Antoine De Wispelaere

Installation and calibration of Kayzero-assisted NAA in three Central European countries via a Copernicus project.

An account is given of the installation and calibration of k0-based NAA--assisted by the DSM Kayzero/Solcoi software package--at the KFKI-AEKI, Budapest, the NPI, Rez and the IJS, Ljubljana. Not only the calibration of the Ge-detectors and the irradiation facilities are discussed, but also other important topics such as gamma-spectrometric hard- and software, QC/QA of the IRMM-530 Al-Au flux monitor and the upgrade of the Kayzero/Solcoi code. The work was performed in the framework of a European Copernicus JRP, coordinated by the Laboratory of Analytical Chemistry, Gent, with DSM Research, Geleen, as the industrial partner.

On the Quality of ENSDF γ‐Ray Intensity Data for γ‐Ray Spectrometric Determination of Th and U and Their Decay Series Disequilibria, in the Assessment of the Radiation Dose Rate in Luminescence Dating of Sediments

In luminescence dating of sediments, one of the most interesting tools for the determination of the annual radiation dose is Ge γ‐ray spectrometry. Indeed, it yields information on both the content of the radioelements K, Th, and U, and on the occurrence — in geological times — of disequilibria in the Th and U decay series. In the present work, two methodological variants of the γ‐spectrometric analysis were tested, which largely depend on the quality of the nuclear decay data involved: (1) a parametric calibration of the sediment measurements, and (2) the correction for the heavy spectral interference of the 226Ra 186.2 keV peak by 235U at 185.7 keV. The performance of these methods was examined via the analysis of three Certified Reference Materials, with the introduction of γ‐ray intensity data originating from ENSDF. Relevant conclusions were drawn as to the accuracy of the data and their uncertainties quoted.