Zhi-Yuan Zhou

Single-photon-level quantum image memory based on cold atomic ensembles

A quantum memory is a key component for quantum networks, which will enable the distribution of quantum information. Its successful development requires storage of single-photon light. Encoding photons with spatial shape through higher-dimensional states significantly increases their information-carrying capability and network capacity. However, constructing such quantum memories is challenging. Here we report the first experimental realization of a true single-photon-carrying orbital angular momentum stored via electromagnetically induced transparency in a cold atomic ensemble. Our experiments show that the non-classical pair correlation between trigger photon and retrieved photon is retained, and the spatial structure of input and retrieved photons exhibits strong similarity. More importantly, we demonstrate that single-photon coherence is preserved during storage. The ability to store spatial structure at the single-photon level opens the possibility for high-dimensional quantum memories.

Quantum Storage of Orbital Angular Momentum Entanglement in an Atomic Ensemble

Constructing a quantum memory for a photonic entanglement is vital for realizing quantum communication and network. Because of the inherent infinite dimension of orbital angular momentum (OAM), the photons OAM has the potential for encoding a photon in a high-dimensional space, enabling the realization of high channel capacity communication. Photons entangled in orthogonal polarizations or optical paths had been stored in a different system, but there have been no reports on the storage of a photon pair entangled in OAM space. Here, we report the first experimental realization of storing an entangled OAM state through the Raman protocol in a cold atomic ensemble. We reconstruct the density matrix of an OAM entangled state with a fidelity of 90.3%±0.8% and obtain the Clauser-Horne-Shimony-Holt inequality parameter S of 2.41±0.06 after a programed storage time. All results clearly show the preservation of entanglement during the storage.

Generation of non-classical correlated photon pairs via a ladder-type atomic configuration: theory and experiment.

We experimentally generate a non-classical correlated two-color photon pair at 780 and 1529.4 nm in a ladder-type configuration using a hot 85Rb atomic vapor with the production rate of ~10(7)/s. The non-classical correlation between these two photons is demonstrated by strong violation of Cauchy-Schwarz inequality by the factor R = 48 ± 12. Besides, we experimentally investigate the relations between the correlation and some important experimental parameters such as the single-photon detuning, the powers of pumps. We also make a theoretical analysis in detail and the theoretical predictions are in reasonable agreement with our experimental results.

Orbital angular momentum photonic quantum interface

Light-carrying orbital angular momentum (OAM) has great potential in enhancing the information channel capacity in both classical and quantum optical communications. Long distance optical communication requires the wavelengths of light are situated in the low-loss communication windows, but most quantum memories currently being developed for use in a quantum repeater work at different wavelengths, so a quantum interface to bridge the wavelength gap is necessary. So far, such an interface for OAM-carried light has not been realized yet. Here, we report the first experimental realization of a quantum interface for a heralded single photon carrying OAM using a nonlinear crystal in an optical cavity. The spatial structures of input and output photons exhibit strong similarity. More importantly, single-photon coherence is preserved during up-conversion as demonstrated.

CW-pumped telecom band polarization entangled photon pair generation in a Sagnac interferometer

Polarization entangled photon pair source is widely used in many quantum information processing applications such as teleportation, quantum communications, quantum computation and high precision quantum metrology. We report on the generation of a continuous-wave pumped 1550 nm polarization entangled photon pair source at telecom wavelength using a type-II periodically poled KTiOPO(4) (PPKTP) crystal in a Sagnac interferometer. Hong-Ou-Mandel (HOM) interference measurement yields signal and idler photon bandwidth of 2.4 nm. High quality of entanglement is verified by various kinds of measurements, for example two-photon interference fringes, Bell inequality and quantum states tomography. The source can be tuned over a broad range against temperature or pump power without loss of visibilities. This source will be used in our future experiments such as generation of orbital angular momentum entangled source at telecom wavelength for quantum frequency up-conversion, entanglement based quantum key distributions and many other quantum optics experiments at telecom wavelengths.

Sum frequency generation with two orbital angular momentum carrying laser beams

The frequency sum of two laser beams carrying orbital angular momentum (OAM) in quasi-phase matching crystals was reported. The situations in which one beam carried OAM, the other was in Gaussian mode, and both beams carried OAM were studied in detail. The sum of the two beams’ OAM was demonstrated in the conversion process, which verified OAM conservation in the sum frequency generation process. We give an analytical expression for the frequency conversion of two OAM-carrying beams; the experimental results are well matched with the theoretical simulations. The methods shown here provide an effective way for OAM light generation. Our study is very promising in constructing hybrid OAM-based optical communication networks and all-optical spatial mode switching.Frequency sum of two light beams carrying orbital angular momentum (OAM) in quasi-phase matching crystals was reported for the first time. The situations in which one light carried OAM and the other is in Gaussian mode and both beams carried OAM were studied in detail. An arbitrary sum arithmetic of lights with OAM was demonstrated in the conversion process. Our study is very promising in constructing hybrid OAM-based optical communication networks and all optical switching.

Orbital angular momentum light frequency conversion and interference with quasi-phase matching crystals

Light with helical phase structures, carrying quantized orbital angular momentum (OAM), has many applications in both classical and quantum optics, such as high-capacity optical communications and quantum information processing. Frequency conversion is a basic technique to expand the frequency range of the fundamental light. The frequency conversion of OAM-carrying light gives rise to new physics and applications such as up-conversion detection of images and generation of high dimensional OAM entanglements. Quasi-phase matching (QPM) nonlinear crystals are good candidates for frequency conversion, particularly due to their high-valued effective nonlinear coefficients and no walk-off effect. Here we report the first experimental second-harmonic generation (SHG) of an OAM-carried light with a QPM crystal, where a UV light with OAM of 100 ℏ is generated. OAM conservation is verified using a specially designed interferometer. With a pump beam carrying an OAM superposition of opposite sign, we observe interesting interference phenomena in the SHG light; specifically, a photonics gear-like structure is obtained that gives direct evidence of OAM conservation, which will be very useful for ultra-sensitive angular measurements. Besides, we also develop a theory to reveal the underlying physics of the phenomena. The methods and theoretical analysis shown here are also applicable to other frequency conversion processes, such as sum frequency generation and difference-frequency generation, and may also be generalized to the quantum regime for single photons.

Light storage based on four-wave mixing and electromagnetically induced transparency in cold atoms

We performed an experiment to observe the storages of an input probe field and an idler field generated through an off-axis four-wave mixing (FWM) process via a double-lambda configuration in a cold atomic ensemble. We analyzed the underlying physics in detail and found that the retrieved idler field came from two parts if there was no single-photon detuning for pump pulse: part 1 was from the collective atomic spin (the input probe field, the coupling field and the pump field combined to generate the idle field through FWM, then the idler was stored through electromagnetically induced transparency.); part 2 was from the generated new FWM process during the retrieval process (the retrieved probe field, the coupling field and the pump field combined to generate a new FWM signal). If there was single-photon detuning for pump pulse, then the retrieved idler was mainly from part 2. The retrieved two fields exhibited damped oscillations with the same oscillatory period when a homogeneous external magnetic field was applied, which was caused by the Larmor spin precession. We also experimentally realized the storage and retrieval of an image of light using FWM for the first time. In which, an image was added into the input signal. After the storage, the retrieved idler beams and input signal carried the same image. This image storage technique holds promises for application in image processing, remote sensing and quantum communication.

Image transfer through two sequential four-wave-mixing processes in hot atomic vapor

Efficient wavelength conversion of images has many potential applications in optical communication, sensing, imaging, and quantum information fields. In this work, we report on here the first demonstration of an image transfer between the light of wavelength 780 nm and the light of wavelength 1530 nm by performing two sequential four-wave mixing processes in two different hot atomic rubidium vapor cells. Furthermore, we confirm the persistence of coherence of the input light during this sequential process experimentally. Our results may be useful to the research fields mentioned above.

Experimental realization of entanglement in multiple degrees of freedom between two quantum memories

Entanglement in multiple degrees of freedom has many benefits over entanglement in a single one. The former enables quantum communication with higher channel capacity and more efficient quantum information processing and is compatible with diverse quantum networks. Establishing multi-degree-of-freedom entangled memories is not only vital for high-capacity quantum communication and computing, but also promising for enhanced violations of nonlocality in quantum systems. However, there have been yet no reports of the experimental realization of multi-degree-of-freedom entangled memories. Here we experimentally established hyper- and hybrid entanglement in multiple degrees of freedom, including path (K-vector) and orbital angular momentum, between two separated atomic ensembles by using quantum storage. The results are promising for achieving quantum communication and computing with many degrees of freedom.