Anne Harth

Two-color pumped OPCPA system emitting spectra spanning 1.5 octaves from VIS to NIR

We present a two-color pumped OPCPA system which delivers an ultra-broadband spectrum spanning from 430 nm to 1.3 µm with a Fourier limited pulse duration of sub-3 fs and 1 µJ of pulse energy at a repetition rate of 200 kHz. All frequency components propagate on a common path, thus the spectral phase along the whole spectrum is well-defined. The inner part of the spectrum has been compressed to sub-5 fs pulses.

Controlled waveforms on the single-cycle scale from a femtosecond oscillator

We present an octave-spanning Ti:sapphire oscillator supporting Fourier-limited pulses as short as 3.7 fs. This laser system can be directly CEO-phase stabilized delivering an average output power of about 90 mW with a pulse duration of 4.4 fs. The phase-stabilization is realized without additional spectral broadening using an f-2f interferometer approach allowing for full control of the electric pulse field on a sub-femtosecond time-scale.

Impact of temporal, spatial and cascaded effects on the pulse formation in ultra-broadband parametric amplifiers

A 2 + 1 dimensional nonlinear pulse propagation model is presented, illustrating the weighting of different effects for the parametric amplification of ultra-broadband spectra in different regimes of energy scaling. Typical features in the distribution of intensity and phase of state-of-the-art OPA-systems can be understood by cascaded spatial and temporal effects.

Few-cycle femtosecond field synthesizer.

We report on an optical field synthesizer consisting of a CEO-phase stabilized octave-spanning Ti:sapphire laser oscillator, a double-LCD prism-based pulse shaper, and a SPIDER pulse characterization apparatus. This field synthesizer allows for generating pulses with durations as short as 3.6 fs and enables to control the electric field on a sub-cycle scale. Within the limits of the ultrabroad spectrum arbitrary spectral and temporal pulse shapes and pulse sequences can be realized. Together with the ability to stabilize the pulses with respect to their CEO-phase, this system forms a versatile tool for coherent control experiments of field sensitive processes and precision spectroscopy.

Nanoscale Imaging of Local Few-Femtosecond Near-Field Dynamics within a Single Plasmonic Nanoantenna

The local enhancement of few-cycle laser pulses by plasmonic nanostructures opens up for spatiotemporal control of optical interactions on a nanometer and few-femtosecond scale. However, spatially resolved characterization of few-cycle plasmon dynamics poses a major challenge due to the extreme length and time scales involved. In this Letter, we experimentally demonstrate local variations in the dynamics during the few strongest cycles of plasmon-enhanced fields within individual rice-shaped silver nanoparticles. This was done using 5.5 fs laser pulses in an interferometric time-resolved photoemission electron microscopy setup. The experiments are supported by finite-difference time-domain simulations of similar silver structures. The observed differences in the field dynamics across a single particle do not reflect differences in plasmon resonance frequency or dephasing time. They instead arise from a combination of retardation effects and the coherent superposition between multiple plasmon modes of the particle, inherent to a few-cycle pulse excitation. The ability to detect and predict local variations in the few-femtosecond time evolution of multimode coherent plasmon excitations in rationally synthesized nanoparticles can be used in the tailoring of nanostructures for ultrafast and nonlinear plasmonics.

Few-cycle oscillator pulse train with constant carrier-envelope- phase and 65 as jitter

We report on an octave-spanning Ti:sapphire laser oscillator stabilized to carrier-envelope-offset frequency zero, generating a pulse train with constant field profile for every pulse. Stabilization is realized using an extended self-referenced locking scheme enabling to lock the carrier envelope-offset phase with less than 65 attosecond rms timing jitter. The stabilized system features a pulse repetition rate of 100 MHz with pulses as short as 4.5 fs and 220 mW average output power. With this laser system it was possible for the first time to demonstrate a spectral interference pattern of 1011 oscillator pulses in an out-of-loop f-to-2f-interferometer.

Temporal and spatial effects inside a compact and CEP stabilized, few-cycle OPCPA system at high repetition rates

We present a compact and ultra-stable few-cycle OPCPA system. In two non-collinear parametric amplification stages pulse energies up to 17 µJ at 200 kHz repetition rate are obtained. Recompression of the broadband pulses down to 6.3 fs is performed with chirped mirrors leading to peak powers above 800 MW. The parametric amplification processes were studied in detail employing (2 + 1) dimensional numerical simulations and compared to experimental observations in terms of spectral shapes, pulse energy, spatial effects as well as delay dependent nonlinear mixing products. This gives new insights into the parametric process and design guidelines for high repetition rate OPCPA systems.

Photoionization in the time and frequency domain

Resetting the clock on photoemission The ability to produce attosecond pulses of light provides access to some of the fastest electronic processes occurring within atoms. Tracking the temporal dynamics of the photoemission process in which an atom absorbs a high-energy photon and the electron escapes has exposed a discrepancy between the initial experimental findings and subsequent theoretical modeling. Isinger et al. present an ultrafast process that can account for and distinguish the different contributions to the photoemission processes in neon atoms. The findings reveal an “electron shake-up” process that may explain the discrepancy, bringing closure to a 7-year discussion. Science, this issue p. 893 An ultrafast technique is developed that can disentangle the different processes in photoionization. Ultrafast processes in matter, such as the electron emission after light absorption, can now be studied using ultrashort light pulses of attosecond duration (10−18 seconds) in the extreme ultraviolet spectral range. The lack of spectral resolution due to the use of short light pulses has raised issues in the interpretation of the experimental results and the comparison with theoretical calculations. We determine photoionization time delays in neon atoms over a 40–electron volt energy range with an interferometric technique combining high temporal and spectral resolution. We spectrally disentangle direct ionization from ionization with shake-up, in which a second electron is left in an excited state, and obtain excellent agreement with theoretical calculations, thereby solving a puzzle raised by 7-year-old measurements.

High power ultra-widely tuneable femtosecond pulses from a non-collinear optical parametric oscillator (NOPO)

We present an ultra-widely tunable non-collinear optical parametric oscillator with an average output power of more than 3 W and a repetition frequency of 34 MHz. The system is pumped by the second harmonic of a femtosecond Yb:KLu(WO4)2 thin-disk laser oscillator. The wavelength of the signal pulse can be rapidly tuned over a wide range from the visible to the NIR just by scanning the resonator length.

Spatiotemporal characterization of ultrashort laser pulses using spatially resolved Fourier transform spectrometry

We present a method for characterizing ultrashort laser pulses in space and time, based on spatially resolved Fourier transform spectrometry. An unknown pulse is interfered with a delayed, spatially uniform reference on a CCD camera. The reference pulse is created by spatially filtering a portion of the unknown pulse. By scanning the delay between the two pulses, an interferogram is obtained at each pixel, allowing us to determine the spatially resolved phase difference between the unknown pulse and the reference pulse. High-resolution spatiotemporal characterization of an ultrashort pulse is demonstrated, and the sensitivity of the method to spatiotemporal coupling is shown for the case of a pulse with pulse front tilt.