Axel Andre

Electromagnetically induced transparency with tunable single-photon pulses

Techniques to facilitate controlled interactions between single photons and atoms are now being actively explored. These techniques are important for the practical realization of quantum networks, in which multiple memory nodes that utilize atoms for generation, storage and processing of quantum states are connected by single-photon transmission in optical fibres. One promising avenue for the realization of quantum networks involves the manipulation of quantum pulses of light in optically dense atomic ensembles using electromagnetically induced transparency (EIT, refs 8, 9). EIT is a coherent control technique that is widely used for controlling the propagation of classical, multi-photon light pulses in applications such as efficient nonlinear optics. Here we demonstrate the use of EIT for the controllable generation, transmission and storage of single photons with tunable frequency, timing and bandwidth. We study the interaction of single photons produced in a ‘source’ ensemble of 87Rb atoms at room temperature with another ‘target’ ensemble. This allows us to simultaneously probe the spectral and quantum statistical properties of narrow-bandwidth single-photon pulses, revealing that their quantum nature is preserved under EIT propagation and storage. We measure the time delay associated with the reduced group velocity of the single-photon pulses and report observations of their storage and retrieval.

Universal Approach to Optimal Photon Storage in Atomic Media

We present a universal physical picture for describing storage and retrieval of photon wave packets in a Lambda-type atomic medium. This physical picture encompasses a variety of different approaches to pulse storage ranging from adiabatic reduction of the photon group velocity and pulse-propagation control via off-resonant Raman fields to photon-echo-based techniques. Furthermore, we derive an optimal control strategy for storage and retrieval of a photon wave packet of any given shape. All these approaches, when optimized, yield identical maximum efficiencies, which only depend on the optical depth of the medium.

Manipulating light pulses via dynamically controlled photonic band gap.

When a resonance associated with electromagnetically induced transparency in an atomic ensemble is modulated by an off-resonant standing light wave, a band of frequencies can appear for which light propagation is forbidden. We show that dynamic control of such a band gap can be used to coherently convert a propagating light pulse into a stationary excitation with nonvanishing photonic component. This can be accomplished with high efficiency and negligible noise even at the level of few-photon quantum fields thereby facilitating possible applications in quantum nonlinear optics and quantum information.

Nonlinear optics with stationary pulses of light.

We show that the recently demonstrated technique for generating stationary pulses of light [M. Bajcsy, A. S. Zibrov, and M. D. Lukin, Nature (London) 426, 638 (2003)] can be extended to localize optical pulses in all three spatial dimensions in a resonant atomic medium. This method can be used to dramatically enhance the nonlinear interaction between weak optical pulses. In particular, we show that an efficient Kerr-like interaction between two pulses can be implemented as a sequence of several purely linear optical processes. The resulting process may enable coherent interactions between single photon pulses.

Photon storage in {lambda}-type optically dense atomic media. I. Cavity model

In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)], we used a universal physical picture to optimize and demonstrate equivalence between a wide range of techniques for storage and retrieval of photon wave packets in {lambda}-type atomic media in free space, including the adiabatic reduction of the photon group velocity, pulse-propagation control via off-resonant Raman techniques, and photon-echo-based techniques. In the present paper, we perform the same analysis for the cavity model. In particular, we show that the retrieval efficiency is equal to C/(1+C) independent of the retrieval technique, where C is the cooperativity parameter. We also derive the optimal strategy for storage and, in particular, demonstrate that at any detuning one can store, with the optimal efficiency of C/(1+C), any smooth input mode satisfying TC{gamma}>>1 and a certain class of resonant input modes satisfying TC{gamma}{approx}1, where T is the duration of the input mode and 2{gamma} is the transition linewidth. In the two subsequent papers of the series, we present the full analysis of the free-space model and discuss the effects of inhomogeneous broadening on photon storage.

Shaping quantum pulses of light via coherent atomic memory.

We describe proof-of-principle experiments demonstrating a novel approach for generating pulses of light with controllable photon numbers, propagation direction, timing, and pulse shapes. The approach is based on preparation of an atomic ensemble in a state with a desired number of atomic spin excitations, which is later converted into a photon pulse. Spatiotemporal control over the pulses is obtained by exploiting long-lived coherent memory for photon states and Electromagnetically Induced Transparency in an optically dense atomic medium. Using photon counting experiments, we observe Electromagnetically Induced Transparency based generation and shaping of few-photon sub-Poissonian light pulses.

Stability of atomic clocks based on entangled atoms

We analyze the effect of realistic noise sources for an atomic clock consisting of a local oscillator that is actively locked to a spin-squeezed (entangled) ensemble of N atoms. We show that the use of entangled states can lead to an improvement of the long-term stability of the clock when the measurement is limited by decoherence associated with instability of the local oscillator combined with fluctuations in the atomic ensembles Bloch vector. Atomic states with a moderate degree of entanglement yield the maximal clock stability, resulting in an improvement that scales as N(1/6) compared to the atomic shot noise level.

Quantum control of light using electromagnetically induced transparency

We present an overview of recent theoretical and experimental work on the control of the propagation and quantum properties of light using electromagnetically induced transparency in atomic ensembles. Specifically, we discuss techniques for the generation and storage of few-photon quantum-mechanical states of light as well as novel approaches to manipulate weak pulses of light via enhanced nonlinear optical processes.

Atom correlations and spin squeezing near the Heisenberg limit: Finite-size effect and decoherence

We analyze a model for spin squeezing based on the so-called countertwisting Hamiltonian, including the effects of dissipation and finite system size. We discuss the conditions under which the Heisenberg limit, i.e., phase sensitivity 1/N, can be achieved. A specific implementation of this model based on atom-atom interactions via quantized photon exchange is presented in detail. The resulting excitation corresponds to the creation of spin-flipped atomic pairs and can be used for fast generation of entangled atomic ensembles, spin squeezing, and applications in quantum information processing. The conditions for achieving strong spin squeezing with this mechanism are also analyzed.

Photon storage in {lambda}-type optically dense atomic media. III. Effects of inhomogeneous broadening

In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)] and in the two preceding papers [Gorshkov et al., this issue, Phys. Rev. A 76, 033804 (2006); 76, 033805 (2006)], we used a universal physical picture to optimize and demonstrate equivalence between a wide range of techniques for storage and retrieval of photon wave packets in homogeneously broadened