Christoph Deutsch

Reversing the pump dependence of a laser at an exceptional point.

When two resonant modes in a system with gain or loss coalesce in both their resonance position and their width, a so-called exceptional point occurs, which acts as a source of non-trivial physics in a diverse range of systems. Lasers provide a natural setting to study such non-Hermitian degeneracies, as they feature resonant modes and a gain material as their basic constituents. Here we show that exceptional points can be conveniently induced in a photonic molecule laser by a suitable variation of the applied pump. Using a pair of coupled microdisk quantum cascade lasers, we demonstrate that in the vicinity of these exceptional points the coupled laser shows a characteristic reversal of its pump dependence, including a strongly decreasing intensity of the emitted laser light for increasing pump power.

High power terahertz quantum cascade lasers with symmetric wafer bonded active regions

We increased the active region/waveguide thickness of terahertz quantum cascade lasers with semi-insulating surface plasmon waveguides by stacking two symmetric active regions on top of each other, via a direct wafer bonding technique. In this way, we enhance the generated optical power in the cavity and the mode confinement. We achieved 470 mW peak output power in pulsed mode from a single facet at a heat sink temperature of 5 K and a maximum operation temperature of 122 K. Furthermore, the devices show a broad band emission spectrum over a range of 420 GHz, centered around 3.9 THz.

Vertically emitting terahertz quantum cascade ring lasers

We describe the fabrication and operation of vertically emitting distributed feedback quantum cascade ring lasers operating in the terahertz frequency range. A twofold increase in radiation efficiency is observed as compared to Fabry–Perot lasers. The emitters exhibit a robust single-mode operation around 3.2 THz with a side mode suppression ratio higher than 30 dB. Modal and threshold characteristics are investigated by performing finite element simulations with results in good agreement with experiments. The ring-shaped resonator facilitates beam collimation which results in a symmetric far-field profile.

Gain and losses in THz quantum cascade laser with metal-metal waveguide.

Coupling of broadband terahertz pulses into metal-metal terahertz quantum cascade lasers is presented. Mode matched terahertz transients are generated on the quantum cascade laser facet of subwavelength dimension. This method provides a full overlap of optical mode and active laser medium. A longitudinal optical-phonon depletion based active region design is investigated in a coupled cavity configuration. Modulation experiments reveal spectral gain and (broadband) losses. The observed gain shows high dynamic behavior when switching from loss to gain around threshold and is clamped at total laser losses.

Terahertz quantum cascade lasers based on type II InGaAs/GaAsSb/InP

We report the demonstration of a terahertz quantum cascade laser based on the In0.53Ga0.47As/GaAs0.51Sb0.49 type II material system. The combination of low effective electron masses and a moderate conduction band offset makes this material system highly suitable for such devices. The active region is a three-well phonon depopulation design and laser ridges have been processed in a double-metal waveguide configuration. The devices exhibit a threshold current density of 2 kA/cm2, provide peak optical powers of 1.8 mW, and operate up to 102 K. Emission frequencies are in the range between 3.6 and 4.2 THz.

High performance InGaAs/GaAsSb terahertz quantum cascade lasers operating up to 142 K

We report on the demonstration of a maximum operating temperature of 142 K for InGaAs-based terahertz quantum cascade lasers. This result is achieved by using the alternative material combination In0.53Ga0.47As/GaAs0.51Sb0.49, lattice-matched to InP, which exhibits fabrication advantages over standard In0.53Ga0.47As/In0.52Al0.48As due to more suitable material parameters. An active region, based on a three-well phonon depletion design, with improved injection and extraction tunneling coupling, was designed. The devices exhibit threshold current densities of 0.75 kA/cm2 and provide peak optical powers up to 9 mW. A broad spectral emission range between 3.3 and 4 THz is measured.

Probing scattering mechanisms with symmetric quantum cascade lasers.

A characteristic feature of quantum cascade lasers is their unipolar carrier transport. We exploit this feature and realize nominally symmetric active regions for terahertz quantum cascade lasers, which should yield equal performance with either bias polarity. However, symmetric devices exhibit a strongly bias polarity dependent performance due to growth direction asymmetries, making them an ideal tool to study the related scattering mechanisms. In the case of an InGaAs/GaAsSb heterostructure, the pronounced interface asymmetry leads to a significantly better performance with negative bias polarity and can even lead to unidirectionally working devices, although the nominal band structure is symmetric. The results are a direct experimental proof that interface roughness scattering has a major impact on transport/lasing performance.

Terahertz active photonic crystals for condensed gas sensing.

The terahertz (THz) spectral region, covering frequencies from 1 to 10 THz, is highly interesting for chemical sensing. The energy of rotational and vibrational transitions of molecules lies within this frequency range. Therefore, chemical fingerprints can be derived, allowing for a simple detection scheme. Here, we present an optical sensor based on active photonic crystals (PhCs), i.e., the pillars are fabricated directly from an active THz quantum-cascade laser medium. The individual pillars are pumped electrically leading to laser emission at cryogenic temperatures. There is no need to couple light into the resonant structure because the PhC itself is used as the light source. An injected gas changes the resonance condition of the PhC and thereby the laser emission frequency. We achieve an experimental frequency shift of 10−3 times the center lasing frequency. The minimum detectable refractive index change is 1.6 × 10−5 RIU.

Direct frequency comb measurement of OD + CO → DOCO kinetics

Combing through CO oxidation kinetics Carbon monoxide reacts with OH radicals to produce CO2. This process is central to combustion and atmospheric oxidation chemistry. The reaction sequence is widely assumed to involve the intermediacy of a HOCO adduct that has eluded direct monitoring under thermal conditions. Bjork et al. successfully observed the formation of the deuterated analog of this intermediate, DOCO, while simultaneously monitoring OD by using a multifrequency infrared comb. The results confirm the termolecular nature of the formation mechanism and its sensitivity to the ambient bath gas. Science, this issue p. 444 A broadband frequency comb tracks the kinetics of a previously elusive intermediate in the oxidation of carbon monoxide to carbon dioxide The kinetics of the hydroxyl radical (OH) + carbon monoxide (CO) reaction, which is fundamental to both atmospheric and combustion chemistry, are complex because of the formation of the hydrocarboxyl radical (HOCO) intermediate. Despite extensive studies of this reaction, HOCO has not been observed under thermal reaction conditions. Exploiting the sensitive, broadband, and high-resolution capabilities of time-resolved cavity-enhanced direct frequency comb spectroscopy, we observed deuteroxyl radical (OD) + CO reaction kinetics and detected stabilized trans-DOCO, the deuterated analog of trans-HOCO. By simultaneously measuring the time-dependent concentrations of the trans-DOCO and OD species, we observed unambiguous low-pressure termolecular dependence of the reaction rate coefficients for N2 and CO bath gases. These results confirm the HOCO formation mechanism and quantify its yield.

Random lasers for broadband directional emission

Broadband coherent light sources are becoming increasingly important for sensing and spectroscopic applications, especially in the mid-infrared and terahertz (THz) spectral regions, where the unique absorption characteristics of a whole host of molecules are located. The desire to miniaturize such light emitters has recently lead to spectacular advances with compact on-chip lasers that cover both of these spectral regions. The long wavelength and the small size of the sources result in a strongly diverging laser beam that is difficult to focus on the target that one aims to perform spectroscopy with. Here, we introduce an unconventional solution to this vexing problem relying on a random laser to produce coherent broadband THz radiation as well as an almost diffraction limited far-field emission profile. Our random lasers do not require any fine-tuning and thus constitute a promising example of practical device applications for random lasing.