A. Lacerda
Los Alamos National Laboratory
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Featured researches published by A. Lacerda.
Journal of Physics: Condensed Matter | 1998
Donald Anthony Gajewski; N. R. Dilley; Eric D. Bauer; Eric James Freeman; Ricky Chau; M. Brian Maple; David Mandrus; Brian C. Sales; A. Lacerda
The low temperature properties of polycrystalline samples of the filled skutterudites and , as well as the unfilled skutterudites and , have been investigated by means of electrical resistivity, specific heat and magnetic susceptibility measurements. The resistivity of exhibits a rather abrupt drop-off with decreasing temperature near 100 K; this drop-off temperature increases with increasing applied hydrostatic pressure, which is reminiscent of the onset of coherence in so-called Kondo lattice materials. The compounds and exhibit values of the electronic specific heat coefficient and Pauli susceptibility at low temperature which are enhanced over those of the lanthanum-filled and unfilled skutterudites. These quantities yield a Wilson ratio of order unity, which indicates that they both correspond to the properties of itinerant electrons. These transport, magnetic and thermodynamic properties suggest a moderately heavy fermion ground state in and .
Journal of Applied Physics | 1991
P.C. Canfield; J. D. Thompson; Ward P. Beyermann; A. Lacerda; M. F. Hundley; E. J. Peterson; Z. Fisk; Hans Rudolf Ott
Members of the RBiPt (R=Ce–Lu with the exceptions of Pm and Eu) series have been grown as single crystals. Magnetic susceptibility and electrical resistance have been measured on all members of the series, and specific heat measurements have been performed on representatives. The high temperature resistance uniformly changes from that of a small‐gap semiconductor or semimetal seen in NdBiPt to that of a heavy‐fermion metal seen in YbBiPt, which shows a linear coefficient of specific heat at low temperatures of 8 J/K2 mole. Further, the lighter rare earth members show an unusually sharp increase in their resistance associated with antiferromagnetic ordering at low temperatures.
Physical Review Letters | 2006
Vivien Zapf; Zocco D; Hansen Br; M. Jaime; N. Harrison; Cristian D. Batista; M. Kenzelmann; Ch. Niedermayer; A. Lacerda; A. Paduan-Filho
It has recently been suggested that the organic compound NiCl2-4SC(NH2)2 (DTN) undergoes field-induced Bose-Einstein condensation (BEC) of the Ni spin degrees of freedom. The Ni S = 1 spins exhibit three-dimensional XY antiferromagnetism above a critical field H(c1) approximately 2 T. The spin fluid can be described as a gas of hard-core bosons where the field-induced antiferromagnetic transition corresponds to Bose-Einstein condensation. We have determined the spin Hamiltonian of DTN using inelastic neutron diffraction measurements, and we have studied the high-field phase diagram by means of specific heat and magnetocaloric effect measurements. Our results show that the field-temperature phase boundary approaches a power-law H - H(c1) proportional variant T(alpha)(c) near the quantum critical point, with an exponent that is consistent with the 3D BEC universal value of alpha = 1.5.
Journal of Low Temperature Physics | 1990
Carley Paulsen; A. Lacerda; L. Puech; P. Haen; P. Lejay; J.L. Tholence; J. Flouquet; A. de Visser
Magnetization measurements performed below 1 K on a single-crystalline sample of the heavy fermion compound CeRu2Si2 are reported. The field variation of the linear term of the specific heat γ derived from these data (via a Maxwell relation) exhibits a large peak at the metamagnetic-like transition at B* (=7.7 atT → 0). Thermal-expansion measurements, show a drastic drop of the temperature where a Fermi liquid behavior is reached whenB →B*. Similar experiments performed on a single-crystalline Ce0.95La0.05Ru2Si2 sample show a broadening of all the anomalies atB* and a reduction of their intensities. These results strongly suggest that pure CeRu2Si2 approaches a magnetic instability atB* forT → 0.
Physical Review B | 2005
W.M. Yuhasz; N. A. Frederick; P.-C. Ho; N. P. Butch; B.J. Taylor; T. A. Sayles; M. B. Maple; J. B. Betts; A. Lacerda; P. Rogl; Gerald Giester
The filled skutterudite compound
Chemical Physics Letters | 2001
Myung-Hwa Jung; Marcelo Jaime; A. Lacerda; G. S. Boebinger; Won Nam Kang; Heon-Jung Kim; E. M. Choi; Sung-Ik Lee
\mathrm{Sm}{\mathrm{Os}}_{4}{\mathrm{Sb}}_{12}
Journal of Magnetism and Magnetic Materials | 1999
Sergey L. Bud'ko; Z. Islam; T. A. Wiener; I. R. Fisher; A. Lacerda; P. C. Canfield
was prepared in single-crystal form and characterized using x-ray diffraction, specific-heat, electrical resistivity, and magnetization measurements. The
Physical Review B | 2005
P.-C. Ho; W.M. Yuhasz; N. P. Butch; N. A. Frederick; T. A. Sayles; J. R. Jeffries; M. B. Maple; J. B. Betts; A. Lacerda; P. Rogl; Gerald Giester
\mathrm{Sm}{\mathrm{Os}}_{4}{\mathrm{Sb}}_{12}
Physical Review B | 2004
C. Capan; Andrea Bianchi; R. Movshovich; A. D. Christianson; A. Malinowski; M. F. Hundley; A. Lacerda; P. G. Pagliuso; John L. Sarrao
crystals have the
Physical Review B | 2001
S. L. Bud’ko; C. Petrovic; G. Lapertot; C. E. Cunningham; Paul C. Canfield; M-H. Jung; A. Lacerda
\mathrm{La}{\mathrm{Fe}}_{4}{\mathrm{P}}_{12}