A. S. Zibrov

Nanoscale magnetic sensing with an individual electronic spin in diamond

Detection of weak magnetic fields with nanoscale spatial resolution is an outstanding problem in the biological and physical sciences. For example, at a distance of 10 nm, the spin of a single electron produces a magnetic field of about 1 μT, and the corresponding field from a single proton is a few nanoteslas. A sensor able to detect such magnetic fields with nanometre spatial resolution would enable powerful applications, ranging from the detection of magnetic resonance signals from individual electron or nuclear spins in complex biological molecules to readout of classical or quantum bits of information encoded in an electron or nuclear spin memory. Here we experimentally demonstrate an approach to such nanoscale magnetic sensing, using coherent manipulation of an individual electronic spin qubit associated with a nitrogen-vacancy impurity in diamond at room temperature. Using an ultra-pure diamond sample, we achieve detection of 3 nT magnetic fields at kilohertz frequencies after 100 s of averaging. In addition, we demonstrate a sensitivity of 0.5 μT Hz-1/2 for a diamond nanocrystal with a diameter of 30 nm.

ULTRASLOW GROUP VELOCITY AND ENHANCED NONLINEAR OPTICAL EFFECTS IN A COHERENTLY DRIVEN HOT ATOMIC GAS

We report the observation of small group velocities of order 90 meters per second, and large group delays of greater than 0.26 ms, in an optically dense hot rubidium gas (≈ 360 K). Media of this kind yield strong nonlinear interactions between very weak optical fields, and very sharp spectral features. The result is in agreement with previous studies on nonlinear spectroscopy of dense coherent media.

Quantum Register Based on Individual Electronic and Nuclear Spin Qubits in Diamond

The key challenge in experimental quantum information science is to identify isolated quantum mechanical systems with long coherence times that can be manipulated and coupled together in a scalable fashion. We describe the coherent manipulation of an individual electron spin and nearby individual nuclear spins to create a controllable quantum register. Using optical and microwave radiation to control an electron spin associated with the nitrogen vacancy (NV) color center in diamond, we demonstrated robust initialization of electron and nuclear spin quantum bits (qubits) and transfer of arbitrary quantum states between them at room temperature. Moreover, nuclear spin qubits could be well isolated from the electron spin, even during optical polarization and measurement of the electronic state. Finally, coherent interactions between individual nuclear spin qubits were observed and their excellent coherence properties were demonstrated. These registers can be used as a basis for scalable, optically coupled quantum information systems.

Quantum entanglement between an optical photon and a solid-state spin qubit

Quantum entanglement is among the most fascinating aspects of quantum theory. Entangled optical photons are now widely used for fundamental tests of quantum mechanics and applications such as quantum cryptography. Several recent experiments demonstrated entanglement of optical photons with trapped ions, atoms and atomic ensembles, which are then used to connect remote long-term memory nodes in distributed quantum networks. Here we realize quantum entanglement between the polarization of a single optical photon and a solid-state qubit associated with the single electronic spin of a nitrogen vacancy centre in diamond. Our experimental entanglement verification uses the quantum eraser technique, and demonstrates that a high degree of control over interactions between a solid-state qubit and the quantum light field can be achieved. The reported entanglement source can be used in studies of fundamental quantum phenomena and provides a key building block for the solid-state realization of quantum optical networks.

Electromagnetically induced transparency with tunable single-photon pulses

Techniques to facilitate controlled interactions between single photons and atoms are now being actively explored. These techniques are important for the practical realization of quantum networks, in which multiple memory nodes that utilize atoms for generation, storage and processing of quantum states are connected by single-photon transmission in optical fibres. One promising avenue for the realization of quantum networks involves the manipulation of quantum pulses of light in optically dense atomic ensembles using electromagnetically induced transparency (EIT, refs 8, 9). EIT is a coherent control technique that is widely used for controlling the propagation of classical, multi-photon light pulses in applications such as efficient nonlinear optics. Here we demonstrate the use of EIT for the controllable generation, transmission and storage of single photons with tunable frequency, timing and bandwidth. We study the interaction of single photons produced in a ‘source’ ensemble of 87Rb atoms at room temperature with another ‘target’ ensemble. This allows us to simultaneously probe the spectral and quantum statistical properties of narrow-bandwidth single-photon pulses, revealing that their quantum nature is preserved under EIT propagation and storage. We measure the time delay associated with the reduced group velocity of the single-photon pulses and report observations of their storage and retrieval.

Stationary pulses of light in an atomic medium

Physical processes that could facilitate coherent control of light propagation are under active exploration. In addition to their fundamental interest, these efforts are stimulated by practical possibilities, such as the development of a quantum memory for photonic states. Controlled localization and storage of photonic pulses may also allow novel approaches to manipulating of light via enhanced nonlinear optical processes. Recently, electromagnetically induced transparency was used to reduce the group velocity of propagating light pulses and to reversibly map propagating light pulses into stationary spin excitations in atomic media. Here we describe and experimentally demonstrate a technique in which light propagating in a medium of Rb atoms is converted into an excitation with localized, stationary electromagnetic energy, which can be held and released after a controllable interval. Our method creates pulses of light with stationary envelopes bound to an atomic spin coherence, offering new possibilities for photon state manipulation and nonlinear optical processes at low light levels.

Efficient all-optical switching using slow light within a hollow fiber

We demonstrate a fiber-optical switch that is activated at tiny energies corresponding to a few hundred optical photons per pulse. This is achieved by simultaneously confining both photons and a small laser-cooled ensemble of atoms inside the microscopic hollow core of a single-mode photonic-crystal fiber and using quantum optical techniques for generating slow light propagation and large nonlinear interaction between light beams.

Repetitive Readout of a Single Electronic Spin via Quantum Logic with Nuclear Spin Ancillae

Extending Quantum Memory Quantum information processing and communication relies on the ability to store, retrieve, and manipulate information stored in quantum memories. In most practical instances, however, the stored quantum information is fragile and susceptible to loss during readout. Jiang et al. (p. 267, published online 10 September) used a combination of quantum logic operations on the electronic spin of a nitrogen vacancy center in diamond to control its interactions with a nearby set of proximal nuclear spins of the carbon network. In this setup, the quantum memory of the electron spin could be made more robust. Extending the lifetime and allowing multiple readouts of the quantum memory should prove a useful technique for quantum information processing. Controlled interactions with nearby nuclear spins help improve the quantum memory of a nitrogen vacancy in diamond. Robust measurement of single quantum bits plays a key role in the realization of quantum computation and communication as well as in quantum metrology and sensing. We have implemented a method for the improved readout of single electronic spin qubits in solid-state systems. The method makes use of quantum logic operations on a system consisting of a single electronic spin and several proximal nuclear spin ancillae in order to repetitively readout the state of the electronic spin. Using coherent manipulation of a single nitrogen vacancy center in room-temperature diamond, full quantum control of an electronic-nuclear system consisting of up to three spins was achieved. We took advantage of a single nuclear-spin memory in order to obtain a 10-fold enhancement in the signal amplitude of the electronic spin readout. We also present a two-level, concatenated procedure to improve the readout by use of a pair of nuclear spin ancillae, an important step toward the realization of robust quantum information processors using electronic- and nuclear-spin qubits. Our technique can be used to improve the sensitivity and speed of spin-based nanoscale diamond magnetometers.

Coupling a Single Trapped Atom to a Nanoscale Optical Cavity

Trapped and Coupled Trapped single atoms are ideal for storing and manipulating quantum information. Thompson et al. (p. 1202, published online 25 April; see the Perspective by Keller) were able to control single atoms interacting coherently with a field mode of a photonic crystal cavity. An optical tweezer was used to trap the single atom, which enabled positioning of the atom in close proximity to the photonic crystal waveguide, coupling the atom to the optical mode of the cavity. Such coupling should prove useful in quantum measurement, sensing, and information processing. A single rubidium atom is positioned in close proximity to an optical cavity so they can interact. [Also see Perspective by Keller] Hybrid quantum devices, in which dissimilar quantum systems are combined in order to attain qualities not available with either system alone, may enable far-reaching control in quantum measurement, sensing, and information processing. A paradigmatic example is trapped ultracold atoms, which offer excellent quantum coherent properties, coupled to nanoscale solid-state systems, which allow for strong interactions. We demonstrate a deterministic interface between a single trapped rubidium atom and a nanoscale photonic crystal cavity. Precise control over the atoms position allows us to probe the cavity near-field with a resolution below the diffraction limit and to observe large atom-photon coupling. This approach may enable the realization of integrated, strongly coupled quantum nano-optical circuits.

Free-Standing Mechanical and Photonic Nanostructures in Single-Crystal Diamond

A variety of nanoscale photonic, mechanical, electronic, and optoelectronic devices require scalable thin film fabrication. Typically, the device layer is defined by thin film deposition on a substrate of a different material, and optical or electrical isolation is provided by the material properties of the substrate or by removal of the substrate. For a number of materials this planar approach is not feasible, and new fabrication techniques are required to realize complex nanoscale devices. Here, we report a three-dimensional fabrication technique based on anisotropic plasma etching at an oblique angle to the sample surface. As a proof of concept, this angled-etching methodology is used to fabricate free-standing nanoscale components in bulk single-crystal diamond, including nanobeam mechanical resonators, optical waveguides, and photonic crystal and microdisk cavities. Potential applications of the fabricated prototypes range from classical and quantum photonic devices to nanomechanical-based sensors and actuators.