Alexander Apolonski

Submicrometer axial resolution optical coherence tomography.

Optical coherence tomography (OCT) with unprecedented submicrometer axial resolution achieved by use of a photonic crystal fiber in combination with a compact sub-10-fs Ti:sapphire laser (Femtolasers Produktions) is demonstrated for what the authors believe is the first time. The emission spectrum ranges from 550 to 950 nm (lambda(c)=725 nm , P(out)=27 mW) , resulting in a free-space axial OCT resolution of ~0.75 mum , corresponding to ~0.5 mum in biological tissue. Submicrometer-resolution OCT is demonstrated in vitro on human colorectal adenocarcinoma cells HT-29. This novel light source has great potential for development of spectroscopic OCT because its spectrum covers the absorption bands of several biological chromophores.

Approaching the microjoule frontier with femtosecond laser oscillators

Broadening the ultrashort laser pulse in a Kerr-lens mode-locked laser by net positive round-trip group-delay dispersion has proven to be a powerful concept for scaling the pulse energy directly achievable with a femtosecond laser oscillator without external amplification. Drawing on this concept, we demonstrate here Ti : Sa chirped-pulse oscillators delivering sub-40 fs pulses of 0.5 μJ and 50 nJ energy at average power levels of 1 and 2.5 W (repetition rate: 2 and 50 MHz), respectively, which to the best of our knowledge constitute the highest pulse energy and average power achieved with a femtosecond ( 1015 W cm−2 (when focused down to ~1 μm2), both of which represent record values from a laser oscillator. These pulse parameters appear to be limited merely by the pump power available, affording promise of scaling chirped-pulse femtosecond Ti : Sa oscillators to microjoule pulse energies and—by simultaneous spectral broadening—towards peak power levels of several hundred megawatts.

Chirped-pulse oscillators: a route to high-power femtosecond pulses without external amplification

We demonstrate a Kerr-lens mode-locked Ti:sapphire oscillator that generates 130-nJ, 26-fs and 220-nJ, 30-fs pulses at a repetition rate of 11 MHz. The generation of stable broadband, high-energy pulses from an extended-cavity oscillator is achieved by the use of chirped multilayer mirrors to produce a small net positive dispersion over a broad spectral range. The resultant chirped picosecond pulses are compressed by a dispersive delay line that is external to the laser cavity. The demonstrated peak powers, in excess of 5 MW, are to our knowledge the highest ever achieved from a cw-pumped laser and are expected to be scalable to tens of megawatts by an increase in the pump power and (or) a decrease in the repetition rate. The demonstrated source permits micromachining of any materials under relaxed focusing conditions.

High-power 200 fs Kerr-lens mode-locked Yb:YAG thin-disk oscillator.

We demonstrate a power-scalable Kerr-lens mode-locked Yb:YAG thin-disk oscillator. It delivers 200 fs pulses at an average power of 17 W and a repetition rate of 40 MHz. At an increased (180 W) pump power level, the laser produces 270 fs 1.1 μJ pulses at an average power of 45 W (optical-to-optical efficiency of 25%). Semiconductor-saturable-absorber-mirror-assisted Kerr-lens mode locking (KLM) and pure KLM with a hard aperture show similar performance. To our knowledge, these are the shortest pulses achieved from a mode-locked Yb:YAG disk oscillator and this is the first demonstration of a Kerr-lens mode-locked thin-disk laser.

Monolithic carrier-envelope phase-stabilization scheme

A new scheme for stabilizing the carrier-envelope (CE) phase of a few-cycle laser pulse train is demonstrated. Self-phase modulation and difference-frequency generation in a single periodically poled lithium niobate crystal that transmits the main laser beam allows CE phase locking directly in the usable output. The monolithic scheme obviates the need for splitting off a fraction of the laser output for CE phase control, coupling into microstructured fiber, and separation and recombination of spectral components. As a consequence, the output yields 6-fs, 800-nm pulses with an unprecedented degree of short- and long-term reproducibility of the electric field waveform.

Self-stabilization of carrier-envelope offset phase by use of difference-frequency generation.

Self-stabilized carrier-envelope offset phase is achieved by use of difference-frequency (DF) generation. The spectrum from a Ti:sapphire oscillator is broadened in a photonic crystal fiber, and a DF (900 nm) between the blue component (490 nm) and the infrared component (1080 nm) is generated. The beat signal between the fundamental and the DF signal is clearly observed. The wavelength of the DF signal can be tuned down to 780 nm, and hence the signal can be used for injection seeding of a Ti:sapphire oscillator.

Power scaling of a high-repetition-rate enhancement cavity

A passive optical resonator is used to enhance the power of a pulsed 78 MHz repetition rate Yb laser providing 200 fs pulses. We find limitations relating to the achievable time-averaged and peak power, which we distinguish by varying the duration of the input pulses. An intracavity average power of 18 kW is generated with close to Fourier-limited pulses of 10 W average power. Beyond this power level, intensity-related effects lead to resonator instabilities, which can be removed by chirping the seed laser pulses. By extending the pulse duration in this way to 2 ps, we could obtain 72 kW of intracavity circulating power with 50 W of input power.

Approaching the microjoule frontier with femtosecond laser oscillators: theory and comparison with experiment

A detailed numerical analysis of heavily chirped pulses in the positive-dispersion regime (PDR) is presented on the basis of the distributed cubic–quintic generalized complex nonlinear Ginzburg–Landau equation. It is demonstrated that there are three main types of pulse spectra: truncated parabolic-top, Π- and M-shaped profiles. The strong chirp broadens the pulse spectrum up to 100 nm for a Ti:Sa oscillator, which provides compressibility of the picosecond pulse down to sub-30 fs. Since the picosecond pulse has a peak power lower than the self-focusing power inside a Ti:Sa crystal, the microjoule energies become directly available from a femtosecond oscillator. The influence of the third- and fourth-order dispersions on the pulse spectrum and stability is analysed. It is demonstrated that the dynamic gain saturation plays an important role in pulse stabilization. The common action of dynamic gain saturation, self-amplified modulation (SAM) and saturation of the SAM provides pulse stabilization inside the limited range of the positive group-delay dispersions (GDDs). Since the stabilizing action of the SAM cannot be essentially enhanced for a pure Kerr-lens mode-locking regime, a semiconductor saturable absorber is required for pulse energies of >0.7 μJ inside an oscillator. The basic results of the numerical analysis are in an excellent agreement with experimental data obtained from oscillators with repetition rates ranging from 50 to 2 MHz.

Sub-fs electron pulses for ultrafast electron diffraction

We present a new concept for an electron gun generating subrelativistic electron pulses with a duration down to the attosecond range. It is based on a cylindrical RF cavity (a so-called pill-box cavity) oscillating in its TM010 eigenmode with a photocathode triggered by a fs-laser pulse. Injecting electrons at an appropriate phase of the RF cycle compensates for their initial velocities and time delays and makes the electrons arrive at a target in a sub-fs temporal window. Such electron pulses will allow nuclear motion and electronic dynamics to be studied on an attosecond time scale.

Spectral shaping of supercontinuum in a cobweb photonic-crystal fiber with sub-20-fs pulses

Multiple approaches to generate a smooth, powerful, and stable supercontinuum in cobweb photonic-crystal fibers were undertaken by use of 18-fs pulses. These approaches include utilization of incident pulses with various chirp, power, and polarization states, as well as fibers with different lengths and core sizes. For long fibers (tens of centimeters) the supercontinuum contains a finely modulated structure that can be smoothed when the oscillator is in a regime of relaxation oscillations. Short fibers provide a supercontinuum free of gaps. By optimization of these parameters supercontinua exceeding one octave with modulations of less than 10 dB have been generated.