A. D. Christianson

Unconventional superconductivity in Ba0.6K0.4Fe2As2 from inelastic neutron scattering

A new family of superconductors containing layers of iron arsenide has attracted considerable interest because of their high transition temperatures (Tc), some of which are >50 K, and because of similarities with the high-Tc copper oxide superconductors. In both the iron arsenides and the copper oxides, superconductivity arises when an antiferromagnetically ordered phase has been suppressed by chemical doping. A universal feature of the copper oxide superconductors is the existence of a resonant magnetic excitation, localized in both energy and wavevector, within the superconducting phase. This resonance, which has also been observed in several heavy-fermion superconductors, is predicted to occur when the sign of the superconducting energy gap takes opposite values on different parts of the Fermi surface, an unusual gap symmetry which implies that the electron pairing interaction is repulsive at short range. Angle-resolved photoelectron spectroscopy shows no evidence of gap anisotropy in the iron arsenides, but such measurements are insensitive to the phase of the gap on separate parts of the Fermi surface. Here we report inelastic neutron scattering observations of a magnetic resonance below Tc in Ba0.6K0.4Fe2As2, a phase-sensitive measurement demonstrating that the superconducting energy gap has unconventional symmetry in the iron arsenide superconductors.

Magnetism in Fe-based superconductors

In this review, we present a summary of experimental studies of magnetism in Fe-based superconductors. The doping dependent phase diagram shows strong similarities to the generic phase diagram of the cuprates. Parent compounds exhibit magnetic order together with a structural phase transition, both of which are progressively suppressed with doping, allowing superconductivity to emerge. The stripe-like spin arrangement of Fe moments in the magnetically ordered state shows identical in-plane structure for the RFeAsO (R = rare earth) and AFe(2)As(2) (A = Sr, Ca, Ba, Eu and K) parent compounds, notably different than the spin configuration of the cuprates. Interestingly, Fe(1 + y)Te orders with a different spin order despite having very similar Fermi surface topology. Studies of the spin dynamics of the parent compounds show that the interactions are best characterized as anisotropic three-dimensional interactions. Despite the room temperature tetragonal structure, analysis of the low temperature spin waves under the assumption of a Heisenberg Hamiltonian indicates strong in-plane anisotropy with a significant next-nearest-neighbor interaction. For the superconducting state, a resonance, localized in both wavevector and energy, is observed in the spin excitation spectrum as for the cuprates. This resonance is observed at a wavevector compatible with a Fermi surface nesting instability independent of the magnetic ordering of the relevant parent compound. The resonance energy (E(r)) scales with the superconducting transition temperature (T(C)) as E(r) ∼ 4.9k(B)T(C), which is consistent with the canonical value of ∼ 5k(B)T(C) observed for the cuprates. Moreover, the relationship between the resonance energy and the superconducting gap, Δ, is similar to that observed for many unconventional superconductors (E(r)/2Δ ∼ 0.64).

Two-dimensional resonant magnetic excitation in BaFe1.84Co0.16As2.

Inelastic neutron scattering measurements on single crystals of superconducting BaFe1.84Co0.16As2 reveal a magnetic excitation located at wave vectors (1/2 1/2 L) in tetragonal notation. On cooling below T_{C}, a clear resonance peak is observed at this wave vector with an energy of 8.6(0.5) meV, corresponding to 4.5(0.3) k_{B}T_{C}. This is in good agreement with the canonical value of 5 k_{B}T_{C} observed in the cuprates. The spectrum shows strong dispersion in the tetragonal plane but very weak dispersion along the c axis, indicating that the magnetic fluctuations are two dimensional in nature. This is in sharp contrast to the anisotropic three dimensional spin excitations seen in the undoped parent compounds.

Three-dimensional magnetic correlations in multiferroic LuFe2O4.

We present single crystal neutron diffraction measurements on multiferroic LuFe(2)O(4). Magnetic reflections are observed below transitions at 240 and 175 K indicating that the magnetic interactions in LuFe(2)O(4) are three-dimensional in character. The magnetic structure is refined as a ferrimagnetic spin configuration below the 240 K transition. Below 175 K a significant broadening of the magnetic peaks is observed along with the buildup of a diffuse component to the magnetic scattering.

Charge order in LuFe2O4: antiferroelectric ground state and coupling to magnetism

X-ray scattering by multiferroic LuFe2O4 is reported. Below 320 K, superstructure reflections indicate an incommensurate charge order with propagation close to (1/3 1/3 3/2). The corresponding charge configuration, also found by electronic structure calculations as most stable, contains polar Fe/O double layers with antiferroelectric stacking. Diffuse scattering at 360 K, with (1/3 1/3 0) propagation, indicates ferroelectric short-range correlations between neighboring double layers. The temperature dependence of the incommensuration indicates that charge order and magnetism are coupled.

Static and dynamic magnetism in underdoped superconductor BaFe1.92Co0.08As2.

We report neutron scattering measurements on single crystals of BaFe1.92Co0.08As2. The magnetic Bragg peak intensity is reduced by 6% upon cooling through TC. The spin dynamics exhibit a gap of 8 meV with anisotropic three-dimensional interactions. Below TC additional intensity appears at an energy of approximately 4.5(0.5) meV, similar to previous observations of a spin resonance in other Fe-based superconductors. No further gapping of the spin excitations is observed below TC for energies down to 2 meV. These observations suggest the redistribution of spectral weight from the magnetic Bragg position to a spin resonance, demonstrating the direct competition between static magnetic order and superconductivity.

Anisotropy of Thermal Conductivity and Possible Signature of the Fulde-Ferrell-Larkin-Ovchinnikov state in CeCoIn5

We have measured the thermal conductivity of the heavy-fermion superconductor

Phonon Self-Energy and Origin of Anomalous Neutron Scattering Spectra in SnTe and PbTe Thermoelectrics

\mathrm{Ce}\mathrm{Co}{\mathrm{In}}_{5}

Competing ferri- and antiferromagnetic phases in geometrically frustrated LuFe2O4.

in the vicinity of the upper critical field, with the magnetic field perpendicular to the

Magnetically Driven Metal-Insulator Transition in NaOsO3

c