stable dual-wavelength Q-switching operation has been achieved using a two-reflection peak fiber Bragg grating as the external cavity mirror. The Q-switched EDF laser has a low pump threshold of 6.5 mW at 974 nm and a wide range of pulse-repetition rate from 3.3 to 65.9 kHz. The pulse duration and the pulse energy have been characterized. This is, to the best of our knowledge, the first demonstration of a graphene-based Q-switched laser.

1.06μm Q-switched ytterbium-doped fiber laser using few-layer topological insulator Bi 2 Se 3 as a saturable absorber

Passive Q-switching of an ytterbium-doped fiber (YDF) laser with few-layer topological insulator (TI) is, to the best of our knowledge, experimentally demonstrated for the first time. The few-layer TI: Bi₂Se₃ (2-4 layer thickness) is firstly fabricated by the liquid-phase exfoliation method, and has a low saturable optical intensity of 53 MW/cm² measured by the Z-scan technique. The optical deposition technique is used to induce the few-layer TI in the solution onto a fiber ferrule for successfully constructing the fiber-integrated TI-based saturable absorber (SA). By inserting this SA into the YDF laser cavity, stable Q-switching operation at 1.06 μm is achieved. The Q-switched pulses have the shortest pulse duration of 1.95 μs, the maximum pulse energy of 17.9 nJ and a tunable pulse-repetition-rate from 8.3 to 29.1 kHz. Our results indicate that the TI as a SA is also available at 1 μm waveband, revealing its potential as another broadband SA (like graphene).

1-, 1.5-, and 2-μm Fiber Lasers Q-Switched by a Broadband Few-Layer MoS 2 Saturable Absorber

We propose and demonstrate 1, 1.5, and 2 μm passively Q-switched fiber lasers by exploiting a few-layer Molybdenum sulfide (MoS2) polymer composite as broadband saturable absorber (SA), respectively. The few-layer MoS2 nanosheets are prepared by the liquid-phase exfoliation method, and are composited with polyvinyl alcohol (PVA). The PVA-MoS2 film is sandwiched between two fiber ferrules to form the fiber-compatible SA. The few-layer MoS2 not only shows good transparency from ultraviolet to mid-infrared spectral region, but also possesses the nonlinear saturable absorption. The modulation depth and saturation optical intensity of the PVA-MoS2 film are measured to be 1.6% and 13 MW/cm2 at 1566 nm by the balanced twin-detector technique, respectively. By further inserting the filmy PVA-MoS2 SA into the cavities of Yb-, Er- and Tm-doped fiber lasers, we achieve stable Q-switching operations at 1.06, 1.56, and 2.03 μm, respectively. The output characteristics of the Q-switched pulses at the three wavelengths have been investigated, respectively. The MoS2-based Q-switching enables the large pulse energy of ~1 μJ with a pulse width of 1.76 μs. This is, to the best of our knowledge, the first demonstration of MoS2 -based Q-switched fiber lasers in a wide wavelength range (from 1 to 2 μm). Our results experimentally confirm that the new-type 2-D material, few-layer MoS2, is a promising broadband SA to Q-switch fiber lasers covering all major wavelengths from near- to mid-infrared region.

Widely-tunable, passively Q-switched erbium-doped fiber laser with few-layer MoS2 saturable absorber

We propose and demonstrate a MoS2-based passively Q-switched Er-doped fiber laser with a wide tuning range of 1519.6-1567.7 nm. The few-layer MoS2 nano-platelets are prepared by the liquid-phase exfoliation method, and are then made into polymer-composite film to construct the fiber-compatible MoS2 saturable absorber (SA). It is measured at 1560 nm wavelength, that such MoS2 SA has the modulation depth of ∼ 2% and the saturable optical intensity of ∼ 10 MW/cm(2). By further inserting the filmy MoS2-SA into an Er-doped fiber laser, stable Q-switching operation with a 48.1 nm continuous tuning from S- to C-waveband is successfully achieved. The shortest pulse duration and the maximum pulse energy are 3.3 μs and 160 nJ, respectively. The repetition rate and the pulse duration under different operation conditions have been also characterized. To the best of our knowledge, it is the first demonstration of MoS2 Q-switched, widely-tunable fiber laser.

Topological-Insulator Passively Q-Switched Double-Clad Fiber Laser at 2

In this paper, Topological insulator (TI) Bi2Se3 as a saturable absorber (SA) is exploited to Q-switch fiber lasers at 2 μm wavelength for the first time. Few-layer TI:Bi 2Se 3 nanosheets in CS-HAc solution are prepared by the liquid-phase exfoliation method, and the thin 2-D structure with the thickness of 3-5 layers is well characterized. The open-aperture Z-scan experiment shows that the few-layer TI:Bi 2Se 3 has the saturable optical intensity of 41 MW/cm 2 at 800 nm and the modulation depth of 3.7%. The optical deposition technique is used to efficiently assemble the TI:Bi 2Se 3 nanosheets in the solution onto a fiber ferrule, therefore constructing a fiber-compatible TI-based SA (FC-TISA). By further inserting the FC-TISA into a diode-pumped Tm 3+-doped double-clad fiber laser (TM-DCFL), stable Q-switching operation at 1.98 μm is successfully achieved with the shortest pulse width of 4.18 μs and the tunable repetition rate from 8.4 to 26.8 kHz. In particular, the TM-DCFL can deliver large-energy Q-switched pulses with the pulse energy as high as 313 nJ (corresponding to average output power of 8.4 mW). Our results suggest that TI-based SA is suitable for pulsed laser operation in the eye-safe region of 2 μm, and potentially develops as an ultra-broadband photonics device.

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Bismuth selenide (Bi2Se3), a new topological insulator, has attracted much attention in recent years owing to its relatively simple band structure and large bulk band gap. Compared to bulk, few-layer Bi2Se3 is recently considered as a highly promising material. Here, we use a liquid-phase exfoliation method to prepare few-layer Bi2Se3 in N-methyl-2-pyrrolidone or chitosan acetic solution. The resulted few-layer Bi2Se3 dispersion demonstrates an interesting absorption in the visible light region, which is different from bulk Bi2Se3 without any absorption in this region. The absorption spectrum of few-layer Bi2Se3 depends on its size and layer number. At the same time, the nonlinear and saturable absorption of few-layer Bi2Se3 thin film in near infrared is also characterized well and further exploited to generate laser pulses by a passive Q-switching technique. Stable Q-switched operation is achieved with a lower pump threshold of 9.3 mW at 974 nm, pulse energy of 39.8 nJ and a wide range of pulse-repetition-rate from 6.2 to 40.1 kHz. Therefore, the few-layer Bi2Se3 may excite a potential applications in laser photonics and optoelectronic devices.

m Wavelength

We demonstrate the fabrication of graphene-deposited tapered fibers (GDTFs), which can be used as saturable absorbers (SAs) for pulsed lasers. The advantages of GDTF SAs include flexibility, all-fiber configuration, and high optical damage threshold. The fabrication process is based on the interaction of the evanescent field of a tapered fiber with graphene. By in situ monitoring the transmitted power, the deposition process can be controlled, and the GDTF with a desirable level of nonsaturable absorption loss can be fabricated. We also study the dynamic deposition process by employing different waist diameters of tapered fibers and the different deposition powers. The results show that the deposition time can be significantly shortened with stronger evanescent field by decreasing the taper diameter or increasing the deposition power. Furthermore, by exploiting the GDTF as an intracavity passive power modulating element, we demonstrate efficient Q-switched and mode-locked erbium-doped fiber lasers, respectively.

Preparation of few-layer bismuth selenide by liquid-phase-exfoliation and its optical absorption properties.

We have demonstrated a high-energy Q-switched double-clad thulium-doped fiber laser (TDFL) using a graphene-oxide-deposited tapered fiber (GODTF) device as a saturable absorber operating at a wavelength of 2 μm for the first time. Because of the side-interaction of the graphene-oxide with the evanescent field on the taper waist, the GODTF devices have potential for offering high laser damage threshold. Using a 788 nm laser diode as the pump source, the TDFL generated stable single transverse mode Q-switched pulses with a single pulse energy of 6.71 μJ (corresponding to an average power of 302 mW) at a wavelength of 2032 nm. This is significantly higher than the highest pulse energy/average power from any rare-earth-doped fiber lasers employing a graphene or graphene-oxide based Q-switch so far. The demonstrated TDFL in this paper represents an encouraging step towards the practical applications of graphene or graphene-oxide based Q-switched 2 μm TDFLs.

Evanescent-Light Deposition of Graphene Onto Tapered Fibers for Passive Q-Switch and Mode-Locker

We report on the first passively Q-switched Nd:YAlO₃ laser at ~1079.5 nm using MoS₂ as saturable absorber. The MoS₂ saturable absorber is fabricated by transferring the liquid-phase-exfoliated MoS₂ nanosheets onto a BK7 glass substrate. By inserting the glass MoS₂ saturable absorber into a plano-concave Nd:YAlO₃ laser cavity, we obtain a stable Q-switched laser operation with a maximum average output power of 0.26 W corresponding to a pulse repetition rate of 232.5 kHz, a pulse width of 227 ns and a pulse energy of about 1.11 μJ. The results experimentally confirm the promising application of the new kind of 2D material, few-layer MoS₂, in solid state lasers.

High-energy passively Q-switched 2 μm Tm 3+ -doped double-clad fiber laser using graphene-oxide-deposited fiber taper

We experimentally confirm that graphene within fiber laser cavities can generate four-wave-mixing (FWM) by observing the laser spectral broadening and the transition from the single-longitudinal-mode oscillation to multiple-longitudinal-mode one. Then, by simultaneously exploiting the graphene-induced nonlinear FWM and its super-broadband saturable absorption, we further achieve for the first time to the best of our knowledge, multiwavelength Q-switched Yb3+- or Er3+-doped fiber lasers at 1 μm and 1.5 μm wavebands, respectively. Simultaneous 23-wavelength Q-switching oscillation with a wavelength spacing of 0.2 nm is stably generated at 1.5 μm waveband. The multiwavelength Q-switched pulses have the minimum pulse duration of 2.5 μs, the maximum pulse energy of 72.5 nJ and a wide range of pulse-repetition-rate (PRR) from 2.8 to 63.0 kHz. At 1 μm waveband, we also obtain five-wavelength simultaneous lasing in Q-switching regime with the pulse duration of ~ 3 μs, pulse energy of 10.3 nJ and PRR between 39.8 and 56.2 kHz.