Zhongquan Nie

Spherical and sub-wavelength longitudinal magnetization generated by 4π tightly focusing radially polarized vortex beams

Based on the vector diffraction theory and the inverse Faraday effect, we numerically study the light-induced magnetization near the focus of a 4π high numerical aperture focusing configuration under the illumination of two counter- propagating radially polarized hollow Gaussian vortex beams. The simulated results demonstrate that, by selecting higher-order vortex beam modes (e.g. n=4with n - the beam order) and proper truncation parameter (e.g. β=1.75 with β- the ratio of the pupil radius to the incident beam waist), spherical and sub-wavelength longitudinal magnetization can be generated in the vicinity of focus. Such special magnetization feature is attributed to not only the interaction between optical vortices and the radially polarized beams, but also the completely destructive interference of azimuthal components and the constructive interference of the longitudinal component of the two counter-propagating radially polarized vortex beams. This spherical and sub-wavelength longitudinal magnetization distribution may be of interest for applications in all-optical magnetic recording and confocal and magnetic resonance microscopy.

Achievement and steering of light-induced sub-wavelength longitudinal magnetization chain

The light-induced magnetization distributions for a high numerical aperture focusing configuration with an azimuthally polarized Bessel-Gaussian beam modulated by optimized vortex binary filters are investigated based on the inverse Faraday effect. It is found that, by adjusting the radii of different rings of the single/ cascaded vortex binary filters, super-long (12λ) and sub-wavelength (0.416λ) longitudinal magnetization chain with single/dual channels can be achieved in the focal region. Such well-behaved magnetization trait is attributed to the mutual effect between the optical polarization singularities of the azimuthally polarized beam and single/cascaded spiral optical elements. In addition, we find that the displacement distance of the longitudinal magnetization chain is proportional to the phase difference between the inner circle and outer ring of the vortex binary filters, thus giving rise to the steerable magnetization chain. It is expected that the research outcomes can be applied in multiple atoms trapping and transport, multilayer magneto-optical data storage, fabrication of magnetic lattices for spin wave operation and development of ultra-compact optomagnetic devices.

Three-dimensional super-resolution longitudinal magnetization spot arrays

We demonstrate an all-optical strategy for realizing spherical three-dimensional (3D) super-resolution (∼λ3/22) spot arrays of pure longitudinal magnetization by exploiting a 4π optical microscopic setup with two high numerical aperture (NA) objective lenses, which focus and interfere two modulated vectorial beams. Multiple phase filters (MPFs) are designed via an analytical approach derived from the vectorial Debye diffraction theory to modulate the two circularly polarized beams. The system is tailored to constructively interfere the longitudinal magnetization components, while simultaneously destructively interfering the azimuthal ones. As a result, the magnetization field is not only purely longitudinal but also super-resolved in all three dimensions. Furthermore, the MPFs can be designed analytically to control the number and locations of the super-resolved magnetization spots to produce both uniform and nonuniform arrays in a 3D volume. Thus, an all-optical control of all the properties of light-induced magnetization spot arrays has been demonstrated for the first time. These results open up broad applications in magnetic-optical devices such as confocal and multifocal magnetic resonance microscopy, 3D ultrahigh-density magneto-optic memory, and light-induced magneto-lithography.

Creation of a three-dimensional super-resolution transversally polarized focal spot by 4π tight focusing of radially polarized vortex beams

The intensity profiles near the focus of a 4? high numerical aperture focusing configuration for two counter-propagating radially polarized hollow Gaussian (HG) vortex beams are examined numerically. Theoretical calculations manifest that, in contrast to the single-objective focusing system, a three-dimensional super-resolution focal spot with purely transverse polarization can be formed. Such an unusual pattern stems from combining the faultlessly destructive interference of the longitudinal component of the electric field with the constructive interference of the transverse components (azimuthal and radial components) created by the two counter-propagating radially polarized vortex beams, as well as benefits from the higher-order HG mode (e.g., n?=?4) to govern the aspect ratio of the focal spot. Moreover, the tolerances on focusing performance for modest displacement from the center of the HG beams with different orders are researched in detail. We expect that such a three-dimensional super-resolution field with transverse polarization can be extensively used in super-resolution confocal microscopy and three-dimensional high-density optical storage.

Formation of a sub-wavelength longitudinally polarized beam using a radially polarized controllable dark-hollow beam

On the basis of vector diffraction theory, the tightly focusing properties of radially polarized controllable dark-hollow (CDH) beams are examined theoretically. Calculation results demonstrate that by choosing the initial parameters of the proposed light beams suitably, a sub-wavelength (0.422λ) longitudinally polarized light beam with high beam quality (82.2%) can be formed without any filters. Meanwhile, we find that a relatively long depth of focus benefits from larger beam order. The dependence of the focal spot size on the parameters such as truncation parameter, variation constant, and beam order is also explored in detail. Moreover, an alternative method to generate the CDH beams is proposed.

Investigation of nonlinear dynamics in CdS by time-resolved nondegenerate pump–probe system with phase object

The time-resolved nondegenerate pump–probe system with phase object is employed for investigation of nonlinear absorption and refraction dynamics in CdS. The 532 nm laser beam with 21 ps duration is used as the excitation and the laser beams of 600 and 680 nm with 10 ps duration from optical parametric generation are used for probing. The experimental results at both probe wavelengths show free-carrier absorption and large free-carrier refraction along with two-photon absorption and bound electronic optical Kerr effect. By numerically fitting the experimental data based on the nondegenerate pump–probe theory, the nondegenerate two-photon absorption coefficient, the nondegenerate Kerr coefficient, the free-carrier decay time, the free-carrier absorptive cross-section and free-carrier refractive coefficient at different wavelengths are all determined.